Assessment of meteorological settings on air quality modeling system—a proposal for UN-SDG and regulatory studies in non-homogeneous regions in Brazil

• Published in: Environmental science and pollution research international 2023, Vol.30 (1), p.1737-1760
• Main Authors: Soares da Silva, Mauricio, Pimentel, Luiz Cláudio Gomes, Duda, Fernando Pereira, Aragão, Leonardo, Silva, Corbiniano, Dragaud, Ian Cunha D’Amato Viana, Vicentini, Pedro Caffaro
• Format: Article
• Language: English
• Subjects: Air Pollutants - analysis; Air Pollution - analysis; Aquatic Pollution; Atmospheric Protection/Air Quality Control/Air Pollution; Brazil; Earth and Environmental Science; Ecotoxicology; Environment; Environmental Chemistry; Environmental Health; Environmental Monitoring - methods; Humans; Models, Theoretical; Research Article; Sustainable Development; Waste Water Technology; Water Management; Water Pollution Control
• ISSN: 0944-1344; 1614-7499
• DOI: 10.1007/s11356-022-22146-1

Air quality models are essential tools to meet the United Nations Sustainable Development Goals (UN-SDG) because they are effective in guiding public policies for the management of air pollutant emissions and their impacts on the environment and human health. Despite its importance, Brazil still lacks a guide for choosing and setting air quality models for regulatory purposes. Based on this, the current research aims to assess the combined WRF/CALMET/CALPUFF models for representing SO 2 dispersion over non-homogeneous regions as a regulatory model for policies in Brazilian Metropolitan Regions to satisfy the UN-SDG. The combined system was applied to the Rio de Janeiro Metropolitan Area (RJMA), which is known for its physiographic complexity. In the first step, the WRF model was evaluated against surface-observed data. The local circulation was underestimated, while the prevailing observational winds were well represented. In the second step, it was verified that all CALMET three meteorological configurations performed better for the most frequent wind speed classes so that the largest SO 2 concentrations errors occurred during light winds. Among the meteorological settings in WRF/CALMET/CALPUFF, the joined use of observed and modeled meteorological data yielded the best results for the dispersion of pollutants. This result emphasizes the relevance of meteorological data composition in complex regions with unsatisfactory monitoring given the inherent limitations of prognostic models and the excessive extrapolation of observed data that can generate distortions of reality. This research concludes with the proposal of the WRF/CALMET/CALPUFF air quality regulatory system as a supporting tool for policies in the Brazilian Metropolitan Regions in the framework of the UN-SDG, particularly in non-homogeneous regions where steady-state Gaussian models are not applicable.