Bridged Silver(I) Complexes of the Polycyclic Aromatic Compounds Tetraphenylethylene and 1,1,4,4-Tetraphenyl-1,3-butadiene

For the purpose of investigating the coordination behavior of the sterically congested alkenes and exploring the possibility of cofacial complexation in the polycyclic aromatic system for formation of extended polymeric networks, tetraphenylethylene (tphe) and 1,1,4,4-tetraphenyl-1,3-butadiene (tphb...

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Published in:Inorganic chemistry 2000-11, Vol.39 (24), p.5430-5436
Main Authors: Ino, Ichiro, Wu, Liang Ping, Munakata, Megumu, Kuroda-Sowa, Takayoshi, Maekawa, Masahiko, Suenaga, Yusaku, Sakai, Ryusuke
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container_end_page 5436
container_issue 24
container_start_page 5430
container_title Inorganic chemistry
container_volume 39
creator Ino, Ichiro
Wu, Liang Ping
Munakata, Megumu
Kuroda-Sowa, Takayoshi
Maekawa, Masahiko
Suenaga, Yusaku
Sakai, Ryusuke
description For the purpose of investigating the coordination behavior of the sterically congested alkenes and exploring the possibility of cofacial complexation in the polycyclic aromatic system for formation of extended polymeric networks, tetraphenylethylene (tphe) and 1,1,4,4-tetraphenyl-1,3-butadiene (tphb) have been studied with regard to their complexation with a silver(I) ion. The crystal structures of [Ag(tphe)(ClO4)(p-xylene)], [Ag2(tphe)(ClO4)2], [Ag4(tphe)(CF3SO3)4], [Ag2(tphb)(ClO4)2], and [Ag2(tphb)(CF3SO3)2], together with the metal-free ligands tphe and tphb, have been determined by single-crystal X-ray diffraction. The π-electron-rich cleft in organic components is found to offer a potential site for complexation, which can be utilized to generate an interesting array of organometallic compounds with one- and two-dimensional frameworks.
doi_str_mv 10.1021/ic000263u
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title Bridged Silver(I) Complexes of the Polycyclic Aromatic Compounds Tetraphenylethylene and 1,1,4,4-Tetraphenyl-1,3-butadiene
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