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Effect of stratosphere-troposphere exchange on the future tropospheric ozone trend
This paper investigates the impact of circulation changes in a changed climate on the exchange of ozone between the stratosphere and the troposphere. We have identified an increase in the net transport of ozone into the troposphere in the future climate of 37%, although a decreased ozone lifetime me...
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Published in: | Journal of Geophysical Research. D. Atmospheres 2003-06, Vol.108 (D12), p.STA13.1-n/a |
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container_issue | D12 |
container_start_page | STA13.1 |
container_title | Journal of Geophysical Research. D. Atmospheres |
container_volume | 108 |
creator | Collins, W. J. Derwent, R. G. Garnier, B. Johnson, C. E. Sanderson, M. G. Stevenson, D. S. |
description | This paper investigates the impact of circulation changes in a changed climate on the exchange of ozone between the stratosphere and the troposphere. We have identified an increase in the net transport of ozone into the troposphere in the future climate of 37%, although a decreased ozone lifetime means that the overall tropospheric burden decreases. There are regions in the midlatitudes to high latitudes where surface ozone is predicted to increase in the spring. However, these increases are not significant. Significant ozone increases are predicted in regions of the upper troposphere. The general increase in the stratospheric contribution (O3s tracer) to tropospheric ozone in the climate changed scenario indicates that the stratosphere will play an even more significant role in the future. |
doi_str_mv | 10.1029/2002JD002617 |
format | article |
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J. ; Derwent, R. G. ; Garnier, B. ; Johnson, C. E. ; Sanderson, M. G. ; Stevenson, D. S.</creator><creatorcontrib>Collins, W. J. ; Derwent, R. G. ; Garnier, B. ; Johnson, C. E. ; Sanderson, M. G. ; Stevenson, D. S.</creatorcontrib><description>This paper investigates the impact of circulation changes in a changed climate on the exchange of ozone between the stratosphere and the troposphere. We have identified an increase in the net transport of ozone into the troposphere in the future climate of 37%, although a decreased ozone lifetime means that the overall tropospheric burden decreases. There are regions in the midlatitudes to high latitudes where surface ozone is predicted to increase in the spring. However, these increases are not significant. Significant ozone increases are predicted in regions of the upper troposphere. The general increase in the stratospheric contribution (O3s tracer) to tropospheric ozone in the climate changed scenario indicates that the stratosphere will play an even more significant role in the future.</description><identifier>ISSN: 0148-0227</identifier><identifier>EISSN: 2156-2202</identifier><identifier>DOI: 10.1029/2002JD002617</identifier><language>eng</language><publisher>Washington, DC: Blackwell Publishing Ltd</publisher><subject>Atmospheric composition. Chemical and photochemical reactions ; Chemical composition and interactions. Ionic interactions and processes ; chemistry transport modeling ; climate change ; Earth, ocean, space ; Exact sciences and technology ; External geophysics ; Meteorology ; Physics of the high neutral atmosphere ; stratosphere-troposphere exchange ; tropospheric chemistry ; tropospheric ozone</subject><ispartof>Journal of Geophysical Research. D. Atmospheres, 2003-06, Vol.108 (D12), p.STA13.1-n/a</ispartof><rights>Copyright 2003 by the American Geophysical Union.</rights><rights>2003 INIST-CNRS</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c5110-a99edd9498ef02aebc04c834aefefeca5bf7658928eb4c99d2aab7f64b30c3d83</citedby><cites>FETCH-LOGICAL-c5110-a99edd9498ef02aebc04c834aefefeca5bf7658928eb4c99d2aab7f64b30c3d83</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://onlinelibrary.wiley.com/doi/pdf/10.1029%2F2002JD002617$$EPDF$$P50$$Gwiley$$H</linktopdf><linktohtml>$$Uhttps://onlinelibrary.wiley.com/doi/full/10.1029%2F2002JD002617$$EHTML$$P50$$Gwiley$$H</linktohtml><link.rule.ids>314,780,784,11512,27922,27923,46466,46890</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=15085204$$DView record in Pascal Francis$$Hfree_for_read</backlink></links><search><creatorcontrib>Collins, W. 