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On-site and off-site atmospheric PBDEs in an electronic dismantling workshop in south China: Gas-particle partitioning and human exposure assessment
Gas samples and total suspended particle during work and off work time were investigated on-site and off-site electronic waste dismantling workshop (I- and O-EWDW), then compared with plastic recycling workshop (PRW) and waste incineration plant (WIP). TSP concentrations and total PBDE were 0.36–2.2...
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Published in: | Environmental pollution (1987) 2011-12, Vol.159 (12), p.3529-3535 |
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creator | An, Taicheng Zhang, Delin Li, Guiying Mai, Bixian Fu, Jiamo |
description | Gas samples and total suspended particle during work and off work time were investigated on-site and off-site electronic waste dismantling workshop (I- and O-EWDW), then compared with plastic recycling workshop (PRW) and waste incineration plant (WIP). TSP concentrations and total PBDE were 0.36–2.21 mg/m
3 and 27–2975 ng/m
3 at different workshops, respectively. BDE-47, -99, and -209 were major ∑PBDE congeners at I-EWDW and WIP, while BDE-209 was only dominant congener in PRW and control sites during work time and all sites during off work time. The gas-particle partitioning result was well correlated with the subcooled liquid vapor pressure for all samples, except for WIP and I-EDWD, at park during work time, and residential area during off work time. The predicted urban curve fitted well with measured
φ values at O-DEWD during work time, whereas it was slightly overestimated or underestimated for others. Exposure assessment revealed the highest exposure site was I-EDWD.
► On- and off-site atmospheric PBDEs was monitored in e-waste dismantling workshops in south China. ► The gas-particle partitioning result was well correlated with the subcooled liquid vapor pressure for some samples. ► Exposure assessment revealed that workers in I-EDWD were the highest exposure population.
The findings of this study may serve as a valuable reference for future risk assessment and environmental management in Guiyu, South China. |
doi_str_mv | 10.1016/j.envpol.2011.08.014 |
format | article |
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3 and 27–2975 ng/m
3 at different workshops, respectively. BDE-47, -99, and -209 were major ∑PBDE congeners at I-EWDW and WIP, while BDE-209 was only dominant congener in PRW and control sites during work time and all sites during off work time. The gas-particle partitioning result was well correlated with the subcooled liquid vapor pressure for all samples, except for WIP and I-EDWD, at park during work time, and residential area during off work time. The predicted urban curve fitted well with measured
φ values at O-DEWD during work time, whereas it was slightly overestimated or underestimated for others. Exposure assessment revealed the highest exposure site was I-EDWD.
► On- and off-site atmospheric PBDEs was monitored in e-waste dismantling workshops in south China. ► The gas-particle partitioning result was well correlated with the subcooled liquid vapor pressure for some samples. ► Exposure assessment revealed that workers in I-EDWD were the highest exposure population.
The findings of this study may serve as a valuable reference for future risk assessment and environmental management in Guiyu, South China.</description><identifier>ISSN: 0269-7491</identifier><identifier>EISSN: 1873-6424</identifier><identifier>DOI: 10.1016/j.envpol.2011.08.014</identifier><identifier>PMID: 21871700</identifier><identifier>CODEN: ENVPAF</identifier><language>eng</language><publisher>Kidlington: Elsevier Ltd</publisher><subject>Air ; Air Pollutants - analysis ; Assessments ; Atmospherics ; Biological and medical sciences ; China ; Congeners ; Dismantling ; Dust - analysis ; E-waste ; Electronic Waste - adverse effects ; Electronics ; Environmental Exposure - analysis ; Environmental Monitoring ; Environmental pollutants toxicology ; exposure assessment ; Flame Retardants - analysis ; Halogenated Diphenyl Ethers - analysis ; Human exposure assessment ; Humans ; Medical sciences ; On-site and off-site ; Partitioning ; PBDE ; plastics ; recycling ; Refuse Disposal ; Residential areas ; Toxicology ; vapor pressure ; waste incineration ; Workshops</subject><ispartof>Environmental pollution (1987), 2011-12, Vol.159 (12), p.3529-3535</ispartof><rights>2011 Elsevier Ltd</rights><rights>2015 INIST-CNRS</rights><rights>Copyright © 2011 Elsevier Ltd. All rights reserved.</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c592t-a151b5ebd6c75a2c1599d9425b225e9af7f4db1efcbe883e715f5733b8165bda3</citedby><cites>FETCH-LOGICAL-c592t-a151b5ebd6c75a2c1599d9425b225e9af7f4db1efcbe883e715f5733b8165bda3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,27924,27925</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=24623284$$DView record in Pascal Francis$$Hfree_for_read</backlink><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/21871700$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>An, Taicheng</creatorcontrib><creatorcontrib>Zhang, Delin</creatorcontrib><creatorcontrib>Li, Guiying</creatorcontrib><creatorcontrib>Mai, Bixian</creatorcontrib><creatorcontrib>Fu, Jiamo</creatorcontrib><title>On-site and off-site atmospheric PBDEs in an electronic dismantling workshop in south China: Gas-particle partitioning and human exposure assessment</title><title>Environmental pollution (1987)</title><addtitle>Environ Pollut</addtitle><description>Gas samples and total suspended particle during work and off work time were investigated on-site and off-site electronic waste dismantling workshop (I- and O-EWDW), then compared with plastic recycling workshop (PRW) and waste incineration plant (WIP). TSP concentrations and total PBDE were 0.36–2.21 mg/m
3 and 27–2975 ng/m
3 at different workshops, respectively. BDE-47, -99, and -209 were major ∑PBDE congeners at I-EWDW and WIP, while BDE-209 was only dominant congener in PRW and control sites during work time and all sites during off work time. The gas-particle partitioning result was well correlated with the subcooled liquid vapor pressure for all samples, except for WIP and I-EDWD, at park during work time, and residential area during off work time. The predicted urban curve fitted well with measured
φ values at O-DEWD during work time, whereas it was slightly overestimated or underestimated for others. Exposure assessment revealed the highest exposure site was I-EDWD.
