Z-Schematic and visible-light-driven CO2 reduction using H2O as an electron donor by a particulate mixture of a Ru-complex/(CuGa)1−xZn2xS2 hybrid catalyst, BiVO4 and an electron mediator

Visible-light-driven Z-schematic CO2 reduction using H2O as an electron donor was achieved using a simple mixture of a metal-sulfide/molecular hybrid photocatalyst for CO2 reduction, a water oxidation photocatalyst and a redox-shuttle electron mediator. This is the first demonstration of a highly se...

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Bibliographic Details
Published in:Chemical communications (Cambridge, England) England), 2018, Vol.54 (72), p.10199-10202
Main Authors: Suzuki, Tomiko M, Yoshino, Shunya, Takayama, Tomoaki, Iwase, Akihide, Kudo, Akihiko, Morikawa, Takeshi
Format: Article
Language:English
Subjects:
Carbon dioxide
Electrons
Oxidation
Photocatalysts
Reduction
Online Access:Get full text
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Summary:Visible-light-driven Z-schematic CO2 reduction using H2O as an electron donor was achieved using a simple mixture of a metal-sulfide/molecular hybrid photocatalyst for CO2 reduction, a water oxidation photocatalyst and a redox-shuttle electron mediator. This is the first demonstration of a highly selective particulate CO2 reduction system accompanying O2 generation utilizing a semiconductor/molecular hybrid photocatalyst.
ISSN:1359-7345
1364-548X
DOI:10.1039/c8cc05505j