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Significant ozone increases are predicted in regions of the upper troposphere. The general increase in the stratospheric contribution (O3s tracer) to tropospheric ozone in the climate changed scenario indicates that the stratosphere will play an even more significant role in the future.</description><subject>Atmospheric composition. Chemical and photochemical reactions</subject><subject>Chemical composition and interactions. Ionic interactions and processes</subject><subject>chemistry transport modeling</subject><subject>climate change</subject><subject>Earth, ocean, space</subject><subject>Exact sciences and technology</subject><subject>External geophysics</subject><subject>Meteorology</subject><subject>Physics of the high neutral atmosphere</subject><subject>stratosphere-troposphere exchange</subject><subject>tropospheric chemistry</subject><subject>tropospheric ozone</subject><issn>0148-0227</issn><issn>2156-2202</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2003</creationdate><recordtype>article</recordtype><recordid>eNqFkU1LxDAQhoMouKg3f0AverKa7yZH8WN18QtRBC8hTSdutTZr0sXVX2-XXdSTzsDMMDzve5hBaJvgfYKpPqAY09FxXyQpVtCAEiFzSjFdRQNMuMoxpcU62krpGffBheSYDNDtiffguiz4LHXRdiFNxhAh72KYLOcMZm5s2yfIQpt1Y8j8tJv26x-kdln4DO18BW21ida8bRJsLfsGuj89uTs6yy-uh-dHhxe5E4Tg3GoNVaW5VuAxtVA6zJ1i3ILv01lR-kIKpamCkjutK2ptWXjJS4YdqxTbQLsL30kMb1NInXmtk4OmsS2EaTK0UFJqKv8FiVKCK8V6cG8BuhhSiuDNJNavNn4Ygs38yOb3kXt8Z-lrk7ONj7Z1dfrRCKwExbzn2IJ7rxv4-NPTjIa3x2T-oF6VL1R16mD2rbLxxciCFcI8XA1NMXpklzc3d-aKfQHS2ZtA</recordid><startdate>20030627</startdate><enddate>20030627</enddate><creator>Collins, W. 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G.</creatorcontrib><creatorcontrib>Garnier, B.</creatorcontrib><creatorcontrib>Johnson, C. E.</creatorcontrib><creatorcontrib>Sanderson, M. G.</creatorcontrib><creatorcontrib>Stevenson, D. S.</creatorcontrib><collection>Istex</collection><collection>Pascal-Francis</collection><collection>CrossRef</collection><collection>Meteorological & Geoastrophysical Abstracts</collection><collection>Meteorological & Geoastrophysical Abstracts - Academic</collection><collection>Technology Research Database</collection><collection>Aerospace Database</collection><collection>Advanced Technologies Database with Aerospace</collection><jtitle>Journal of Geophysical Research. D. Atmospheres</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Collins, W. J.</au><au>Derwent, R. G.</au><au>Garnier, B.</au><au>Johnson, C. E.</au><au>Sanderson, M. G.</au><au>Stevenson, D. S.</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Effect of stratosphere-troposphere exchange on the future tropospheric ozone trend</atitle><jtitle>Journal of Geophysical Research. D. Atmospheres</jtitle><addtitle>J. Geophys. Res</addtitle><date>2003-06-27</date><risdate>2003</risdate><volume>108</volume><issue>D12</issue><spage>STA13.1</spage><epage>n/a</epage><pages>STA13.1-n/a</pages><issn>0148-0227</issn><eissn>2156-2202</eissn><abstract>This paper investigates the impact of circulation changes in a changed climate on the exchange of ozone between the stratosphere and the troposphere. We have identified an increase in the net transport of ozone into the troposphere in the future climate of 37%, although a decreased ozone lifetime means that the overall tropospheric burden decreases. There are regions in the midlatitudes to high latitudes where surface ozone is predicted to increase in the spring. However, these increases are not significant. Significant ozone increases are predicted in regions of the upper troposphere. The general increase in the stratospheric contribution (O3s tracer) to tropospheric ozone in the climate changed scenario indicates that the stratosphere will play an even more significant role in the future.</abstract><cop>Washington, DC</cop><pub>Blackwell Publishing Ltd</pub><doi>10.1029/2002JD002617</doi><tpages>10</tpages><oa>free_for_read</oa></addata></record> |
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subjects | Atmospheric composition. Chemical and photochemical reactions Chemical composition and interactions. Ionic interactions and processes chemistry transport modeling climate change Earth, ocean, space Exact sciences and technology External geophysics Meteorology Physics of the high neutral atmosphere stratosphere-troposphere exchange tropospheric chemistry tropospheric ozone |
title | Effect of stratosphere-troposphere exchange on the future tropospheric ozone trend |
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