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Lanthanum-based magnetic biopolymers for brilliant green removal from aqueous solutions
In this study, lanthanum (La)-based magnetic biopolymers were synthesized, and the first adsorption study was conducted on the removal of brilliant green dye from aqueous water with these biopolymers. For the adsorption study, adsorption parameters were investigated and the ideal adsorption conditio...
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| Published in: | Environmental science and pollution research international 2024-07, Vol.31 (35), p.47714-47726 |
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| container_title | Environmental science and pollution research international |
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| creator | Karaaslan Ayhan, Nagihan |
| description | In this study, lanthanum (La)-based magnetic biopolymers were synthesized, and the first adsorption study was conducted on the removal of brilliant green dye from aqueous water with these biopolymers. For the adsorption study, adsorption parameters were investigated and the ideal adsorption conditions determined for the removal of brilliant green dye from aqueous solutions are pH 11,
t
60 min,
m
10 mg,
C
0
25 mg/L,
T
298 K. It was determined that the adsorption process was compatible with the single-layer Langmuir isotherm, and maximum adsorption capacity obtained according to the Langmuir isotherm was calculated as 256.41 mg/g. The adsorption process was found to be in accordance with the pseudo-second-order, and the adsorption process was explained by intra-particle diffusion. According to studies of adsorption thermodynamics, it has been established that the nature of the adsorption reaction is spontaneous, and this process is endothermic and has increasing randomness. Moreover, the reusability of magnetic lanthanum/alginate (La/Alg) biopolymers was investigated, and it was determined that the biopolymers could be used successfully. In summary, brilliant green dye has been successfully removed with simple, low-cost, environmentally friendly, and easily obtained magnetic La/Alg biopolymers. It can be stated that even low amounts of these biopolymers can be effective in the treatment of highly concentrated dye wastewaters. |
| doi_str_mv | 10.1007/s11356-024-34274-x |
| format | article |
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t
60 min,
m
10 mg,
C
0
25 mg/L,
T
298 K. It was determined that the adsorption process was compatible with the single-layer Langmuir isotherm, and maximum adsorption capacity obtained according to the Langmuir isotherm was calculated as 256.41 mg/g. The adsorption process was found to be in accordance with the pseudo-second-order, and the adsorption process was explained by intra-particle diffusion. According to studies of adsorption thermodynamics, it has been established that the nature of the adsorption reaction is spontaneous, and this process is endothermic and has increasing randomness. Moreover, the reusability of magnetic lanthanum/alginate (La/Alg) biopolymers was investigated, and it was determined that the biopolymers could be used successfully. In summary, brilliant green dye has been successfully removed with simple, low-cost, environmentally friendly, and easily obtained magnetic La/Alg biopolymers. It can be stated that even low amounts of these biopolymers can be effective in the treatment of highly concentrated dye wastewaters.</description><identifier>ISSN: 1614-7499</identifier><identifier>ISSN: 0944-1344</identifier><identifier>EISSN: 1614-7499</identifier><identifier>DOI: 10.1007/s11356-024-34274-x</identifier><identifier>PMID: 39007971</identifier><language>eng</language><publisher>Berlin/Heidelberg: Springer Berlin Heidelberg</publisher><subject>Adsorption ; Alginates ; Alginic acid ; Aquatic Pollution ; Aqueous solutions ; Atmospheric Protection/Air Quality Control/Air Pollution ; Biopolymers ; Biopolymers - chemistry ; Diffusion layers ; Dyes ; Earth and Environmental Science ; Ecotoxicology ; Endothermic reactions ; Environment ; Environmental Chemistry ; Environmental Health ; Industrial wastewater ; Isotherms ; Kinetics ; Lanthanum ; Lanthanum - chemistry ; Particle diffusion ; Quaternary Ammonium Compounds ; Research Article ; Thermodynamics ; Waste Water Technology ; Water Management ; Water Pollutants, Chemical - chemistry ; Water Pollution Control ; Water Purification - methods</subject><ispartof>Environmental science and pollution research international, 2024-07, Vol.31 (35), p.47714-47726</ispartof><rights>The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature 2024. Springer Nature or its licensor (e.g. a society or other partner) holds exclusive rights to this article under a publishing agreement with the author(s) or other rightsholder(s); author self-archiving of the accepted manuscript version of this article is solely governed by the terms of such publishing agreement and applicable law.