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Simulation of sputtering induced by high energy gold clusters

Recently Andersen et al. reported exceptionally large nonlinear sputtering yields following the bombardment of gold targets with small, high energy gold clusters (H.H. Andersen, A. Brunelle, S. Della-Negra, J. Depauw, Y. LeBeyec, Phys. Rev. Lett. 80 (1998) 5433). Nonlinearities up to ∼1000% were obs...

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Published in:Nuclear instruments & methods in physics research. Section B, Beam interactions with materials and atoms Beam interactions with materials and atoms, 1999-05, Vol.152 (2-3), p.221-231
Main Authors: Shapiro, M.H, Tombrello, T.A
Format: Article
Language:English
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Summary:Recently Andersen et al. reported exceptionally large nonlinear sputtering yields following the bombardment of gold targets with small, high energy gold clusters (H.H. Andersen, A. Brunelle, S. Della-Negra, J. Depauw, Y. LeBeyec, Phys. Rev. Lett. 80 (1998) 5433). Nonlinearities up to ∼1000% were observed for Au5 clusters with a total energy of 800 keV. We have carried out molecular dynamics simulations on a massively parallel computer to model the Aun→Au system. The results suggest that both collisional and thermal spike mechanisms contribute to the large nonlinear yields observed by Andersen et al. Our simulations also indicate that sputtering statistics are very important at high cluster bombarding energies. A substantial fraction of the simulated impacts produce no sputtered atoms, while individual sputtering events producing very large numbers of sputtered atoms contribute significantly to the total sputtering yield at high energy.
ISSN:0168-583X
1872-9584
DOI:10.1016/S0168-583X(99)00141-X