Crystalline shielding mitigates structural rearrangement and localizes memory in jammed systems under oscillatory shear

The nature of yield in amorphous materials under stress has yet to be fully elucidated. In particular, understanding how microscopic rearrangement gives rise to macroscopic structural and rheological signatures in disordered systems is vital for the prediction and characterization of yield and the s...

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Bibliographic Details
Published in:Science advances 2021-05, Vol.7 (20)
Main Authors: Teich, Erin G, Galloway, K Lawrence, Arratia, Paulo E, Bassett, Danielle S
Format: Article
Language:English
Subjects:
Condensed Matter Physics
Materials Science
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Summary:The nature of yield in amorphous materials under stress has yet to be fully elucidated. In particular, understanding how microscopic rearrangement gives rise to macroscopic structural and rheological signatures in disordered systems is vital for the prediction and characterization of yield and the study of how memory is stored in disordered materials. Here, we investigate the evolution of local structural homogeneity on an individual particle level in amorphous jammed two-dimensional (athermal) systems under oscillatory shear and relate this evolution to rearrangement, memory, and macroscale rheological measurements. We define the structural metric crystalline shielding, and show that it is predictive of rearrangement propensity and structural volatility of individual particles under shear. We use this metric to identify localized regions of the system in which the material's memory of its preparation is preserved. Our results contribute to a growing understanding of how local structure relates to dynamic response and memory in disordered systems.
ISSN:2375-2548
2375-2548
DOI:10.1126/sciadv.abe3392