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Formaldehyde recognition through aminal formation in a luminescent metal-organic framework
Two isostructural pillar-layer MOFs (JNU-105 and JNU-105-(NH 2 ) 2 ) have been successfully synthesized. JNU-105-(NH 2 ) 2 exhibits a red-shifted luminescence "turn on" for formaldehyde without the interference from other VOCs and a detection limit of 1.87 ppb. In situ single-crystal trans...
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| Published in: | Chemical communications (Cambridge, England) England), 2022-06, Vol.58 (45), p.649-6493 |
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| Main Authors: | , , , , , |
| Format: | Article |
| Language: | English |
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| cites | cdi_FETCH-LOGICAL-c337t-e9c432c4752cc5e2e5c7ed8c0ee912a075db5edb133bb1300096bd9d2d9d832d3 |
| container_end_page | 6493 |
| container_issue | 45 |
| container_start_page | 649 |
| container_title | Chemical communications (Cambridge, England) |
| container_volume | 58 |
| creator | Li, Jia-Li Xiong, Xiao Luo, Dong Wei, Yu-Bai Lu, Weigang Li, Dan |
| description | Two isostructural pillar-layer MOFs (JNU-105 and
JNU-105-(NH
2
)
2
) have been successfully synthesized.
JNU-105-(NH
2
)
2
exhibits a red-shifted luminescence "turn on" for formaldehyde without the interference from other VOCs and a detection limit of 1.87 ppb.
In situ
single-crystal transformation studies confirm the aminal formation on the pillar linker, which was attributed to the exclusive luminescence response toward formaldehyde.
Reticular synthesis of a pillar-layer metal-organic framework with a diamino-functionalized dicarboxylate as a pillar linker, realizing an exclusive luminescence response toward formaldehyde through aminal formation. |
| doi_str_mv | 10.1039/d2cc02041f |
| format | article |
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JNU-105-(NH
2
)
2
) have been successfully synthesized.
JNU-105-(NH
2
)
2
exhibits a red-shifted luminescence "turn on" for formaldehyde without the interference from other VOCs and a detection limit of 1.87 ppb.
In situ
single-crystal transformation studies confirm the aminal formation on the pillar linker, which was attributed to the exclusive luminescence response toward formaldehyde.
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JNU-105-(NH
2
)
2
) have been successfully synthesized.
JNU-105-(NH
2
)
2
exhibits a red-shifted luminescence "turn on" for formaldehyde without the interference from other VOCs and a detection limit of 1.87 ppb.
In situ
single-crystal transformation studies confirm the aminal formation on the pillar linker, which was attributed to the exclusive luminescence response toward formaldehyde.
Reticular synthesis of a pillar-layer metal-organic framework with a diamino-functionalized dicarboxylate as a pillar linker, realizing an exclusive luminescence response toward formaldehyde through aminal formation.</description><subject>Formaldehyde</subject><subject>Luminescence</subject><subject>Metal-organic frameworks</subject><subject>Single crystals</subject><issn>1359-7345</issn><issn>1364-548X</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2022</creationdate><recordtype>article</recordtype><recordid>eNpdkd9LwzAQx4Mobk5ffFcKvohQzc_-eJTqVBj4oiC-lDS5bp1tM5MW2X9vuk0FD5ILuQ_Hfb-H0CnB1wSz9EZTpTDFnJR7aExYxEPBk7f94S3SMGZcjNCRc0vsg4jkEI2YEAJHgo3R-9TYRtYaFmsNgQVl5m3VVaYNuoU1_XwRyKZqZR2UA7cpVG0gg7r33-AUtF3QQCfr0Ni5bCsVlFY28GXsxzE6KGXt4GSXJ-h1ev-SPYaz54en7HYWKsbiLoRUcUYVj4WXIYCCUDHoRGGAlFCJY6ELAbogjBX-8hrSqNCppv4kjGo2QZfbvitrPntwXd5UfrC6li2Y3uU0inicCBYxj178Q5emt17eQMUkSajgwlNXW0pZ45yFMl_ZqpF2nROcD47ndzTLNo5PPXy-a9kXDehf9MdiD5xtAevUb_VvZewbdO6GMA</recordid><startdate>20220601</startdate><enddate>20220601</enddate><creator>Li, Jia-Li</creator><creator>Xiong, Xiao</creator><creator>Luo, Dong</creator><creator>Wei, Yu-Bai</creator><creator>Lu, Weigang</creator><creator>Li, Dan</creator><general>Royal