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Abrupt change of the superconducting gap structure at the nematic critical point in FeSe1—xSₓ
The emergence of the nematic electronic state that breaks rotational symmetry is one of the most fascinating properties of the iron-based superconductors, and has relevance to cuprates as well. FeSe has a unique ground state in which superconductivity coexists with a nematic order without long-range...
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Published in: | Proceedings of the National Academy of Sciences - PNAS 2018-02, Vol.115 (6), p.1227-1231 |
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container_title | Proceedings of the National Academy of Sciences - PNAS |
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creator | Sato, Yuki Kasahara, Shigeru Taniguchi, Tomoya Xing, Xiangzhuo Kasahara, Yuichi Tokiwa, Yoshifumi Yamakawa, Youichi Kontani, Hiroshi Shibauchi, Takasada Matsuda, Yuji |
description | The emergence of the nematic electronic state that breaks rotational symmetry is one of the most fascinating properties of the iron-based superconductors, and has relevance to cuprates as well. FeSe has a unique ground state in which superconductivity coexists with a nematic order without long-range magnetic ordering, providing a significant opportunity to investigate the role of nematicity in the superconducting pairing interaction. Here, to reveal how the superconducting gap evolves with nematicity, we measure the thermal conductivity and specific heat of FeSe1—xSₓ, in which the nematicity is suppressed by isoelectronic sulfur substitution and a nematic critical point (NCP) appears at xc
≈ 0.17. We find that, in the whole nematic regime (0 < x |
doi_str_mv | 10.1073/pnas.1717331115 |
format | article |
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≈ 0.17. We find that, in the whole nematic regime (0 < x <0.17), the field dependence of two quantities consistently shows two-gap behavior; one gap is small but highly anisotropic with deep minima or line nodes, and the other is larger and more isotropic. In stark contrast, in the tetragonal regime (x = 0.20), the larger gap becomes strongly anisotropic, demonstrating an abrupt change in the superconducting gap structure at the NCP. Near the NCP, charge fluctuations of dxz
and dyz
orbitals are enhanced equally in the tetragonal side, whereas they develop differently in the orthorhombic side. Our observation therefore directly implies that the orbital-dependent nature of the nematic fluctuations has a strong impact on the superconducting gap structure and hence on the pairing interaction.</description><identifier>ISSN: 0027-8424</identifier><identifier>EISSN: 1091-6490</identifier><identifier>DOI: 10.1073/pnas.1717331115</identifier><identifier>PMID: 29363600</identifier><language>eng</language><publisher>National Academy of Sciences</publisher><subject>Physical Sciences</subject><ispartof>Proceedings of the National Academy of Sciences - PNAS, 2018-02, Vol.115 (6), p.1227-1231</ispartof><rights>Volumes 1–89 and 106–114, copyright as a collective work only; author(s) retains copyright to individual articles</rights><rights>2018</rights><lds50>peer_reviewed</lds50><oa>free_for_read</oa><woscitedreferencessubscribed>false</woscitedreferencessubscribed></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><linktopdf>$$Uhttps://www.jstor.org/stable/pdf/26507164$$EPDF$$P50$$Gjstor$$H</linktopdf><linktohtml>$$Uhttps://www.jstor.org/stable/26507164$$EHTML$$P50$$Gjstor$$H</linktohtml><link.rule.ids>230,314,727,780,784,885,27923,27924,53790,53792,58237,58470</link.rule.ids></links><search><creatorcontrib>Sato, Yuki</creatorcontrib><creatorcontrib>Kasahara, Shigeru</creatorcontrib><creatorcontrib>Taniguchi, Tomoya</creatorcontrib><creatorcontrib>Xing, Xiangzhuo</creatorcontrib><creatorcontrib>Kasahara, Yuichi</creatorcontrib><creatorcontrib>Tokiwa, Yoshifumi</creatorcontrib><creatorcontrib>Yamakawa, Youichi</creatorcontrib><creatorcontrib>Kontani, Hiroshi</creatorcontrib><creatorcontrib>Shibauchi, Takasada</creatorcontrib><creatorcontrib>Matsuda, Yuji</creatorcontrib><title>Abrupt change of the superconducting gap structure at the nematic critical point in FeSe1—xSₓ</title><title>Proceedings of the National Academy of Sciences - PNAS</title><description>The emergence of the nematic electronic state that breaks rotational symmetry is one of the most fascinating properties of the iron-based superconductors, and has relevance to cuprates as well. FeSe has a unique ground state in which superconductivity coexists with a nematic order without long-range magnetic ordering, providing a significant opportunity to investigate the role of nematicity in the superconducting pairing interaction. Here, to reveal how the superconducting gap evolves with nematicity, we measure the thermal conductivity and specific heat of FeSe1—xSₓ, in which the nematicity is suppressed by isoelectronic sulfur substitution and a nematic critical point (NCP) appears at xc
≈ 0.17. We find that, in the whole nematic regime (0 < x <0.17), the field dependence of two quantities consistently shows two-gap behavior; one gap is small but highly anisotropic with deep minima or line nodes, and the other is larger and more isotropic. In stark contrast, in the tetragonal regime (x = 0.20), the larger gap becomes strongly anisotropic, demonstrating an abrupt change in the superconducting gap structure at the NCP. Near the NCP, charge fluctuations of dxz
