Copper(II) and Zinc(II) Complexes Can Fix Atmospheric Carbon Dioxide

Carbonato bridges from atmospheric carbon dioxide: The copper(II) and zinc(II) complexes of the novel imidazole‐containing polyamine ligand N1‐(2‐aminoethyl)‐N1‐(2‐imidazolethyl)ethane‐1,2‐diamine are found to fix carbon dioxide by hydration to μ3‐carbonate ligands. This is revealed by IR and solid‐...

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Published in:Angewandte Chemie International Edition 2005-07, Vol.44 (28), p.4352-4355
Main Authors: Kong, Ling-Yan, Zhang, Zheng-Hua, Zhu, Hui-Fang, Kawaguchi, Hiroyuki, Okamura, Taka-aki, Doi, Mototsugu, Chu, Qian, Sun, Wei-Yin, Ueyama, Norikazu
Format: Article
Language:English
Subjects:
Atmosphere - chemistry
Carbon Dioxide - chemistry
Carbon Dioxide - metabolism
carbon dioxide fixation
copper
Copper - chemistry
Ligands
Macromolecular Substances - chemistry
Magnetic Resonance Spectroscopy
Models, Molecular
networks
NMR spectroscopy
zinc
Zinc - chemistry
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container_title Angewandte Chemie International Edition
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creator Kong, Ling-Yan
Zhang, Zheng-Hua
Zhu, Hui-Fang
Kawaguchi, Hiroyuki
Okamura, Taka-aki
Doi, Mototsugu
Chu, Qian
Sun, Wei-Yin
Ueyama, Norikazu
description Carbonato bridges from atmospheric carbon dioxide: The copper(II) and zinc(II) complexes of the novel imidazole‐containing polyamine ligand N1‐(2‐aminoethyl)‐N1‐(2‐imidazolethyl)ethane‐1,2‐diamine are found to fix carbon dioxide by hydration to μ3‐carbonate ligands. This is revealed by IR and solid‐state 13C NMR spectroscopic and X‐ray crystallographic studies of the two‐dimensional complexes (see picture).
doi_str_mv 10.1002/anie.200500587
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subjects Atmosphere - chemistry
Carbon Dioxide - chemistry
Carbon Dioxide - metabolism
carbon dioxide fixation
copper
Copper - chemistry
Ligands
Macromolecular Substances - chemistry
Magnetic Resonance Spectroscopy
Models, Molecular
networks
NMR spectroscopy
zinc
Zinc - chemistry
title Copper(II) and Zinc(II) Complexes Can Fix Atmospheric Carbon Dioxide
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