Society of Chemistry</general><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SR</scope><scope>7U5</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>L7M</scope><scope>7X8</scope><orcidid>https://orcid.org/0000-0002-0433-0328</orcidid><orcidid>https://orcid.org/0000-0002-4936-4599</orcidid><orcidid>https://orcid.org/0000-0001-6960-4783</orcidid><orcidid>https://orcid.org/0000-0001-9751-8241</orcidid><orcidid>https://orcid.org/0000-0001-8066-1906</orcidid></search><sort><creationdate>20220601</creationdate><title>Formaldehyde recognition through aminal formation in a luminescent metal-organic framework</title><author>Li, Jia-Li ; Xiong, Xiao ; Luo, Dong ; Wei, Yu-Bai ; Lu, Weigang ; Li, Dan</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c337t-e9c432c4752cc5e2e5c7ed8c0ee912a075db5edb133bb1300096bd9d2d9d832d3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2022</creationdate><topic>Formaldehyde</topic><topic>Luminescence</topic><topic>Metal-organic frameworks</topic><topic>Single crystals</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Li, Jia-Li</creatorcontrib><creatorcontrib>Xiong, Xiao</creatorcontrib><creatorcontrib>Luo, Dong</creatorcontrib><creatorcontrib>Wei, Yu-Bai</creatorcontrib><creatorcontrib>Lu, Weigang</creatorcontrib><creatorcontrib>Li, Dan</creatorcontrib><collection>PubMed</collection><collection>CrossRef</collection><collection>Engineered Materials Abstracts</collection><collection>Solid State and Superconductivity Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>Advanced Technologies Database with Aerospace</collection><collection>MEDLINE - Academic</collection><jtitle>Chemical communications (Cambridge, England)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Li, Jia-Li</au><au>Xiong, Xiao</au><au>Luo, Dong</au><au>Wei, Yu-Bai</au><au>Lu, Weigang</au><au>Li, Dan</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Formaldehyde recognition through aminal formation in a luminescent metal-organic framework</atitle><jtitle>Chemical communications (Cambridge, England)</jtitle><addtitle>Chem Commun (Camb)</addtitle><date>2022-06-01</date><risdate>2022</risdate><volume>58</volume><issue>45</issue><spage>649</spage><epage>6493</epage><pages>649-6493</pages><issn>1359-7345</issn><eissn>1364-548X</eissn><abstract>Two isostructural pillar-layer MOFs (JNU-105 and
JNU-105-(NH
2
)
2
) have been successfully synthesized.
JNU-105-(NH
2
)
2
exhibits a red-shifted luminescence "turn on" for formaldehyde without the interference from other VOCs and a detection limit of 1.87 ppb.
In situ
single-crystal transformation studies confirm the aminal formation on the pillar linker, which was attributed to the exclusive luminescence response toward formaldehyde.
Reticular synthesis of a pillar-layer metal-organic framework with a diamino-functionalized dicarboxylate as a pillar linker, realizing an exclusive luminescence response toward formaldehyde through aminal formation.</abstract><cop>England</cop><pub>Royal Society of Chemistry</pub><pmid>35550653</pmid><doi>10.1039/d2cc02041f</doi><tpages>4</tpages><orcidid>https://orcid.org/0000-0002-0433-0328</orcidid><orcidid>https://orcid.org/0000-0002-4936-4599</orcidid><orcidid>https://orcid.org/0000-0001-6960-4783</orcidid><orcidid>https://orcid.org/0000-0001-9751-8241</orcidid><orcidid>https://orcid.org/0000-0001-8066-1906</orcidid></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 1359-7345 |
| ispartof | Chemical communications (Cambridge, England), 2022-06, Vol.58 (45), p.649-6493 |
| issn | 1359-7345 1364-548X |
| language | eng |
| recordid | cdi_proquest_miscellaneous_2664785363 |
| source | Royal Society of Chemistry Journals |
| subjects | Formaldehyde Luminescence Metal-organic frameworks Single crystals |
| title | Formaldehyde recognition through aminal formation in a luminescent metal-organic framework |
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