Loading…

Carrier trapping and confinement in Ge nanocrystals surrounded by Ge3N4

We investigated the optical properties of Ge nanocrystals surrounded by Ge 3 N 4 . The broad emission ranging from infrared to blue is due to the dependence on the crystal size and preparation methods. Here, we report high resolution Photoluminescence (PL) attributed to emission from individual Ge n...

Full description

Saved in:
Bibliographic Details
Published in:Scientific reports 2016-05, Vol.6 (1), p.25449-25449, Article 25449
Main Authors: Park, Youngsin, Chan, Christopher C. S., Reid, Benjamin P. L., Nuttall, Luke, Taylor, Robert A., Lee, Nam-Suk, Lee, Young Mi
Format: Article
Language:English
Subjects:
Citations: Items that this one cites
Items that cite this one
Online Access:Get full text
Tags: Add Tag
No Tags, Be the first to tag this record!
cited_by cdi_FETCH-LOGICAL-c438t-91dcb1265bbeacd3dd5559c5f865aa1ed09dea6d92e35bc1748b3548131223ab3
cites cdi_FETCH-LOGICAL-c438t-91dcb1265bbeacd3dd5559c5f865aa1ed09dea6d92e35bc1748b3548131223ab3
container_end_page 25449
container_issue 1
container_start_page 25449
container_title Scientific reports
container_volume 6
creator Park, Youngsin
Chan, Christopher C. S.
Reid, Benjamin P. L.
Nuttall, Luke
Taylor, Robert A.
Lee, Nam-Suk
Lee, Young Mi
description We investigated the optical properties of Ge nanocrystals surrounded by Ge 3 N 4 . The broad emission ranging from infrared to blue is due to the dependence on the crystal size and preparation methods. Here, we report high resolution Photoluminescence (PL) attributed to emission from individual Ge nanocrystals ( nc -Ge) spatially resolved using micro-photoluminescence and detailed using temperature and power-dependent photoluminescence studies. The measured peaks are shown to behave with excitonic characteristics and we argue that the spread of the nc -Ge peaks in the PL spectrum is due to different confinement energies arising from the variation in size of the nanocrystals.
doi_str_mv 10.1038/srep25449
format article
fullrecord <record><control><sourceid>proquest_pubme</sourceid><recordid>TN_cdi_pubmedcentral_primary_oai_pubmedcentral_nih_gov_4857120</recordid><sourceformat>XML</sourceformat><sourcesystem>PC</sourcesystem><sourcerecordid>1787475581</sourcerecordid><originalsourceid>FETCH-LOGICAL-c438t-91dcb1265bbeacd3dd5559c5f865aa1ed09dea6d92e35bc1748b3548131223ab3</originalsourceid><addsrcrecordid>eNplkV9LwzAUxYMobsw9-AWk4IsK1eZfm7wIMnQKQ1_0OaRJOjvapCatsG9vZHNMvS-5cH6ce8IB4BRm1zDD7CZ40yFKCD8AY5QRmiKM0OHePgLTEFZZHIo4gfwYjFABSQE5HYP5THpfG5_0XnZdbZeJtDpRzla1Na2xfVLbZG4SK61Tfh162YQkDN67wWqjk3IdVfxMTsBRFSUz3b4T8PZw_zp7TBcv86fZ3SJVBLM-5VCrEqKclqWRSmOtKaVc0YrlVEpodMa1kbnmyGBaKlgQVmJKGMQQISxLPAG3G99uKFujVUzoZSM6X7fSr4WTtfit2PpdLN2nIIwWEGXR4GJr4N3HYEIv2joo0zTSGjcEAQtWkILSeHICzv-gKzd4G78nIOMxMcc5i9TlhlLehVhGtQsDM_HdkNg1FNmz_fQ78qePCFxtgBAluzR-7-Q_ty8v5JqX</addsrcrecordid><sourcetype>Open Access Repository</sourcetype><iscdi>true</iscdi><recordtype>article</recordtype><pqid>1898659368</pqid></control><display><type>article</type><title>Carrier trapping and confinement in Ge nanocrystals surrounded by Ge3N4</title><source>Publicly Available Content Database</source><source>PubMed Central</source><source>Free Full-Text Journals in Chemistry</source><source>Springer Nature - nature.com Journals - Fully Open Access</source><creator>Park, Youngsin ; Chan, Christopher C. S. ; Reid, Benjamin P. L. ; Nuttall, Luke ; Taylor, Robert A. ; Lee, Nam-Suk ; Lee, Young Mi</creator><creatorcontrib>Park, Youngsin ; Chan, Christopher C. S. ; Reid, Benjamin P. L. ; Nuttall, Luke ; Taylor, Robert A. ; Lee, Nam-Suk ; Lee, Young Mi</creatorcontrib><description>We investigated the optical properties of Ge nanocrystals surrounded by Ge 3 N 4 . The broad emission ranging from infrared to blue is due to the dependence on the crystal size and preparation methods. Here, we report high resolution Photoluminescence (PL) attributed to emission from individual Ge nanocrystals ( nc -Ge) spatially resolved using micro-photoluminescence and detailed using temperature and power-dependent photoluminescence studies. The measured peaks are shown to behave with excitonic characteristics and we argue that the spread of the nc -Ge peaks in the PL spectrum is due to different confinement energies arising from the variation in size of the nanocrystals.