Transport and deposition of radionuclides from northern Africa to the southern Iberian Peninsula and the Canary Islands during the intense dust intrusions of March 2022

• Published in: Chemosphere (Oxford) 2024-03, Vol.352, p.141303-141303, Article 141303
• Main Authors: Liger, Esperanza, Hernández, Francisco, Expósito, Francisco Javier, Díaz, Juan Pedro, Salazar-Carballo, Pedro A., Gordo, Elisa, González, Cristina, López-Pérez, María
• Format: Article
• Language: English
• Subjects: Aerosol; Aerosols - analysis; Africa, Northern; Atmospheric deposition; Caesium; Cesium Radioisotopes - analysis; Dust - analysis; Long-range transport; Plutonium; Saharan dust; Spain
• ISSN: 0045-6535; 1879-1298
• DOI: 10.1016/j.chemosphere.2024.141303

The present study focuses on the two consecutive and markedly intense Saharan dust intrusion episodes that greatly affected southern Spain (Málaga) and, to a lesser extent, the Canary Islands (Tenerife), in March 2022. These two episodes were the result of atypical meteorological conditions in the region and resulted in record levels of aerosols in the air at the Málaga location. The activity levels of various natural and artificial radionuclides (7Be, 210Pb, 40K, 137Cs, 239Pu, 240Pu, 239+240Pu) and radioactive indicators (gross alpha and gross beta) were impacted by these events and the results are described herein. These episodes caused, for example, the activities of 137Cs in aerosol samples at the Málaga monitoring station to reach the highest concentrations ever recorded since high-volume aerosol monitoring started at this site in 2009. A link between the activity levels of 137Cs, 40K and gross alpha in the atmospheric aerosols and daily PM10 concentrations during the episodes is also reported. In addition, isotopic ratios are discussed in the context of the source and destination of the various anthropogenic radionuclides measured. The atmospheric residence time of aerosols during these episodes is also evaluated because it concerns how intrusions to the Canary Islands should be analysed. Finally, for the first time, the concentrations of 137Cs deposition by rainwater during a Saharan dust intrusion are reported and the deposition rate of these radionuclides during these episodes is discussed. [Display omitted] •Two atypical and intense dust Saharan events affected Spain during March 2022.•These Saharan dust events caused increments of radionuclides in atmospheric aerosols.•Record concentrations of 137Cs were recorded during these events in Málaga.•PM10,137Cs, 40K and gross alpha concentrations correlated during these dust events.•Rainfall enhanced aerosols deposition to approximately 26–56 days of dry deposition.