</rights><rights>2024. The Author(s), under exclusive licence to Springer-Verlag GmbH Germany, part of Springer Nature.</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><cites>FETCH-LOGICAL-c171x-22915cbca46f434ac7942fba1f40836c42ebb56b03c105b8cc45abe9c9454aaf3</cites><orcidid>0000-0001-9083-9149</orcidid></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,27923,27924</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/39007971$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Karaaslan Ayhan, Nagihan</creatorcontrib><title>Lanthanum-based magnetic biopolymers for brilliant green removal from aqueous solutions</title><title>Environmental science and pollution research international</title><addtitle>Environ Sci Pollut Res</addtitle><addtitle>Environ Sci Pollut Res Int</addtitle><description>In this study, lanthanum (La)-based magnetic biopolymers were synthesized, and the first adsorption study was conducted on the removal of brilliant green dye from aqueous water with these biopolymers. For the adsorption study, adsorption parameters were investigated and the ideal adsorption conditions determined for the removal of brilliant green dye from aqueous solutions are pH 11,
t
60 min,
m
10 mg,
C
0
25 mg/L,
T
298 K. It was determined that the adsorption process was compatible with the single-layer Langmuir isotherm, and maximum adsorption capacity obtained according to the Langmuir isotherm was calculated as 256.41 mg/g. The adsorption process was found to be in accordance with the pseudo-second-order, and the adsorption process was explained by intra-particle diffusion. According to studies of adsorption thermodynamics, it has been established that the nature of the adsorption reaction is spontaneous, and this process is endothermic and has increasing randomness. Moreover, the reusability of magnetic lanthanum/alginate (La/Alg) biopolymers was investigated, and it was determined that the biopolymers could be used successfully. In summary, brilliant green dye has been successfully removed with simple, low-cost, environmentally friendly, and easily obtained magnetic La/Alg biopolymers. It can be stated that even low amounts of these biopolymers can be effective in the treatment of highly concentrated dye wastewaters.</description><subject>Adsorption</subject><subject>Alginates</subject><subject>Alginic acid</subject><subject>Aquatic Pollution</subject><subject>Aqueous solutions</subject><subject>Atmospheric Protection/Air Quality Control/Air Pollution</subject><subject>Biopolymers</subject><subject>Biopolymers - chemistry</subject><subject>Diffusion layers</subject><subject>Dyes</subject><subject>Earth and Environmental Science</subject><subject>Ecotoxicology</subject><subject>Endothermic reactions</subject><subject>Environment</subject><subject>Environmental Chemistry</subject><subject>Environmental Health</subject><subject>Industrial wastewater</subject><subject>Isotherms</subject><subject>Kinetics</subject><subject>Lanthanum</subject><subject>Lanthanum - chemistry</subject><subject>Particle diffusion</subject><subject>Quaternary Ammonium Compounds</subject><subject>Research Article</subject><subject>Thermodynamics</subject><subject>Waste Water Technology</subject><subject>Water Management</subject><subject>Water Pollutants, Chemical - chemistry</subject><subject>Water Pollution Control</subject><subject>Water Purification - methods</subject><issn>1614-7499</issn><issn>0944-1344</issn><issn>1614-7499</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2024</creationdate><recordtype>article</recordtype><recordid>eNp9kE1LwzAAhoMobk7_gAcJePFSzVeb5ijDLxh4UTyGJEtnR9rMpJXt35vZ-YEHTwnked-8PACcYnSJEeJXEWOaFxkiLKOMcJat98AYF5hlnAmx_-s-AkcxLhEiSBB-CEZUpLzgeAxeZqrtXlXbN5lW0c5hoxat7WoDde1X3m0aGyKsfIA61M7ViYaLYG0Lg238u3KwCr6B6q23vo8wetd3tW_jMTiolIv2ZHdOwPPtzdP0Pps93j1Mr2eZwRyvM0IEzo02ihUVo0wZLhiptMIVQyUtDCNW67zQiBqMcl0aw3KlrTCC5Uypik7AxdC7Cj5tiJ1s6misc6rdDpIUlaigJUcsoed_0KXvQ5vWbSleICYQSRQZKBN8jMFWchXqRoWNxEhutctBu0za5ad2uU6hs111rxs7_458eU4AHYCYntqFDT9__1P7ATdnjzY</recordid><startdate>202407</startdate><enddate>202407</enddate><creator>Karaaslan Ayhan, Nagihan</creator><general>Springer Berlin Heidelberg</general><general>Springer Nature B.V</general><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7QL</scope><scope>7SN</scope><scope>7T7</scope><scope>7TV</scope><scope>7U7</scope><scope>8FD</scope><scope>C1K</scope><scope>FR3</scope><scope>K9.