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Feasibility of nanoscale zerovalent iron-loaded sediment-based biochar (nZVI-SBC) for simultaneous removal of nitrate and phosphate: high selectivity toward dinitrogen and synergistic mechanism
In the process of water treatment, excessive nitrogen and phosphorus pollutants are of great concern. Therefore, we prepared nanoscale zerovalent iron loaded on sediment-based biochar (nZVI-SBC) to conduct nitrate and phosphate removal at the same time. The characterization demonstrated that nZVI-SB...
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| Published in: | Environmental science and pollution research international 2021-07, Vol.28 (28), p.37448-37458 |
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| container_issue | 28 |
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| container_title | Environmental science and pollution research international |
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| creator | Liu, Xiaohui Wei, Jia Hou, Liangang Zhu, Yuhan Wu, Yaodong Xing, Luyi Zhang, Yifei Li, Jun |
| description | In the process of water treatment, excessive nitrogen and phosphorus pollutants are of great concern. Therefore, we prepared nanoscale zerovalent iron loaded on sediment-based biochar (nZVI-SBC) to conduct nitrate and phosphate removal at the same time. The characterization demonstrated that nZVI-SBC was successfully synthesized, which had obvious advantages for larger specific surface area and better dispersion compared with pure nZVI. The batch experiments indicated that the best loading ratio of nZVI to SBC and optimum dosage for nitrate and phosphate were 1:1and 2 g L
−1
, respectively. Their removal by nZVI-SBC was an acid-driven process. Anoxic environment was more conducive to the reduction of nitrate while the phosphate removal was fond of oxygen environment. A total of 77.78% of nitrate and 99.21% of phosphate have been successfully removed, mainly depending on reduction and complexation mechanism, respectively. Moreover, nZVI-SBC had higher N
2
selectivity and produced less ammonium than nZVI. The interaction between nitrate and phosphate was studied to manifest that they had different degrees of inhibition during the removal of the other. Our research indicated that nZVI-SBC has great potential for remediation of nitrogen and phosphorus polluted water.
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| doi_str_mv | 10.1007/s11356-021-13322-w |
| format | article |
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−1
, respectively. Their removal by nZVI-SBC was an acid-driven process. Anoxic environment was more conducive to the reduction of nitrate while the phosphate removal was fond of oxygen environment. A total of 77.78% of nitrate and 99.21% of phosphate have been successfully removed, mainly depending on reduction and complexation mechanism, respectively. Moreover, nZVI-SBC had higher N
2
selectivity and produced less ammonium than nZVI. The interaction between nitrate and phosphate was studied to manifest that they had different degrees of inhibition during the removal of the other. Our research indicated that nZVI-SBC has great potential for remediation of nitrogen and phosphorus polluted water.
Graphical abstract</description><identifier>ISSN: 0944-1344</identifier><identifier>EISSN: 1614-7499</identifier><identifier>DOI: 10.1007/s11356-021-13322-w</identifier><identifier>PMID: 33715122</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Ammonium ; anaerobic conditions ; Aquatic Pollution ; Atmospheric Protection/Air Quality Control/Air Pollution ; biochar ; Charcoal ; Earth and Environmental Science ; Ecotoxicology ; Environment ; Environmental Chemistry ; Environmental Health ; Environmental science ; Iron ; Nitrate removal ; Nitrates ; Nitrogen ; Nitrogen removal ; oxygen ; Phosphate ; Phosphates ; Phosphorus ; Phosphorus removal ; Pollutants ; Reduction ; remediation ; Research Article ; Selectivity ; surface area ; Waste Water Technology ; Water Management ; Water pollution ; Water Pollution Control ; Water treatment</subject><ispartof>Environmental science and pollution research international, 2021-07, Vol.28 (28), p.37448-37458</ispartof><rights>The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2021</rights><rights>The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2021.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c408t-77e18ce414c4c26cf1791ba32cd63e25fed9876bf5fdf86c9ef13285dfbab82a3</citedby><cites>FETCH-LOGICAL-c408t-77e18ce414c4c26cf1791ba32cd63e25fed9876bf5fdf86c9ef13285dfbab82a3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://www.proquest.com/docview/2554498502/fulltextPDF?pq-origsite=primo$$EPDF$$P50$$Gproquest$$H</linktopdf><linktohtml>$$Uhttps://www.proquest.com/docview/2554498502?pq-origsite=primo$$EHTML$$P50$$Gproquest$$H</linktohtml><link.rule.ids>314,776,780,11667,27901,27902,36037,36038,44339,74638</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/33715122$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Liu, Xiaohui</creatorcontrib><creatorcontrib>Wei, Jia</creatorcontrib><creatorcontrib>Hou, Liangang</creatorcontrib><creatorcontrib>Zhu, Yuhan</creatorcontrib><creatorcontrib>Wu, Yaodong</creatorcontrib><creatorcontrib>Xing, Luyi</creatorcontrib><creatorcontrib>Zhang, Yifei</creatorcontrib><creatorcontrib>Li, Jun</creatorcontrib><title>Feasibility of nanoscale zerovalent iron-loaded sediment-based biochar (nZVI-SBC) for simultaneous removal of nitrate and phosphate: high selectivity toward dinitrogen and synergistic mechanism</title><title>Environmental science and pollution research international</title><addtitle>Environ Sci Pollut Res</addtitle><addtitle>Environ Sci Pollut Res Int</addtitle><description>In the process of water treatment, excessive nitrogen and phosphorus pollutants are of great concern. Therefore, we prepared nanoscale zerovalent iron loaded on sediment-based biochar (nZVI-SBC) to conduct nitrate and phosphate removal at the same time. The characterization demonstrated that nZVI-SBC was successfully synthesized, which had obvious advantages for larger specific surface area and better dispersion compared with pure nZVI. The batch experiments indicated that the best loading ratio of nZVI to SBC and optimum dosage for nitrate and phosphate were 1:1and 2 g L
−1
, respectively. Their removal by nZVI-SBC was an acid-driven process. Anoxic environment was more conducive to the reduction of nitrate while the phosphate removal was fond of oxygen environment. A total of 77.78% of nitrate and 99.21% of phosphate have been successfully removed, mainly depending on reduction and complexation mechanism, respectively. Moreover, nZVI-SBC had higher N
2
selectivity and produced less ammonium than nZVI. The interaction between nitrate and phosphate was studied to manifest that they had different degrees of inhibition during the removal of the other. Our research indicated that nZVI-SBC has great potential for remediation of nitrogen and phosphorus polluted water.
