Organic persistent toxic substances in soils, waters and sediments along an altitudinal gradient at Mt. Sagarmatha, Himalayas, Nepal

• Published in: Environmental pollution (1987) 2011-10, Vol.159 (10), p.2552-2564
• Main Authors: Guzzella, Licia, Poma, Giulia, De Paolis, Adolfo, Roscioli, Claudio, Viviano, Gaetano
• Format: Article
• Language: English
• Subjects: Altitude; Applied sciences; Biological and physicochemical phenomena; Earth sciences; Earth, ocean, space; Engineering and environment geology. Geothermics; Environmental Monitoring; Environmental Pollutants - analysis; Environmental Pollutants - toxicity; Environmental Pollution - statistics & numerical data; Exact sciences and technology; Fresh Water - chemistry; Geologic Sediments - chemistry; Halogenated Diphenyl Ethers - analysis; Hazardous Substances - analysis; Hazardous Substances - toxicity; Himalayas; Lake water; Natural water pollution; Nepal; Organic Chemicals - analysis; Organic Chemicals - toxicity; Pollution; Pollution sources. Measurement results; Pollution, environment geology; Polychlorinated Biphenyls - analysis; Polycyclic Aromatic Hydrocarbons - analysis; PTSs; Sediment; Soil; Soil - chemistry; Soil and sediments pollution; Water treatment and pollution
• ISSN: 0269-7491; 1873-6424
• DOI: 10.1016/j.envpol.2011.06.015

Persistent Organic Pollutants (POPs) and Polycyclic Aromatic Hydrocarbons (PAHs) are important classes of compounds of serious environmental concern. These compounds were measured in waters, sediments and soils from several high altitude sites in the Sagarmatha National Park (Nepal) and included in the Himalayan ridge. In water samples, low-level substituted PCBs and PBDEs, along with more volatile PAHs, were the most common contaminants. In sediment and soil samples, the PCB profile was mainly composed of medium-level chlorinated congeners and significantly correlated with altitude. The PAH profile for water and soil samples showed the main contribution of pyrogenic PAHs due to emissions of solid combustion, whereas the profile for sediments indicated the main contribution of pyrogenic PAHs from gasoline emissions. The PAH levels measured in Himalayan samples must be considered as low to medium contaminated, whereas the regarded Himalayan stations can be considered undisturbed remote areas concerning PCB, PBDE and OC compounds. ► POPs were measured in environmental samples from remote lakes in the Himalaya ridge. ► It was confirmed the hypothesis of Long-Range Atmospheric Transport for lighter POPs. ► PAH levels in Himalayan samples must be considered as low to medium contaminated. ► The stations can be considered undisturbed remote areas concerning PCB, PBDE and OCC. Organic PTSs in environmental matrices in remote regions of the Himalayan ridge.