► On- and off-site atmospheric PBDEs was monitored in e-waste dismantling workshops in south China. ► The gas-particle partitioning result was well correlated with the subcooled liquid vapor pressure for some samples. ► Exposure assessment revealed that workers in I-EDWD were the highest exposure population.
The findings of this study may serve as a valuable reference for future risk assessment and environmental management in Guiyu, South China.</description><subject>Air</subject><subject>Air Pollutants - analysis</subject><subject>Assessments</subject><subject>Atmospherics</subject><subject>Biological and medical sciences</subject><subject>China</subject><subject>Congeners</subject><subject>Dismantling</subject><subject>Dust - analysis</subject><subject>E-waste</subject><subject>Electronic Waste - adverse effects</subject><subject>Electronics</subject><subject>Environmental Exposure - analysis</subject><subject>Environmental Monitoring</subject><subject>Environmental pollutants toxicology</subject><subject>exposure assessment</subject><subject>Flame Retardants - analysis</subject><subject>Halogenated Diphenyl Ethers - analysis</subject><subject>Human exposure assessment</subject><subject>Humans</subject><subject>Medical sciences</subject><subject>On-site and off-site</subject><subject>Partitioning</subject><subject>PBDE</subject><subject>plastics</subject><subject>recycling</subject><subject>Refuse Disposal</subject><subject>Residential areas</subject><subject>Toxicology</subject><subject>vapor pressure</subject><subject>waste incineration</subject><subject>Workshops</subject><issn>0269-7491</issn><issn>1873-6424</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2011</creationdate><recordtype>article</recordtype><recordid>eNqNksuO1DAQRS0EYpqGP0CQDYJNGj_zmAUSNMOANNIgwawtx6lMu0ns4EoG-A8-GIduYDdi5YfOrVuqW4Q8ZnTDKCte7jfgb8bQbzhlbEOrDWXyDlmxqhR5Ibm8S1aUF3VeypqdkAeIe0qpFELcJyc8UaykdEV-Xvoc3QSZ8W0Wuu74mIaA4w6is9nHN2_PMHM-ERn0YKcYfPpuHQ7GT73z19m3EL_gLowLhWGedtl257w5zc4N5qOJk7M9ZL8vk0vqJFnsdvOw1Pw-BpxjMkUExAH89JDc60yP8Oh4rsnVu7PP2_f5xeX5h-3ri9yqmk-5YYo1Cpq2sKUy3DJV120tuWo4V1Cbruxk2zDobANVJaBkqlOlEE3FCtW0RqzJ80PdMYavM-CkB4cW-t54CDPqmoqioLxS_0FyUdS1lIl8cSvJynIZvUyCNZEH1MaAGKHTY3SDiT80o3rJWO_1IWO9ZKxppVPGSfbk6DA3A7R_RX9CTcCzI2DQmr6LxluH_zhZcMGrpdDTA9eZoM11TMzVp-Sk0qKwNMwqEa8OBKQUbhxEjdaBt9C6mDZBt8Hd3usvDPTSOA</recordid><startdate>20111201</startdate><enddate>20111201</enddate><creator>An, Taicheng</creator><creator>Zhang, Delin</creator><creator>Li, Guiying</creator><creator>Mai, Bixian</creator><creator>Fu, Jiamo</creator><general>Elsevier Ltd</general><general>Elsevier</general><scope>FBQ</scope><scope>IQODW</scope><scope>CGR</scope><scope>CUY</scope><scope>CVF</scope><scope>ECM</scope><scope>EIF</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>7SU</scope><scope>8FD</scope><scope>C1K</scope><scope>FR3</scope><scope>KR7</scope><scope>7ST</scope><scope>7TG</scope><scope>7TV</scope><scope>7U7</scope><scope>KL.</scope><scope>SOI</scope><scope>7X8</scope></search><sort><creationdate>20111201</creationdate><title>On-site and off-site atmospheric PBDEs in an electronic dismantling workshop in south China: Gas-particle partitioning and human exposure assessment</title><author>An, Taicheng ; Zhang, Delin ; Li, Guiying ; Mai, Bixian ; Fu, Jiamo</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c592t-a151b5ebd6c75a2c1599d9425b225e9af7f4db1efcbe883e715f5733b8165bda3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2011</creationdate><topic>Air</topic><topic>Air Pollutants - analysis</topic><topic>Assessments</topic><topic>Atmospherics</topic><topic>Biological and medical sciences</topic><topic>China</topic><topic>Congeners</topic><topic>Dismantling</topic><topic>Dust - analysis</topic><topic>E-waste</topic><topic>Electronic Waste - adverse effects</topic><topic>Electronics</topic><topic>Environmental Exposure - analysis</topic><topic>Environmental Monitoring</topic><topic>Environmental pollutants toxicology</topic><topic>exposure assessment</topic><topic>Flame Retardants - analysis</topic><topic>Halogenated Diphenyl Ethers - analysis</topic><topic>Human exposure assessment</topic><topic>Humans</topic><topic>Medical sciences</topic><topic>On-site and off-site</topic><topic>Partitioning</topic><topic>PBDE</topic><topic>plastics</topic><topic>recycling</topic><topic>Refuse