Electromagnetic Wave Absorbing, Thermal-Conductive Flexible Membrane with Shape-Modulated FeCo Nanobelts

• Published in: ACS applied materials & interfaces 2022-08, Vol.14 (34), p.39255-39264
• Main Authors: Chang, Mi Se, Kwon, Suk Jin, Jeong, Jae Won, Ryu, Seung Han, Jeong, Seung Jae, Lee, Kyunbae, Kim, Taehoon, Yang, Sangsun, Park, Chong Rae, Park, Byeongjin, Kwon, Young-Tae
• Format: Article
• Language: English
• Subjects: Functional Nanostructured Materials (including low-D carbon)
• ISSN: 1944-8244; 1944-8252
• DOI: 10.1021/acsami.2c11094

Electromagnetic wave (EMW)-absorbing materials, manufactured with composites of magnetic particles, are essential for maintaining a high complex permeability and modulated permittivity for impedance matching. However, commonly available EMW-absorbing materials are unsatisfactory owing to their low complex permeability in the high-frequency band. Herein, we report a thin, flexible EMW-absorbing membrane comprising shape-modulated FeCo nanobelts/boron nitride nanoparticles, which enables enhanced complex permeability in the S, C, and X bands (2–12 GHz). The boron nitride nanoparticles that are introduced to the FeCo nanobelts demonstrate control of the complex permittivity, leading to an effective impedance matching close to 1, consequently resulting in a high reflection loss value of −42.2 dB at 12.0 GHz with only 1.6 mm thickness. In addition, the incorporation of boron nitride nanoparticles improves the thermal conductivity for the heat dissipation of the absorbed electromagnetic wave energy. Overall, the comprehensive study of nanomaterial preparation and shape modulation technologies can lead to the fabrication of an excellent EMW-absorbing flexible composite membrane.