</description><identifier>ISSN: 2045-2322</identifier><identifier>EISSN: 2045-2322</identifier><identifier>DOI: 10.1038/srep25449</identifier><identifier>PMID: 27147195</identifier><language>eng</language><publisher>London: Nature Publishing Group UK</publisher><subject>639/766/1130/2799 ; 639/766/94 ; Annealing ; Crystals ; Emissions ; Energy ; Humanities and Social Sciences ; Laboratories ; Luminescence ; Microscopy ; multidisciplinary ; Nanocrystals ; Optical properties ; Photons ; Science ; Science (multidisciplinary) ; Temperature effects</subject><ispartof>Scientific reports, 2016-05, Vol.6 (1), p.25449-25449, Article 25449</ispartof><rights>The Author(s) 2016</rights><rights>Copyright Nature Publishing Group May 2016</rights><rights>Copyright © 2016, Macmillan Publishers Limited 2016 Macmillan Publishers Limited</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c438t-91dcb1265bbeacd3dd5559c5f865aa1ed09dea6d92e35bc1748b3548131223ab3</citedby><cites>FETCH-LOGICAL-c438t-91dcb1265bbeacd3dd5559c5f865aa1ed09dea6d92e35bc1748b3548131223ab3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://www.proquest.com/docview/1898659368/fulltextPDF?pq-origsite=primo$$EPDF$$P50$$Gproquest$$Hfree_for_read</linktopdf><linktohtml>$$Uhttps://www.proquest.com/docview/1898659368?pq-origsite=primo$$EHTML$$P50$$Gproquest$$Hfree_for_read</linktohtml><link.rule.ids>230,314,723,776,780,881,25731,27901,27902,36989,36990,44566,53766,53768,74869</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/27147195$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Park, Youngsin</creatorcontrib><creatorcontrib>Chan, Christopher C. S.</creatorcontrib><creatorcontrib>Reid, Benjamin P. L.</creatorcontrib><creatorcontrib>Nuttall, Luke</creatorcontrib><creatorcontrib>Taylor, Robert A.</creatorcontrib><creatorcontrib>Lee, Nam-Suk</creatorcontrib><creatorcontrib>Lee, Young Mi</creatorcontrib><title>Carrier trapping and confinement in Ge nanocrystals surrounded by Ge3N4</title><title>Scientific reports</title><addtitle>Sci Rep</addtitle><addtitle>Sci Rep</addtitle><description>We investigated the optical properties of Ge nanocrystals surrounded by Ge 3 N 4 . The broad emission ranging from infrared to blue is due to the dependence on the crystal size and preparation methods. Here, we report high resolution Photoluminescence (PL) attributed to emission from individual Ge nanocrystals ( nc -Ge) spatially resolved using micro-photoluminescence and detailed using temperature and power-dependent photoluminescence studies. The measured peaks are shown to behave with excitonic characteristics and we argue that the spread of the nc -Ge peaks in the PL spectrum is due to different confinement energies arising from the variation in size of the nanocrystals.</description><subject>639/766/1130/2799</subject><subject>639/766/94</subject><subject>Annealing</subject><subject>Crystals</subject><subject>Emissions</subject><subject>Energy</subject><subject>Humanities and Social Sciences</subject><subject>Laboratories</subject><subject>Luminescence</subject><subject>Microscopy</subject><subject>multidisciplinary</subject><subject>Nanocrystals</subject><subject>Optical properties</subject><subject>Photons</subject><subject>Science</subject><subject>Science (multidisciplinary)</subject><subject>Temperature effects</subject><issn>2045-2322</issn><issn>2045-2322</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2016</creationdate><recordtype>article</recordtype><sourceid>PIMPY</sourceid><recordid>eNplkV9LwzAUxYMobsw9-AWk4IsK1eZfm7wIMnQKQ1_0OaRJOjvapCatsG9vZHNMvS-5cH6ce8IB4BRm1zDD7CZ40yFKCD8AY5QRmiKM0OHePgLTEFZZHIo4gfwYjFABSQE5HYP5THpfG5_0XnZdbZeJtDpRzla1Na2xfVLbZG4SK61Tfh162YQkDN67wWqjk3IdVfxMTsBRFSUz3b4T8PZw_zp7TBcv86fZ3SJVBLM-5VCrEqKclqWRSmOtKaVc0YrlVEpodMa1kbnmyGBaKlgQVmJKGMQQISxLPAG3G99uKFujVUzoZSM6X7fSr4WTtfit2PpdLN2nIIwWEGXR4GJr4N3HYEIv2joo0zTSGjcEAQtWkILSeHICzv-gKzd4G78nIOMxMcc5i9TlhlLehVhGtQsDM_HdkNg1FNmz_fQ78qePCFxtgBAluzR-7-Q_ty8v5JqX</recordid><startdate>20160505</startdate><enddate>20160505</enddate><creator>Park, Youngsin</creator><creator>Chan, Christopher C. S.