Room-Temperature Strong Coupling Between a Single Quantum Dot and a Single Plasmonic Nanoparticle

A single quantum dot (QD) strongly coupled with a plasmonic nanoparticle yields a promising qubit for scalable solid-state quantum information processing at room temperature. However, realizing such a strong coupling remains challenging due to the difficulty of spatial overlap of the QD excitons wit...

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Bibliographic Details
Published in:Nano letters 2022-06, Vol.22 (12), p.4686-4693
Main Authors: Li, Jun-Yu, Li, Wei, Liu, Jin, Zhong, Jie, Liu, Renming, Chen, Huanjun, Wang, Xue-Hua
Format: Article
Language:English
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Summary:A single quantum dot (QD) strongly coupled with a plasmonic nanoparticle yields a promising qubit for scalable solid-state quantum information processing at room temperature. However, realizing such a strong coupling remains challenging due to the difficulty of spatial overlap of the QD excitons with the plasmonic electric fields (EFs). Here, by using a transmission electron microscope we demonstrate for the first time that this overlap can be realized by integrating a deterministic single QD with a single Au nanorod. When a wedge nanogap cavity consisting of them and the substrate is constructed, the plasmonic EFs can be more effectively “dragged” and highly confined in the QD’s nanoshell where the excitons mainly reside. With these advantages, we observed the largest spectral Rabi splitting (reported so far) of ∼234 meV for a single QD strong coupling with plasmons. Our work opens a pathway to the massive construction of room-temperature strong coupling solid qubits.
ISSN:1530-6984
1530-6992
DOI:10.1021/acs.nanolett.2c00606