and dyz
orbitals are enhanced equally in the tetragonal side, whereas they develop differently in the orthorhombic side. Our observation therefore directly implies that the orbital-dependent nature of the nematic fluctuations has a strong impact on the superconducting gap structure and hence on the pairing interaction.</description><subject>Physical Sciences</subject><issn>0027-8424</issn><issn>1091-6490</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2018</creationdate><recordtype>article</recordtype><recordid>eNpVjsFq3DAURUVoaKZp11kVtOzG0yfLkqxNYRiatDCQRZK1keTnGQ0e2ZXkku5CfiH5wnxJTBMCWV0e93DeJeSMwZKB4t_HYNKSKaY4Z4yJI7JgoFkhKw0fyAKgVEVdldUJ-ZTSHgC0qOEjOSk1l1wCLIhZ2TiNmbqdCVukQ0fzDmmaRoxuCO3ksg9bujUjTTnO1xSRmvwfCngw2Tvqop_D9HQcfMjUB3qOV8ie7h5vr57uHz6T4870Cb-85im5Of95vf5VbC4vfq9Xm2I_b89FJ8pWOqusVhbBYi0QWN0ayTumwHaOl6JCLlvTtkpbXVrBTdkZiRzqGh0_JT9evONkD9g6DDmavhmjP5j4rxmMb943we-a7fC3ETXTFeez4NurIA5_Jky5OfjksO9NwGFKDdMaaqFkpWb06wu6T3mIbz9KKUAxWfFndCR-6g</recordid><startdate>20180206</startdate><enddate>20180206</enddate><creator>Sato, Yuki</creator><creator>Kasahara, Shigeru</creator><creator>Taniguchi, Tomoya</creator><creator>Xing, Xiangzhuo</creator><creator>Kasahara, Yuichi</creator><creator>Tokiwa, Yoshifumi</creator><creator>Yamakawa, Youichi</creator><creator>Kontani, Hiroshi</creator><creator>Shibauchi, Takasada</creator><creator>Matsuda, Yuji</creator><general>National Academy of Sciences</general><scope>7X8</scope><scope>5PM</scope></search><sort><creationdate>20180206</creationdate><title>Abrupt change of the superconducting gap structure at the nematic critical point in FeSe1—xSₓ</title><author>Sato, Yuki ; Kasahara, Shigeru ; Taniguchi, Tomoya ; Xing, Xiangzhuo ; Kasahara, Yuichi ; Tokiwa, Yoshifumi ; Yamakawa, Youichi ; Kontani, Hiroshi ; Shibauchi, Takasada ; Matsuda, Yuji</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-j331t-f52d6cb7b97be0be85e018da63f170bfc3254e36dadd79b92b53a2fa6e3088ec3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2018</creationdate><topic>Physical Sciences</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Sato, Yuki</creatorcontrib><creatorcontrib>Kasahara, Shigeru</creatorcontrib><creatorcontrib>Taniguchi, Tomoya</creatorcontrib><creatorcontrib>Xing, Xiangzhuo</creatorcontrib><creatorcontrib>Kasahara, Yuichi</creatorcontrib><creatorcontrib>Tokiwa, Yoshifumi</creatorcontrib><creatorcontrib>Yamakawa, Youichi</creatorcontrib><creatorcontrib>Kontani, Hiroshi</creatorcontrib><creatorcontrib>Shibauchi, Takasada</creatorcontrib><creatorcontrib>Matsuda, Yuji</creatorcontrib><collection>MEDLINE - Academic</collection><collection>PubMed Central (Full Participant titles)</collection><jtitle>Proceedings of the National Academy of Sciences - PNAS</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Sato, Yuki</au><au>Kasahara, Shigeru</au><au>Taniguchi, Tomoya</au><au>Xing, Xiangzhuo</au><au>Kasahara, Yuichi</au><au>Tokiwa, Yoshifumi</au><au>Yamakawa, Youichi</au><au>Kontani, Hiroshi</au><au>Shibauchi, Takasada</au><au>Matsuda, Yuji</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Abrupt change of the superconducting gap structure at the nematic critical point in FeSe1—xSₓ</atitle><jtitle>Proceedings of the National Academy of Sciences - PNAS</jtitle><date>2018-02-06</date><risdate>2018</risdate><volume>115</volume><issue>6</issue><spage>1227</spage><epage>1231</epage><pages>1227-1231</pages><issn>0027-8424</issn><eissn>1091-6490</eissn><abstract>The emergence of the nematic electronic state that breaks rotational symmetry is one of the most fascinating properties of the iron-based superconductors, and has relevance to cuprates as well. FeSe has a unique ground state in which superconductivity coexists with a nematic order without long-range magnetic ordering, providing a significant opportunity to investigate the role of nematicity in the superconducting pairing interaction. Here, to reveal how the superconducting gap evolves with nematicity, we measure the thermal conductivity and specific heat of FeSe1—xSₓ, in which the nematicity is suppressed by isoelectronic sulfur substitution and a nematic critical point (NCP) appears at xc
≈ 0.17. We find that, in the whole nematic regime (0 < x <0.17), the field dependence of two quantities consistently shows two-gap behavior; one gap is small but highly anisotropic with deep minima or line nodes, and the other is larger and more isotropic. In stark contrast, in the tetragonal regime (x = 0.20), the larger gap becomes strongly anisotropic, demonstrating an abrupt change in the superconducting gap structure at the NCP. Near the NCP, charge fluctuations of dxz
and dyz
orbitals are enhanced equally in the tetragonal side, whereas they develop differently in the orthorhombic side. Our observation therefore directly implies that the orbital-dependent nature of the nematic fluctuations has a strong impact on the superconducting gap structure and hence on the pairing interaction.</abstract><pub>National Academy of Sciences</pub><pmid>29363600</pmid><doi>10.1073/pnas.1717331115</doi><tpages>5</tpages><oa>free_for_read</oa></addata></record> |
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title | Abrupt change of the superconducting gap structure at the nematic critical point in FeSe1—xSₓ |
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