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Dynamical coupling and separation of multiple degrees of freedom in a photoexcited double-exchange system

We present a theory of ultrafast photoinduced dynamics in a spin-charge coupled system, motivated by pump-probe experiments in perovskite manganites. A microscopic picture for multiple dynamics in spin and charge degrees is examined. Real-time simulations are carried out by two complimentary methods...

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Bibliographic Details
Published in:Physical review letters 2009-12, Vol.103 (26), p.267401-267401, Article 267401
Main Authors: Kanamori, Y, Matsueda, H, Ishihara, S
Format: Article
Language:English
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Summary:We present a theory of ultrafast photoinduced dynamics in a spin-charge coupled system, motivated by pump-probe experiments in perovskite manganites. A microscopic picture for multiple dynamics in spin and charge degrees is examined. Real-time simulations are carried out by two complimentary methods. Our calculation demonstrates that electron motion governs a short-time scale where charge and spin dynamics are combined strongly, while, in a long-time scale controlled by spin relaxation, the charge sector does not follow the remarkable change in the spin sector. The present results are in contrast to a conventional double-exchange picture in equilibrium states.
ISSN:0031-9007
1079-7114
DOI:10.1103/physrevlett.103.267401