Graphical abstract</description><subject>Ammonium</subject><subject>anaerobic conditions</subject><subject>Aquatic Pollution</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>biochar</subject><subject>Charcoal</subject><subject>Earth and Environmental Science</subject><subject>Ecotoxicology</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Environmental science</subject><subject>Iron</subject><subject>Nitrate removal</subject><subject>Nitrates</subject><subject>Nitrogen</subject><subject>Nitrogen removal</subject><subject>oxygen</subject><subject>Phosphate</subject><subject>Phosphates</subject><subject>Phosphorus</subject><subject>Phosphorus removal</subject><subject>Pollutants</subject><subject>Reduction</subject><subject>remediation</subject><subject>Research Article</subject><subject>Selectivity</subject><subject>surface area</subject><subject>Waste Water Technology</subject><subject>Water Management</subject><subject>Water pollution</subject><subject>Water Pollution Control</subject><subject>Water 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of nanoscale zerovalent iron-loaded sediment-based biochar (nZVI-SBC) for simultaneous removal of nitrate and phosphate: high selectivity toward dinitrogen and synergistic mechanism</title><author>Liu, Xiaohui ; Wei, Jia ; Hou, Liangang ; Zhu, Yuhan ; Wu, Yaodong ; Xing, Luyi ; Zhang, Yifei ; Li, Jun</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c408t-77e18ce414c4c26cf1791ba32cd63e25fed9876bf5fdf86c9ef13285dfbab82a3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2021</creationdate><topic>Ammonium</topic><topic>anaerobic conditions</topic><topic>Aquatic Pollution</topic><topic>Atmospheric Protection/Air Quality Control/Air Pollution</topic><topic>biochar</topic><topic>Charcoal</topic><topic>Earth and Environmental Science</topic><topic>Ecotoxicology</topic><topic>Environment</topic><topic>Environmental Chemistry</topic><topic>Environmental Health</topic><topic>Environmental 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simultaneous removal of nitrate and phosphate: high selectivity toward dinitrogen and synergistic mechanism</atitle><jtitle>Environmental science and pollution research international</jtitle><stitle>Environ Sci Pollut Res</stitle><addtitle>Environ Sci Pollut Res Int</addtitle><date>2021-07-01</date><risdate>2021</risdate><volume>28</volume><issue>28</issue><spage>37448</spage><epage>37458</epage><pages>37448-37458</pages><issn>0944-1344</issn><eissn>1614-7499</eissn><abstract>In the process of water treatment, excessive nitrogen and phosphorus pollutants are of great concern. Therefore, we prepared nanoscale zerovalent iron loaded on sediment-based biochar (nZVI-SBC) to conduct nitrate and phosphate removal at the same time. The characterization demonstrated that nZVI-SBC was successfully synthesized, which had obvious advantages for larger specific surface area and better dispersion compared with pure nZVI. The batch experiments indicated that the best loading ratio of nZVI to SBC and optimum dosage for nitrate and phosphate were 1:1and 2 g L
−1
, respectively. Their removal by nZVI-SBC was an acid-driven process. Anoxic environment was more conducive to the reduction of nitrate while the phosphate removal was fond of oxygen environment. A total of 77.78% of nitrate and 99.21% of phosphate have been successfully removed, mainly depending on reduction and complexation mechanism, respectively. Moreover, nZVI-SBC had higher N
2
selectivity and produced less ammonium than nZVI. The interaction between nitrate and phosphate was studied to manifest that they had different degrees of inhibition during the removal of the other. Our research indicated that nZVI-SBC has great potential for remediation of nitrogen and phosphorus polluted water.
Graphical abstract</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><pmid>33715122</pmid><doi>10.1007/s11356-021-13322-w</doi><tpages>11</tpages></addata></record> |
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| subjects | Ammonium anaerobic conditions Aquatic Pollution Atmospheric Protection/Air Quality Control/Air Pollution biochar Charcoal Earth and Environmental Science Ecotoxicology Environment Environmental Chemistry Environmental Health Environmental science Iron Nitrate removal Nitrates Nitrogen Nitrogen removal oxygen Phosphate Phosphates Phosphorus Phosphorus removal Pollutants Reduction remediation Research Article Selectivity surface area Waste Water Technology Water Management Water pollution Water Pollution Control Water treatment |
| title | Feasibility of nanoscale zerovalent iron-loaded sediment-based biochar (nZVI-SBC) for simultaneous removal of nitrate and phosphate: high selectivity toward dinitrogen and synergistic mechanism |
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