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Dynamical coupling and separation of multiple degrees of freedom in a photoexcited double-exchange system
We present a theory of ultrafast photoinduced dynamics in a spin-charge coupled system, motivated by pump-probe experiments in perovskite manganites. A microscopic picture for multiple dynamics in spin and charge degrees is examined. Real-time simulations are carried out by two complimentary methods...
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Published in: | Physical review letters 2009-12, Vol.103 (26), p.267401-267401, Article 267401 |
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Main Authors: | , , |
Format: | Article |
Language: | English |
Citations: | Items that this one cites Items that cite this one |
Online Access: | Get full text |
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Summary: | We present a theory of ultrafast photoinduced dynamics in a spin-charge coupled system, motivated by pump-probe experiments in perovskite manganites. A microscopic picture for multiple dynamics in spin and charge degrees is examined. Real-time simulations are carried out by two complimentary methods. Our calculation demonstrates that electron motion governs a short-time scale where charge and spin dynamics are combined strongly, while, in a long-time scale controlled by spin relaxation, the charge sector does not follow the remarkable change in the spin sector. The present results are in contrast to a conventional double-exchange picture in equilibrium states. |
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ISSN: | 0031-9007 1079-7114 |
DOI: | 10.1103/physrevlett.103.267401 |