Engineering lithiophilic Ni-Al@LDH interlayers on a garnet-type electrolyte for solid-state lithium metal batteries

In this work, a lithiophilic Ni-Al@LDH interlayer is engineered at the Li 6.4 La 3 Zr 1.4 Ta 0.6 O 12 (LLZTO) electrolyte and Li anode interface. The Ni-Al@LDH interlayer can significantly reduce the interfacial resistance as well as give excellent cycling performance both in a symmetric Li//Li cell...

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Bibliographic Details
Published in:Chemical communications (Cambridge, England) England), 2021-10, Vol.57 (79), p.1214-1217
Main Authors: Liu, Wei, Lu, Guanjie, Yang, Zuguang, Zhao, Qiannan, Hu, Xiaolin, Wu, Dan, Li, Zongyang, Wang, Ronghua, Sun, Shikuan, Xu, Chaohe
Format: Article
Language:English
Subjects:
Aluminum
Electrolytes
Interlayers
Lithium batteries
Nickel
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Summary:In this work, a lithiophilic Ni-Al@LDH interlayer is engineered at the Li 6.4 La 3 Zr 1.4 Ta 0.6 O 12 (LLZTO) electrolyte and Li anode interface. The Ni-Al@LDH interlayer can significantly reduce the interfacial resistance as well as give excellent cycling performance both in a symmetric Li//Li cell and solid full lithium metal batteries. In this work, a lithiophilic Ni-Al@LDH interlayer is engineered at the Li 6.4 La 3 Zr 1.4 Ta 0.6 O 12 (LLZTO) electrolyte and Li anode interface.
ISSN:1359-7345
1364-548X
DOI:10.1039/d1cc02932k