</creator><creator>Reid, Benjamin P. L.</creator><creator>Nuttall, Luke</creator><creator>Taylor, Robert A.</creator><creator>Lee, Nam-Suk</creator><creator>Lee, Young Mi</creator><general>Nature Publishing Group UK</general><general>Nature Publishing Group</general><scope>C6C</scope><scope>NPM</scope><scope>AAYXX</scope><scope>CITATION</scope><scope>3V.</scope><scope>7X7</scope><scope>7XB</scope><scope>88A</scope><scope>88E</scope><scope>88I</scope><scope>8FE</scope><scope>8FH</scope><scope>8FI</scope><scope>8FJ</scope><scope>8FK</scope><scope>ABUWG</scope><scope>AEUYN</scope><scope>AFKRA</scope><scope>AZQEC</scope><scope>BBNVY</scope><scope>BENPR</scope><scope>BHPHI</scope><scope>CCPQU</scope><scope>DWQXO</scope><scope>FYUFA</scope><scope>GHDGH</scope><scope>GNUQQ</scope><scope>HCIFZ</scope><scope>K9.</scope><scope>LK8</scope><scope>M0S</scope><scope>M1P</scope><scope>M2P</scope><scope>M7P</scope><scope>PIMPY</scope><scope>PQEST</scope><scope>PQQKQ</scope><scope>PQUKI</scope><scope>Q9U</scope><scope>7X8</scope><scope>5PM</scope></search><sort><creationdate>20160505</creationdate><title>Carrier trapping and confinement in Ge nanocrystals surrounded by Ge3N4</title><author>Park, Youngsin ; Chan, Christopher C. S. ; Reid, Benjamin P. L. ; Nuttall, Luke ; Taylor, Robert A. ; Lee, Nam-Suk ; Lee, Young Mi</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c438t-91dcb1265bbeacd3dd5559c5f865aa1ed09dea6d92e35bc1748b3548131223ab3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2016</creationdate><topic>639/766/1130/2799</topic><topic>639/766/94</topic><topic>Annealing</topic><topic>Crystals</topic><topic>Emissions</topic><topic>Energy</topic><topic>Humanities and Social Sciences</topic><topic>Laboratories</topic><topic>Luminescence</topic><topic>Microscopy</topic><topic>multidisciplinary</topic><topic>Nanocrystals</topic><topic>Optical properties</topic><topic>Photons</topic><topic>Science</topic><topic>Science (multidisciplinary)</topic><topic>Temperature effects</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Park, Youngsin</creatorcontrib><creatorcontrib>Chan, Christopher C. S.</creatorcontrib><creatorcontrib>Reid, Benjamin P. L.</creatorcontrib><creatorcontrib>Nuttall, Luke</creatorcontrib><creatorcontrib>Taylor, Robert A.</creatorcontrib><creatorcontrib>Lee, Nam-Suk</creatorcontrib><creatorcontrib>Lee, Young Mi</creatorcontrib><collection>Springer Nature OA Free Journals</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>ProQuest Central (Corporate)</collection><collection>Health &amp; Medical Collection</collection><collection>ProQuest Central (purchase pre-March 2016)</collection><collection>Biology Database (Alumni Edition)</collection><collection>Medical Database (Alumni Edition)</collection><collection>Science Database (Alumni Edition)</collection><collection>ProQuest SciTech Collection</collection><collection>ProQuest Natural Science Collection</collection><collection>Hospital Premium Collection</collection><collection>Hospital Premium Collection (Alumni Edition)</collection><collection>ProQuest Central (Alumni) (purchase pre-March 2016)</collection><collection>ProQuest Central (Alumni)</collection><collection>ProQuest One Sustainability</collection><collection>ProQuest Central</collection><collection>ProQuest Central Essentials</collection><collection>Biological Science Collection</collection><collection>ProQuest Central</collection><collection>Natural Science Collection</collection><collection>ProQuest One Community College</collection><collection>ProQuest Central</collection><collection>Health Research Premium Collection</collection><collection>Health Research Premium Collection (Alumni)</collection><collection>ProQuest