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Carrier trapping and confinement in Ge nanocrystals surrounded by Ge3N4
We investigated the optical properties of Ge nanocrystals surrounded by Ge 3 N 4 . The broad emission ranging from infrared to blue is due to the dependence on the crystal size and preparation methods. Here, we report high resolution Photoluminescence (PL) attributed to emission from individual Ge n...
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Published in: | Scientific reports 2016-05, Vol.6 (1), p.25449-25449, Article 25449 |
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creator | Park, Youngsin Chan, Christopher C. S. Reid, Benjamin P. L. Nuttall, Luke Taylor, Robert A. Lee, Nam-Suk Lee, Young Mi |
description | We investigated the optical properties of Ge nanocrystals surrounded by Ge
3
N
4
. The broad emission ranging from infrared to blue is due to the dependence on the crystal size and preparation methods. Here, we report high resolution Photoluminescence (PL) attributed to emission from individual Ge nanocrystals (
nc
-Ge) spatially resolved using micro-photoluminescence and detailed using temperature and power-dependent photoluminescence studies. The measured peaks are shown to behave with excitonic characteristics and we argue that the spread of the
nc
-Ge peaks in the PL spectrum is due to different confinement energies arising from the variation in size of the nanocrystals. |
doi_str_mv | 10.1038/srep25449 |
format | article |
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3
N
4
. The broad emission ranging from infrared to blue is due to the dependence on the crystal size and preparation methods. Here, we report high resolution Photoluminescence (PL) attributed to emission from individual Ge nanocrystals (
nc
-Ge) spatially resolved using micro-photoluminescence and detailed using temperature and power-dependent photoluminescence studies. The measured peaks are shown to behave with excitonic characteristics and we argue that the spread of the
nc
-Ge peaks in the PL spectrum is due to different confinement energies arising from the variation in size of the nanocrystals.</description><identifier>ISSN: 2045-2322</identifier><identifier>EISSN: 2045-2322</identifier><identifier>DOI: 10.1038/srep25449</identifier><identifier>PMID: 27147195</identifier><language>eng</language><publisher>London: Nature Publishing Group UK</publisher><subject>639/766/1130/2799 ; 639/766/94 ; Annealing ; Crystals ; Emissions ; Energy ; Humanities and Social Sciences ; Laboratories ; Luminescence ; Microscopy ; multidisciplinary ; Nanocrystals ; Optical properties ; Photons ; Science ; Science (multidisciplinary) ; Temperature effects</subject><ispartof>Scientific reports, 2016-05, Vol.6 (1), p.25449-25449, Article 25449</ispartof><rights>The Author(s) 2016</rights><rights>Copyright Nature Publishing Group May 2016</rights><rights>Copyright © 2016, Macmillan Publishers Limited 2016 Macmillan Publishers Limited</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c438t-91dcb1265bbeacd3dd5559c5f865aa1ed09dea6d92e35bc1748b3548131223ab3</citedby><cites>FETCH-LOGICAL-c438t-91dcb1265bbeacd3dd5559c5f865aa1ed09dea6d92e35bc1748b3548131223ab3</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://www.proquest.com/docview/1898659368/fulltextPDF?pq-origsite=primo$$EPDF$$P50$$Gproquest$$Hfree_for_read</linktopdf><linktohtml>$$Uhttps://www.proquest.com/docview/1898659368?pq-origsite=primo$$EHTML$$P50$$Gproquest$$Hfree_for_read</linktohtml><link.rule.ids>230,314,723,776,780,881,25731,27901,27902,36989,36990,44566,53766,53768,74869</link.rule.ids><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/27147195$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Park, Youngsin</creatorcontrib><creatorcontrib>Chan, Christopher C. S.</creatorcontrib><creatorcontrib>Reid, Benjamin P. L.</creatorcontrib><creatorcontrib>Nuttall, Luke</creatorcontrib><creatorcontrib>Taylor, Robert A.</creatorcontrib><creatorcontrib>Lee, Nam-Suk</creatorcontrib><creatorcontrib>Lee, Young Mi</creatorcontrib><title>Carrier trapping and confinement in Ge nanocrystals surrounded by Ge3N4</title><title>Scientific reports</title><addtitle>Sci Rep</addtitle><addtitle>Sci Rep</addtitle><description>We investigated the optical properties of Ge nanocrystals surrounded by Ge
3
N
4
. The broad emission ranging from infrared to blue is due to the dependence on the crystal size and preparation methods. Here, we report high resolution Photoluminescence (PL) attributed to emission from individual Ge nanocrystals (
nc
