Role of wavelength in photocarrier absorption and plasma formation threshold under excitation of dielectrics by high-intensity laser field tunable from visible to mid-IR

• Published in: Scientific reports 2020-08, Vol.10 (1), p.14007-14007, Article 14007
• Main Authors: Migal, Ekaterina, Mareev, Evgenii, Smetanina, Evgeniya, Duchateau, Guillaume, Potemkin, Fedor
• Format: Article
• Language: English
• Subjects: 639/301/119/995; 639/624/400/385; 639/624/400/584; 639/766/1960/1135; Absorption; Humanities and Social Sciences; Lasers; multidisciplinary; Science; Science (multidisciplinary); Silicon dioxide; Wavelength; Wavelengths
• ISSN: 2045-2322; 2045-2322
• DOI: 10.1038/s41598-020-70862-w

The development of high power mid-IR laser applications requires a study on laser induced damage threshold (LIDT) in the mid-IR. In this paper we have measured the wavelength dependence of the plasma formation threshold (PFT) that is a LIDT precursor. In order to interpret the observed trends numerically, a model describing the laser induced electron dynamics, based on multiple rate equations, has been developed. We show both theoretically and experimentally that PFT at mid-IR wavelengths is controlled by a transition from weak- to strong-field regime of free carrier absorption. In the case of MgF 2 this transition occurs around 3–4  μ m corresponding to the region of the lowermost PFT. The region of the uppermost PFT is reached around 1  μ m and is governed by an interplay of photoionization and weak-field free carrier absorption which manifests itself in both MgF 2 and SiO 2 . The PFT observed in considered materials exhibits a universal dependence on the excitation wavelength in dielectrics. Thus, the presented results pave the route towards efficient and controllable laser-induced material modifications and should be of direct interest to laser researchers and application engineers for prevention of laser-induced damage of optical components in high-intensity mid-IR laser systems.