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Quantized hyperfine field at an implanted micro+ site in PrPb3: interplay between localized f electrons and an interstitial charged particle

The local effect of an interstitial hydrogenlike particle on localized f electrons was studied in PrPb3 by means of micro+ spin rotation and relaxation. Spontaneous micro+ spin precession with harmonic frequencies was observed for the first time in f electron compounds. We demonstrate that the signa...

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Bibliographic Details
Published in:Physical review letters 2009-03, Vol.102 (9), p.096403-096403
Main Authors: Ito, T U, Higemoto, W, Ohishi, K, Nishida, N, Heffner, R H, Aoki, Y, Amato, A, Onimaru, T, Suzuki, H S
Format: Article
Language:English
Online Access:Get full text
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Summary:The local effect of an interstitial hydrogenlike particle on localized f electrons was studied in PrPb3 by means of micro+ spin rotation and relaxation. Spontaneous micro+ spin precession with harmonic frequencies was observed for the first time in f electron compounds. We demonstrate that the signal is derived from a coupling between the micro+ spin and the hyperfine-enhanced nuclear spin of nearest neighbor (NN) 141Pr with Ising-like anisotropy. The signal also suggests a marked suppression of spin dynamics of the NN 141Pr in comparison with that of the bulk 141Pr. These facts strongly indicate modification of the f electronic state due to the interstitial charged particle.
ISSN:0031-9007