A tin porphyrin axially-coordinated two-dimensional covalent organic polymer for efficient hydrogen evolution

Herein, we demonstrate a facile strategy for constructing an efficient and stable hydrogen evolution reaction (HER) catalyst, i.e. a tin porphyrin axially-coordinated 2D covalent organic polymer (SnTPPCOP). SnTPPCOP exhibits promising HER activity with a low overpotential of 147 mV at 10 mA cm −2 du...

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Published in:Chemical communications (Cambridge, England) England), 2022-06, Vol.58 (53), p.7423-7426
Main Authors: Wang, Qi, Wang, Aijian, Dou, Yuqin, Shen, Xiaoliang, Sudi, M. Shire, Zhao, Long, Zhu, Weihua, Li, Longhua
Format: Article
Language:English
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Hydrogen evolution reactions
Polymers
Porphyrins
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cited_by cdi_FETCH-LOGICAL-c337t-1f1acfb019629880ba754c353c03a21cf384ef5879a7a56110f3d2a1804d0ae03
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container_end_page 7426
container_issue 53
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container_title Chemical communications (Cambridge, England)
container_volume 58
creator Wang, Qi
Wang, Aijian
Dou, Yuqin
Shen, Xiaoliang
Sudi, M. Shire
Zhao, Long
Zhu, Weihua
Li, Longhua
description Herein, we demonstrate a facile strategy for constructing an efficient and stable hydrogen evolution reaction (HER) catalyst, i.e. a tin porphyrin axially-coordinated 2D covalent organic polymer (SnTPPCOP). SnTPPCOP exhibits promising HER activity with a low overpotential of 147 mV at 10 mA cm −2 due to its unique structural properties, ranking among the best records reported recently. The prepared tin porphyrin axially-coordinated 2D covalent organic polymer exhibits excellent HER activity due to its unique structural properties, ranking among the best records reported recently.
doi_str_mv 10.1039/d2cc02775e
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subjects Hydrogen evolution reactions
Polymers
Porphyrins
title A tin porphyrin axially-coordinated two-dimensional covalent organic polymer for efficient hydrogen evolution
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