Central Student</collection><collection>SciTech Premium Collection</collection><collection>ProQuest Health &amp; Medical Complete (Alumni)</collection><collection>Biological Sciences</collection><collection>Health &amp; Medical Collection (Alumni Edition)</collection><collection>PML(ProQuest Medical Library)</collection><collection>Science Database</collection><collection>Biological Science Database</collection><collection>Publicly Available Content Database</collection><collection>ProQuest One Academic Eastern Edition (DO NOT USE)</collection><collection>ProQuest One Academic</collection><collection>ProQuest One Academic UKI Edition</collection><collection>ProQuest Central Basic</collection><collection>MEDLINE - Academic</collection><collection>PubMed Central (Full Participant titles)</collection><jtitle>Scientific reports</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Park, Youngsin</au><au>Chan, Christopher C. S.</au><au>Reid, Benjamin P. L.</au><au>Nuttall, Luke</au><au>Taylor, Robert A.</au><au>Lee, Nam-Suk</au><au>Lee, Young Mi</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Carrier trapping and confinement in Ge nanocrystals surrounded by Ge3N4</atitle><jtitle>Scientific reports</jtitle><stitle>Sci Rep</stitle><addtitle>Sci Rep</addtitle><date>2016-05-05</date><risdate>2016</risdate><volume>6</volume><issue>1</issue><spage>25449</spage><epage>25449</epage><pages>25449-25449</pages><artnum>25449</artnum><issn>2045-2322</issn><eissn>2045-2322</eissn><abstract>We investigated the optical properties of Ge nanocrystals surrounded by Ge 3 N 4 . The broad emission ranging from infrared to blue is due to the dependence on the crystal size and preparation methods. Here, we report high resolution Photoluminescence (PL) attributed to emission from individual Ge nanocrystals ( nc -Ge) spatially resolved using micro-photoluminescence and detailed using temperature and power-dependent photoluminescence studies. The measured peaks are shown to behave with excitonic characteristics and we argue that the spread of the nc -Ge peaks in the PL spectrum is due to different confinement energies arising from the variation in size of the nanocrystals.</abstract><cop>London</cop><pub>Nature Publishing Group UK</pub><pmid>27147195</pmid><doi>10.1038/srep25449</doi><tpages>1</tpages><oa>free_for_read</oa></addata></record>
fulltext fulltext
identifier ISSN: 2045-2322
ispartof Scientific reports, 2016-05, Vol.6 (1), p.25449-25449, Article 25449
issn 2045-2322
2045-2322
language eng
recordid cdi_pubmedcentral_primary_oai_pubmedcentral_nih_gov_4857120
source Publicly Available Content Database; PubMed Central; Free Full-Text Journals in Chemistry; Springer Nature - nature.com Journals - Fully Open Access
subjects 639/766/1130/2799
639/766/94
Annealing
Crystals
Emissions
Energy
Humanities and Social Sciences
Laboratories
Luminescence
Microscopy
multidisciplinary
Nanocrystals
Optical properties
Photons
Science
Science (multidisciplinary)
Temperature effects
title Carrier trapping and confinement in Ge nanocrystals surrounded by Ge3N4
url http://sfxeu10.hosted.exlibrisgroup.com/loughborough?ctx_ver=Z39.88-2004&ctx_enc=info:ofi/enc:UTF-8&ctx_tim=2025-02-06T16%3A42%3A35IST&url_ver=Z39.88-2004&url_ctx_fmt=infofi/fmt:kev:mtx:ctx&rfr_id=info:sid/primo.exlibrisgroup.com:primo3-Article-proquest_pubme&rft_val_fmt=info:ofi/fmt:kev:mtx:journal&rft.genre=article&rft.atitle=Carrier%20trapping%20and%20confinement%20in%20Ge%20nanocrystals%20surrounded%20by%20Ge3N4&rft.jtitle=Scientific%20reports&rft.au=Park,%20Youngsin&rft.date=2016-05-05&rft.volume=6&rft.issue=1&rft.spage=25449&rft.epage=25449&rft.pages=25449-25449&rft.artnum=25449&rft.issn=2045-2322&rft.eissn=2045-2322&rft_id=info:doi/10.1038/srep25449&rft_dat=%3Cproquest_pubme%3E1787475581%3C/proquest_pubme%3E%3Cgrp_id%3Ecdi_FETCH-LOGICAL-c438t-91dcb1265bbeacd3dd5559c5f865aa1ed09dea6d92e35bc1748b3548131223ab3%3C/grp_id%3E%3Coa%3E%3C/oa%3E%3Curl%3E%3C/url%3E&rft_id=info:oai/&rft_pqid=1898659368&rft_id=info:pmid/27147195&rfr_iscdi=true