Toward the total synthesis of spirastrellolide A. Part 3: intelligence gathering and preparation of a ring-expanded analogue

Different methods for the formation of the C.25-C.26 bond of spirastrellolide A () are evaluated that might qualify for the end game of the projected total synthesis, with emphasis on metathetic ways to forge the macrocyclic frame.

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Bibliographic Details
Published in:Chemical communications (Cambridge, England) England), 2007-01 (29), p.3045-3047
Main Authors: Fürstner, Alois, Fasching, Bernhard, O'Neil, Gregory W, Fenster, Michaël D B, Godbout, Cédrickx, Ceccon, Julien
Format: Article
Language:English
Subjects:
Cyclization
Indicators and Reagents - chemistry
Macrolides - chemical synthesis
Spiro Compounds
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Summary:Different methods for the formation of the C.25-C.26 bond of spirastrellolide A () are evaluated that might qualify for the end game of the projected total synthesis, with emphasis on metathetic ways to forge the macrocyclic frame.
ISSN:1359-7345
1364-548X
DOI:10.1039/b707835h