Efficient electrocatalytic reduction of CO2 to CO enhanced by synergistic effect of N, P on carbon aerogel

Metal-free catalyst, N, P-codoped carbon aerogel, was used to realize the high efficiency reduction of CO2 to CO. Therein, the pyridinic N acts as the active center to active and reduce CO2 and the atom of P acts as the "transition atom" of proton to reduce the free energy barrier from *CO...

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Bibliographic Details
Published in:Chemical communications (Cambridge, England) England), 2024-06, Vol.60 (50), p.6439-6442
Main Authors: Yan, Yifan, Wang, Hongzhi, Bi, Xinze, Zhao, Yuezhu, Wu, Mingbo
Format: Article
Language:English
Subjects:
Aerogels
Carbon dioxide
Carbon monoxide
Chemical reduction
Free energy
Synergistic effect
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Summary:Metal-free catalyst, N, P-codoped carbon aerogel, was used to realize the high efficiency reduction of CO2 to CO. Therein, the pyridinic N acts as the active center to active and reduce CO2 and the atom of P acts as the "transition atom" of proton to reduce the free energy barrier from *CO2 to *COOH.
ISSN:1359-7345
1364-548X
1364-548X
DOI:10.1039/d4cc01537a