Novel high‐efficiency 2D position‐sensitive ZnS:Ag/6LiF scintillator detector for neutron diffraction

• Published in: Journal of applied crystallography 2024-06, Vol.57 (3), p.690-699
• Main Authors: Mauri, Giacomo, Sykora, G. Jeff, Schooneveld, E. M., Capelli, S. C., Gutmann, M. J., Howarth, S., Mann, S. E., Zuddas, F., Rhodes, N. J.
• Format: Article
• Language: English
• Subjects: Detectors; Efficiency; Fibers; high efficiency; Neutron counters; neutron detectors; Neutron diffraction; Neutrons; R&D; Research & development; Research Papers; Scintillation counters; scintillator detectors; Sensors; Spatial discrimination; Spatial resolution; SXD diffractometer; Wavelength; wavelength‐shifting fibre detector
• ISSN: 1600-5767; 0021-8898; 1600-5767
• DOI: 10.1107/S1600576724002462

Scintillator‐based ZnS:Ag/6LiF neutron detectors have been under development at ISIS for more than three decades. Continuous research and development aim to improve detector capabilities, achieve better performance and meet the increasingly demanding requirements set by neutron instruments. As part of this program, a high‐efficiency 2D position‐sensitive scintillator detector with wavelength‐shifting fibres has been developed for neutron‐diffraction applications. The detector consists of a double scintillator‐fibre layer to improve detection efficiency. Each layer is made up of two orthogonal fibre planes placed between two ZnS:Ag/6LiF scintillator screens. Thin reflective foils are attached to the front and back scintillators of each layer to minimize light cross‐talk between layers. The detector has an active area of 192 × 192 mm with a square pixel size of 3 × 3 mm. As part of the development process of the double‐layer detector, a single‐layer detector was built, together with a prototype detector in which the two layers of the detector could be read out separately. Efficiency calculations and measurements of all three detectors are discussed. The novel double‐layer detector has been installed and tested on the SXD diffractometer at ISIS. The detector performance is compared with the current scintillator detectors employed on SXD by studying reference crystal samples. More than a factor of 3 improvement in efficiency is achieved with the double‐layer wavelength‐shifting‐fibre detector. Software routines for further optimizations in spatial resolution and uniformity of response have been implemented and tested for 2D detectors. The methods and results are discussed in this manuscript. A novel high‐efficiency 2D position‐sensitive wavelength‐shifting‐fibre ZnS:Ag/6LiF scintillator detector has been developed at ISIS for single‐crystal diffraction applications. More than a factor of 3 improvement in efficiency was achieved with this detector compared with clear‐fibre scintillator detectors, and software routines for further optimizations in position sensitivity and uniformity have been implemented.