Electrical Control of Magnetic Resonance in Phase Change Materials

• Published in: Nano letters 2024-09, Vol.24 (37), p.11476-11481
• Main Authors: Chen, Tian-Yue, Ren, Haowen, Ghazikhanian, Nareg, Hage, Ralph El, Sasaki, Dayne Y., Salev, Pavel, Takamura, Yayoi, Schuller, Ivan K., Kent, Andrew D.
• Format: Article
• Language: English
• Subjects: Letter; magnetic properties; materials; MATERIALS SCIENCE; metal−insulator transition (MIT); phase separation; phase transitions; resonance structures; spin-torque ferromagnetic resonance; synaptic weights tuning; transition metal oxide; voltage-triggered MIT
• ISSN: 1530-6984; 1530-6992; 1530-6992
• DOI: 10.1021/acs.nanolett.4c02697

Metal–insulator transitions (MITs) in resistive switching materials can be triggered by an electric stimulus that produces significant changes in the electrical response. When these phases have distinct magnetic characteristics, dramatic changes in the spin excitations are also expected. The transition metal oxide La0.7Sr0.3MnO3 (LSMO) is a ferromagnetic metal at low temperatures and a paramagnetic insulator above room temperature. When LSMO is in its metallic phase, a critical electrical bias has been shown to lead to an MIT that results in the formation of a paramagnetic resistive barrier transverse to the applied electric field. Using spin-transfer ferromagnetic resonance spectroscopy, we show that even for electrical biases less than the critical value that triggers the MIT, there is magnetic phase separation, with the spin-excitation resonances varying systematically with applied bias. Therefore, voltage-triggered MITs in LSMO can alter magnetic resonance characteristics, offering an effective method for tuning synaptic weights in neuromorphic circuits.