Disposal</topic><topic>Residential areas</topic><topic>Toxicology</topic><topic>vapor pressure</topic><topic>waste incineration</topic><topic>Workshops</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>An, Taicheng</creatorcontrib><creatorcontrib>Zhang, Delin</creatorcontrib><creatorcontrib>Li, Guiying</creatorcontrib><creatorcontrib>Mai, Bixian</creatorcontrib><creatorcontrib>Fu, Jiamo</creatorcontrib><collection>AGRIS</collection><collection>Pascal-Francis</collection><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>Environmental Engineering Abstracts</collection><collection>Technology Research Database</collection><collection>Environmental Sciences and Pollution Management</collection><collection>Engineering Research Database</collection><collection>Civil Engineering Abstracts</collection><collection>Environment Abstracts</collection><collection>Meteorological & Geoastrophysical Abstracts</collection><collection>Pollution Abstracts</collection><collection>Toxicology Abstracts</collection><collection>Meteorological & Geoastrophysical Abstracts - Academic</collection><collection>Environment Abstracts</collection><collection>MEDLINE - Academic</collection><jtitle>Environmental pollution (1987)</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>An, Taicheng</au><au>Zhang, Delin</au><au>Li, Guiying</au><au>Mai, Bixian</au><au>Fu, Jiamo</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>On-site and off-site atmospheric PBDEs in an electronic dismantling workshop in south China: Gas-particle partitioning and human exposure assessment</atitle><jtitle>Environmental pollution (1987)</jtitle><addtitle>Environ Pollut</addtitle><date>2011-12-01</date><risdate>2011</risdate><volume>159</volume><issue>12</issue><spage>3529</spage><epage>3535</epage><pages>3529-3535</pages><issn>0269-7491</issn><eissn>1873-6424</eissn><coden>ENVPAF</coden><abstract>Gas samples and total suspended particle during work and off work time were investigated on-site and off-site electronic waste dismantling workshop (I- and O-EWDW), then compared with plastic recycling workshop (PRW) and waste incineration plant (WIP). TSP concentrations and total PBDE were 0.36–2.21 mg/m
3 and 27–2975 ng/m
3 at different workshops, respectively. BDE-47, -99, and -209 were major ∑PBDE congeners at I-EWDW and WIP, while BDE-209 was only dominant congener in PRW and control sites during work time and all sites during off work time. The gas-particle partitioning result was well correlated with the subcooled liquid vapor pressure for all samples, except for WIP and I-EDWD, at park during work time, and residential area during off work time. The predicted urban curve fitted well with measured
φ values at O-DEWD during work time, whereas it was slightly overestimated or underestimated for others. Exposure assessment revealed the highest exposure site was I-EDWD.
► On- and off-site atmospheric PBDEs was monitored in e-waste dismantling workshops in south China. ► The gas-particle partitioning result was well correlated with the subcooled liquid vapor pressure for some samples. ► Exposure assessment revealed that workers in I-EDWD were the highest exposure population.
The findings of this study may serve as a valuable reference for future risk assessment and environmental management in Guiyu, South China.</abstract><cop>Kidlington</cop><pub>Elsevier Ltd</pub><pmid>21871700</pmid><doi>10.1016/j.envpol.2011.08.014</doi><tpages>7</tpages><oa>free_for_read</oa></addata></record> |
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subjects | Air Air Pollutants - analysis Assessments Atmospherics Biological and medical sciences China Congeners Dismantling Dust - analysis E-waste Electronic Waste - adverse effects Electronics Environmental Exposure - analysis Environmental Monitoring Environmental pollutants toxicology exposure assessment Flame Retardants - analysis Halogenated Diphenyl Ethers - analysis Human exposure assessment Humans Medical sciences On-site and off-site Partitioning PBDE plastics recycling Refuse Disposal Residential areas Toxicology vapor pressure waste incineration Workshops |
title | On-site and off-site atmospheric PBDEs in an electronic dismantling workshop in south China: Gas-particle partitioning and human exposure assessment |
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