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Exploring the spatial heterogeneity and temporal homogeneity of ambient PM 10 in nine core cities of China
We focus on the causes of fluctuations in wintertime PM in nine regional core cities of China using two machine learning models, Random Forest (RF) and Recurrent Neural Network (RNN). RF and RNN both show high performance in predicting hourly PM using only gaseous air pollutants (SO , NO and CO) as...
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Published in: | Scientific reports 2021-04, Vol.11 (1), p.8991 |
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Main Authors: | , , , , |
Format: | Article |
Language: | English |
Online Access: | Get full text |
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Summary: | We focus on the causes of fluctuations in wintertime PM
in nine regional core cities of China using two machine learning models, Random Forest (RF) and Recurrent Neural Network (RNN). RF and RNN both show high performance in predicting hourly PM
using only gaseous air pollutants (SO
, NO
and CO) as inputs, showing the predominance of the secondary inorganic aerosol and implying the existence of thermodynamic equilibrium between gaseous air pollutants and PM
. Also, we find the following results. The correlation of gaseous air pollutants and PM
were more relevant than that of meteorological conditions and PM
. CO was the predominant factor for PM
in the Beijing-Tianjin-Hebei Plain and the Yangtze River Delta while SO
and NO
were also important features for PM
in the Pearl River Delta and Sichuan Basin. The spatial heterogeneity and temporal homogeneity of PM
in China are revealed. The long-range transported PM
was substantiated to be insignificant, except in the sandstorms. The severity of PM
was attributable to the lopsided shift of thermodynamic equilibrium and the phenology of indigenous flora. |
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ISSN: | 2045-2322 |