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Photoexcitation of a dipole-forbidden resonance in helium

We have observed photoexcitation of the dipole-forbidden 1s(2) 1S0-->2p(2) 1D2 resonance in helium by measuring the nondipolar forward-backward asymmetry of photoelectron angular distributions in the 2l2l(') autoionizing region. By exploiting the electric dipole-quadrupole interference in th...

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Bibliographic Details
Published in:Physical review letters 2002-05, Vol.88 (20), p.203002-203002, Article 203002
Main Authors: Krässig, B, Kanter, E P, Southworth, S H, Guillemin, R, Hemmers, O, Lindle, D W, Wehlitz, R, Martin, N L S
Format: Article
Language:English
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Summary:We have observed photoexcitation of the dipole-forbidden 1s(2) 1S0-->2p(2) 1D2 resonance in helium by measuring the nondipolar forward-backward asymmetry of photoelectron angular distributions in the 2l2l(') autoionizing region. By exploiting the electric dipole-quadrupole interference in the excitation of both the 2s2p 1P1 and 2p(2) 1D2 levels, we have observed the quadrupole resonance in photoabsorption and extracted its Fano line shape parameters and the relative phase of the 1sEp and 1sEd continua. We find the quadrupole line profile index q(2) to be markedly different from theoretical expectations.
ISSN:0031-9007
1079-7114
DOI:10.1103/PhysRevLett.88.203002