</scope><scope>M7N</scope><scope>P64</scope><scope>7X8</scope><orcidid>https://orcid.org/0000-0001-9083-9149</orcidid></search><sort><creationdate>202407</creationdate><title>Lanthanum-based magnetic biopolymers for brilliant green removal from aqueous solutions</title><author>Karaaslan Ayhan, Nagihan</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c171x-22915cbca46f434ac7942fba1f40836c42ebb56b03c105b8cc45abe9c9454aaf3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2024</creationdate><topic>Adsorption</topic><topic>Alginates</topic><topic>Alginic acid</topic><topic>Aquatic Pollution</topic><topic>Aqueous solutions</topic><topic>Atmospheric Protection/Air Quality Control/Air Pollution</topic><topic>Biopolymers</topic><topic>Biopolymers - chemistry</topic><topic>Diffusion layers</topic><topic>Dyes</topic><topic>Earth and Environmental Science</topic><topic>Ecotoxicology</topic><topic>Endothermic reactions</topic><topic>Environment</topic><topic>Environmental Chemistry</topic><topic>Environmental Health</topic><topic>Industrial wastewater</topic><topic>Isotherms</topic><topic>Kinetics</topic><topic>Lanthanum</topic><topic>Lanthanum - chemistry</topic><topic>Particle diffusion</topic><topic>Quaternary Ammonium Compounds</topic><topic>Research Article</topic><topic>Thermodynamics</topic><topic>Waste Water Technology</topic><topic>Water Management</topic><topic>Water Pollutants, Chemical - chemistry</topic><topic>Water Pollution Control</topic><topic>Water Purification - methods</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Karaaslan Ayhan, Nagihan</creatorcontrib><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>Bacteriology Abstracts (Microbiology B)</collection><collection>Ecology Abstracts</collection><collection>Industrial and Applied Microbiology Abstracts (Microbiology A)</collection><collection>Pollution Abstracts</collection><collection>Toxicology Abstracts</collection><collection>Technology Research Database</collection><collection>Environmental Sciences and Pollution Management</collection><collection>Engineering Research Database</collection><collection>ProQuest Health & Medical Complete (Alumni)</collection><collection>Algology Mycology and Protozoology Abstracts (Microbiology C)</collection><collection>Biotechnology and BioEngineering Abstracts</collection><collection>MEDLINE - Academic</collection><jtitle>Environmental science and pollution research international</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Karaaslan Ayhan, Nagihan</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Lanthanum-based magnetic biopolymers for brilliant green removal from aqueous solutions</atitle><jtitle>Environmental science and pollution research international</jtitle><stitle>Environ Sci Pollut Res</stitle><addtitle>Environ Sci Pollut Res Int</addtitle><date>2024-07</date><risdate>2024</risdate><volume>31</volume><issue>35</issue><spage>47714</spage><epage>47726</epage><pages>47714-47726</pages><issn>1614-7499</issn><issn>0944-1344</issn><eissn>1614-7499</eissn><abstract>In this study, lanthanum (La)-based magnetic biopolymers were synthesized, and the first adsorption study was conducted on the removal of brilliant green dye from aqueous water with these biopolymers. For the adsorption study, adsorption parameters were investigated and the ideal adsorption conditions determined for the removal of brilliant green dye from aqueous solutions are pH 11,
t
60 min,
m
10 mg,
C
0
25 mg/L,
T
298 K. It was determined that the adsorption process was compatible with the single-layer Langmuir isotherm, and maximum adsorption capacity obtained according to the Langmuir isotherm was calculated as 256.41 mg/g. The adsorption process was found to be in accordance with the pseudo-second-order, and the adsorption process was explained by intra-particle diffusion. According to studies of adsorption thermodynamics, it has been established that the nature of the adsorption reaction is spontaneous, and this process is endothermic and has increasing randomness. Moreover, the reusability of magnetic lanthanum/alginate (La/Alg) biopolymers was investigated, and it was determined that the biopolymers could be used successfully. In summary, brilliant green dye has been successfully removed with simple, low-cost, environmentally friendly, and easily obtained magnetic La/Alg biopolymers. It can be stated that even low amounts of these biopolymers can be effective in the treatment of highly concentrated dye wastewaters.</abstract><cop>Berlin/Heidelberg</cop><pub>Springer Berlin Heidelberg</pub><pmid>39007971</pmid><doi>10.1007/s11356-024-34274-x</doi><tpages>13</tpages><orcidid>https://orcid.org/0000-0001-9083-9149</orcidid></addata></record> |
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| subjects | Adsorption Alginates Alginic acid Aquatic Pollution Aqueous solutions Atmospheric Protection/Air Quality Control/Air Pollution Biopolymers Biopolymers - chemistry Diffusion layers Dyes Earth and Environmental Science Ecotoxicology Endothermic reactions Environment Environmental Chemistry Environmental Health Industrial wastewater Isotherms Kinetics Lanthanum Lanthanum - chemistry Particle diffusion Quaternary Ammonium Compounds Research Article Thermodynamics Waste Water Technology Water Management Water Pollutants, Chemical - chemistry Water Pollution Control Water Purification - methods |
| title | Lanthanum-based magnetic biopolymers for brilliant green removal from aqueous solutions |
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