Drop formation via breakup of a liquid bridge in an AC electric field

• Published in: Journal of colloid and interface science 2006-10, Vol.302 (1), p.294-307
• Main Authors: Lee, Beom Seok, Cho, Hye-Jung, Lee, Jeong-Gun, Huh, Nam, Choi, Jeong-Woo, Kang, In Seok
• Format: Article
• Language: English
• Subjects: AC electric field; Chemistry; DNA - chemistry; EHD method; Electrodes; Electromagnetic Fields; Electrowetting; Exact sciences and technology; General and physical chemistry; Insulator; Liquid bridge; Oligonucleotide Array Sequence Analysis - instrumentation; Oligonucleotide Array Sequence Analysis - methods; Oscillometry; Particle Size; Resonant frequency; Surface Properties; Water - chemistry
• ISSN: 0021-9797; 1095-7103
• DOI: 10.1016/j.jcis.2006.05.060

Experimental results are presented for the study of drop formation mechanism in a newly proposed electrohydrodynamic (EHD) method of drop generation in an AC electric field. In the method, a small drop is generated in two stages. A pendant drop is elongated with large oscillation by an electric force in the first stage. Then, it undergoes formation and breakup of a liquid bridge between the upper nozzle and the insulator-coated lower flat plate in the second stage. It is found that there exists a resonant frequency for maximum oscillation, which leads to an efficient drop formation in the latter stage. It is also found that breakup of liquid bridge is accelerated by the electrowetting tension acting on the drop perimeter contacting the insulator-coated flat plate. Thus the whole procedure of drop formation depends heavily on the frequency of AC field and the properties of the insulator such as hydrophilicity, thickness, and the dielectric constant. It is demonstrated that a wide range of drop size, from picoliter to nanoliter, can be obtained by controlling such key parameters without changing the nozzle diameter. Mechanism in a newly proposed EHD method of drop formation in an AC electric field is studied and it is divided into two stages, such as drop elongation and breakup of a liquid bridge.