-Ge) spatially resolved using micro-photoluminescence and detailed using temperature and power-dependent photoluminescence studies. The measured peaks are shown to behave with excitonic characteristics and we argue that the spread of the
nc
-Ge peaks in the PL spectrum is due to different confinement energies arising from the variation in size of the nanocrystals.</description><subject>639/766/1130/2799</subject><subject>639/766/94</subject><subject>Annealing</subject><subject>Crystals</subject><subject>Emissions</subject><subject>Energy</subject><subject>Humanities and Social Sciences</subject><subject>Laboratories</subject><subject>Luminescence</subject><subject>Microscopy</subject><subject>multidisciplinary</subject><subject>Nanocrystals</subject><subject>Optical properties</subject><subject>Photons</subject><subject>Science</subject><subject>Science (multidisciplinary)</subject><subject>Temperature effects</subject><issn>2045-2322</issn><issn>2045-2322</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2016</creationdate><recordtype>article</recordtype><sourceid>PIMPY</sourceid><recordid>eNplkV9LwzAUxYMobsw9-AWk4IsK1eZfm7wIMnQKQ1_0OaRJOjvapCatsG9vZHNMvS-5cH6ce8IB4BRm1zDD7CZ40yFKCD8AY5QRmiKM0OHePgLTEFZZHIo4gfwYjFABSQE5HYP5THpfG5_0XnZdbZeJtDpRzla1Na2xfVLbZG4SK61Tfh162YQkDN67wWqjk3IdVfxMTsBRFSUz3b4T8PZw_zp7TBcv86fZ3SJVBLM-5VCrEqKclqWRSmOtKaVc0YrlVEpodMa1kbnmyGBaKlgQVmJKGMQQISxLPAG3G99uKFujVUzoZSM6X7fSr4WTtfit2PpdLN2nIIwWEGXR4GJr4N3HYEIv2joo0zTSGjcEAQtWkILSeHICzv-gKzd4G78nIOMxMcc5i9TlhlLehVhGtQsDM_HdkNg1FNmz_fQ78qePCFxtgBAluzR-7-Q_ty8v5JqX</recordid><startdate>20160505</startdate><enddate>20160505</enddate><creator>Park, Youngsin</creator><creator>Chan, Christopher C. 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S. ; Reid, Benjamin P. L. ; Nuttall, Luke ; Taylor, Robert A. ; Lee, Nam-Suk ; Lee, Young Mi</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-c438t-91dcb1265bbeacd3dd5559c5f865aa1ed09dea6d92e35bc1748b3548131223ab3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2016</creationdate><topic>639/766/1130/2799</topic><topic>639/766/94</topic><topic>Annealing</topic><topic>Crystals</topic><topic>Emissions</topic><topic>Energy</topic><topic>Humanities and Social Sciences</topic><topic>Laboratories</topic><topic>Luminescence</topic><topic>Microscopy</topic><topic>multidisciplinary</topic><topic>Nanocrystals</topic><topic>Optical properties</topic><topic>Photons</topic><topic>Science</topic><topic>Science (multidisciplinary)</topic><topic>Temperature effects</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Park, Youngsin</creatorcontrib><creatorcontrib>Chan, Christopher C. S.</creatorcontrib><creatorcontrib>Reid, Benjamin P. 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S.</au><au>Reid, Benjamin P. L.</au><au>Nuttall, Luke</au><au>Taylor, Robert A.</au><au>Lee, Nam-Suk</au><au>Lee, Young Mi</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Carrier trapping and confinement in Ge nanocrystals surrounded by Ge3N4</atitle><jtitle>Scientific reports</jtitle><stitle>Sci Rep</stitle><addtitle>Sci Rep</addtitle><date>2016-05-05</date><risdate>2016</risdate><volume>6</volume><issue>1</issue><spage>25449</spage><epage>25449</epage><pages>25449-25449</pages><artnum>25449</artnum><issn>2045-2322</issn><eissn>2045-2322</eissn><abstract>We investigated the optical properties of Ge nanocrystals surrounded by Ge
3
N
4
. The broad emission ranging from infrared to blue is due to the dependence on the crystal size and preparation methods. Here, we report high resolution Photoluminescence (PL) attributed to emission from individual Ge nanocrystals (
nc
-Ge) spatially resolved using micro-photoluminescence and detailed using temperature and power-dependent photoluminescence studies. The measured peaks are shown to behave with excitonic characteristics and we argue that the spread of the
nc
-Ge peaks in the PL spectrum is due to different confinement energies arising from the variation in size of the nanocrystals.</abstract><cop>London</cop><pub>Nature Publishing Group UK</pub><pmid>27147195</pmid><doi>10.1038/srep25449</doi><tpages>1</tpages><oa>free_for_read</oa></addata></record> |
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source | Publicly Available Content Database; PubMed Central; Free Full-Text Journals in Chemistry; Springer Nature - nature.com Journals - Fully Open Access |
subjects | 639/766/1130/2799 639/766/94 Annealing Crystals Emissions Energy Humanities and Social Sciences Laboratories Luminescence Microscopy multidisciplinary Nanocrystals Optical properties Photons Science Science (multidisciplinary) Temperature effects |
title | Carrier trapping and confinement in Ge nanocrystals surrounded by Ge3N4 |
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