Iron(II) Metal–Organic Framework with unh Topology and Tetrazole-Padded Helical Channels

A unique metal–organic framework (MOF) with tetrazole-padded helical channels has been successfully synthesized in one pot from iron­(II) trifluoromethanesulfonate, 4-formylimidazole, hydrazine, and sodium azide under solvothermal conditions and features a rare unh topology and porous structure for...

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Published in:Inorganic chemistry 2021-01, Vol.60 (2), p.565-569
Main Authors: Dai, Rui-Rong, Ding, Chong-Wei, Zhou, Jie-Yi, Wei, Rong-Jia, Wang, Xue-Zhi, Zhou, Xiao-Ping, Li, Dan
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container_end_page 569
container_issue 2
container_start_page 565
container_title Inorganic chemistry
container_volume 60
creator Dai, Rui-Rong
Ding, Chong-Wei
Zhou, Jie-Yi
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Wang, Xue-Zhi
Zhou, Xiao-Ping
Li, Dan
description A unique metal–organic framework (MOF) with tetrazole-padded helical channels has been successfully synthesized in one pot from iron­(II) trifluoromethanesulfonate, 4-formylimidazole, hydrazine, and sodium azide under solvothermal conditions and features a rare unh topology and porous structure for gas adsorption. Transformations of condensation, cycloaddition, and coordination occurred during the synthetic process, in which a 1,5-disubstituted tetrazole ligand was formed in situ.
doi_str_mv 10.1021/acs.inorgchem.0c03216
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title Iron(II) Metal–Organic Framework with unh Topology and Tetrazole-Padded Helical Channels
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