Anisotropic dynamics of two-photon ionization: An attosecond movie of photoemission

Imaging in real time the complete dynamics of a process as fundamental as photoemission has long been out of reach because of the difficulty of combining attosecond temporal resolution with fine spectral and angular resolutions. Here, we achieve full decoding of the intricate angle-dependent dynamic...

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Published in:Science advances 2022-03, Vol.8 (12), p.eabl7594-eabl7594
Main Authors: Autuori, Alice, Platzer, Dominique, Lejman, Mariusz, Gallician, Guillaume, Maëder, Lucie, Covolo, Antoine, Bosse, Lea, Dalui, Malay, Bresteau, David, Hergott, Jean-François, Tcherbakoff, Olivier, Marroux, Hugo J B, Loriot, Vincent, Lépine, Franck, Poisson, Lionel, Taïeb, Richard, Caillat, Jérémie, Salières, Pascal
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cited_by cdi_FETCH-LOGICAL-c424t-ea5f8a4e43d6f5407f1058f8c641bc10bf0e79a886387582b69ae544a7fa1e453
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container_issue 12
container_start_page eabl7594
container_title Science advances
container_volume 8
creator Autuori, Alice
Platzer, Dominique
Lejman, Mariusz
Gallician, Guillaume
Maëder, Lucie
Covolo, Antoine
Bosse, Lea
Dalui, Malay
Bresteau, David
Hergott, Jean-François
Tcherbakoff, Olivier
Marroux, Hugo J B
Loriot, Vincent
Lépine, Franck
Poisson, Lionel
Taïeb, Richard
Caillat, Jérémie
Salières, Pascal
description Imaging in real time the complete dynamics of a process as fundamental as photoemission has long been out of reach because of the difficulty of combining attosecond temporal resolution with fine spectral and angular resolutions. Here, we achieve full decoding of the intricate angle-dependent dynamics of a photoemission process in helium, spectrally and anisotropically structured by two-photon transitions through intermediate bound states. Using spectrally and angularly resolved attosecond electron interferometry, we characterize the complex-valued transition probability amplitude toward the photoelectron quantum state. This allows reconstructing in space, time, and energy the complete formation of the photoionized wave packet.
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subjects Applied Physics
Chemical Sciences
or physical chemistry
Physical and Materials Sciences
SciAdv r-articles
Theoretical and
title Anisotropic dynamics of two-photon ionization: An attosecond movie of photoemission
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