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Bismuth ferrite dielectric nanoparticles excited at telecom wavelengths as multicolor sources by second, third, and fourth harmonic generation

We demonstrate the simultaneous generation of second, third, and fourth harmonics from a single dielectric bismuth ferrite nanoparticle excited using a telecom fiber laser at 1560 nm. We first characterize the signals associated with different nonlinear orders in terms of spectrum, excitation intens...

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Published in:Nanoscale 2018-01, Vol.1 (17), p.8146-8152
Main Authors: Riporto, Jérémy, Demierre, Alexis, Kilin, Vasyl, Balciunas, Tadas, Schmidt, Cédric, Campargue, Gabriel, Urbain, Mathias, Baltuska, Andrius, Le Dantec, Ronan, Wolf, Jean-Pierre, Mugnier, Yannick, Bonacina, Luigi
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cited_by cdi_FETCH-LOGICAL-c371t-558f76e31edb7acbd1673d1afca6c96d7cb33bf7c489841d7b04cf7f5aaaeee3
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container_issue 17
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container_title Nanoscale
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creator Riporto, Jérémy
Demierre, Alexis
Kilin, Vasyl
Balciunas, Tadas
Schmidt, Cédric
Campargue, Gabriel
Urbain, Mathias
Baltuska, Andrius
Le Dantec, Ronan
Wolf, Jean-Pierre
Mugnier, Yannick
Bonacina, Luigi
description We demonstrate the simultaneous generation of second, third, and fourth harmonics from a single dielectric bismuth ferrite nanoparticle excited using a telecom fiber laser at 1560 nm. We first characterize the signals associated with different nonlinear orders in terms of spectrum, excitation intensity dependence, and relative signal strengths. Successively, on the basis of the polarization-resolved emission curves of the three harmonics, we discuss the interplay of susceptibility tensor components at different orders and show how polarization can be used as an optical handle to control the relative frequency conversion properties. We demonstrate the simultaneous generation of second, third, and fourth harmonics from a dielectric nanoparticle using a telecom laser at 1560 nm.
doi_str_mv 10.1039/c7nr08102b
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source Royal Society of Chemistry:Jisc Collections:Royal Society of Chemistry Read and Publish 2022-2024 (reading list)
subjects Bismuth ferrite
Dependence
Engineering Sciences
Excitation spectra
Fiber lasers
Harmonic generations
Nanoparticles
Optical properties
Optics
Photonic
Polarization
Telecommunications
title Bismuth ferrite dielectric nanoparticles excited at telecom wavelengths as multicolor sources by second, third, and fourth harmonic generation
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