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Dimensionality Effects in the Lifetime of Surface States
A long-standing discrepancy between experimental and theoretical values for the lifetimes of holes in the surface-state electron bands on noble metal surfaces is resolved; previous determinations of both are found to have been in error. The ability of the scanning tunneling microscope to verify surf...
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Published in: | Science (American Association for the Advancement of Science) 2000-05, Vol.288 (5470), p.1399-1402 |
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creator | Kliewer, J. Berndt, R. Chulkov, E. V. Silkin, V. M. Echenique, P. M. Crampin, S. |
description | A long-standing discrepancy between experimental and theoretical values for the lifetimes of holes in the surface-state electron bands on noble metal surfaces is resolved; previous determinations of both are found to have been in error. The ability of the scanning tunneling microscope to verify surface quality before taking spectroscopic measurements is used to remove the effects of defect scattering on experimental lifetimes, found to have been a significant contribution to prior determinations. A theoretical treatment of inelastic electron-electron scattering is developed that explicitly includes intraband transitions within the surface state band. In our model, two-dimensional decay channels dominate the electron-electron interactions that contribute to the hole decay and are screened by the electron states of the underlying three-dimensional electron system. |
doi_str_mv | 10.1126/science.288.5470.1399 |
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A theoretical treatment of inelastic electron-electron scattering is developed that explicitly includes intraband transitions within the surface state band. In our model, two-dimensional decay channels dominate the electron-electron interactions that contribute to the hole decay and are screened by the electron states of the underlying three-dimensional electron system.</description><subject>Applied sciences</subject><subject>Atoms</subject><subject>Condensed matter: electronic structure, electrical, magnetic, and optical properties</subject><subject>Electron tunneling</subject><subject>Electronic structure</subject><subject>Electronic structure and electrical properties of surfaces, interfaces, thin films and low-dimensional structures</subject><subject>Electrons</subject><subject>Energy</subject><subject>Exact sciences and technology</subject><subject>Fundamental Concepts</subject><subject>Laboratory Equipment</subject><subject>Metals</subject><subject>Metals. 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The ability of the scanning tunneling microscope to verify surface quality before taking spectroscopic measurements is used to remove the effects of defect scattering on experimental lifetimes, found to have been a significant contribution to prior determinations. A theoretical treatment of inelastic electron-electron scattering is developed that explicitly includes intraband transitions within the surface state band. In our model, two-dimensional decay channels dominate the electron-electron interactions that contribute to the hole decay and are screened by the electron states of the underlying three-dimensional electron system.</abstract><cop>Washington, DC</cop><pub>American Society for the Advancement of Science</pub><pmid>10827945</pmid><doi>10.1126/science.288.5470.1399</doi><tpages>4</tpages></addata></record> |
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subjects | Applied sciences Atoms Condensed matter: electronic structure, electrical, magnetic, and optical properties Electron tunneling Electronic structure Electronic structure and electrical properties of surfaces, interfaces, thin films and low-dimensional structures Electrons Energy Exact sciences and technology Fundamental Concepts Laboratory Equipment Metals Metals. Metallurgy Noble metals Physics Quasiparticles Scientific imaging Spectral reconnaissance Spectroscopy Surface and interface electron states Surface states, band structure, electron density of states Wave functions |
title | Dimensionality Effects in the Lifetime of Surface States |
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