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Synergetic photoluminescence enhancement of monolayer MoS2via surface plasmon resonance and defect repair
The weak light-absorption and low quantum yield (QY) in monolayer MoS2 are great challenges for the applications of this material in practical optoelectronic devices. Here, we report on a synergistic strategy to obtain highly enhanced photoluminescence (PL) of monolayer MoS2 by simultaneously improv...
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Published in: | RSC advances 2018-01, Vol.8 (42), p.23591-23598 |
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creator | Zeng, Yi Chen, Weibing Tang, Bin Liao, Jianhui Lou, Jun Chen, Qing |
description | The weak light-absorption and low quantum yield (QY) in monolayer MoS2 are great challenges for the applications of this material in practical optoelectronic devices. Here, we report on a synergistic strategy to obtain highly enhanced photoluminescence (PL) of monolayer MoS2 by simultaneously improving the intensity of the electromagnetic field around MoS2 and the QY of MoS2. Self-assembled sub-monolayer Au nanoparticles underneath the monolayer MoS2 and bis(trifluoromethane)sulfonimide (TFSI) treatment to the MoS2 surface are used to boost the excitation field and the QY, respectively. An enhancement factor of the PL intensity as high as 280 is achieved. The enhancement mechanisms are analyzed by inspecting the contribution of the PL spectra from A excitons and A− trions under different conditions. Our study takes a further step to developing high-performance optoelectronic devices based on monolayer MoS2. |
doi_str_mv | 10.1039/c8ra03779e |
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Here, we report on a synergistic strategy to obtain highly enhanced photoluminescence (PL) of monolayer MoS2 by simultaneously improving the intensity of the electromagnetic field around MoS2 and the QY of MoS2. Self-assembled sub-monolayer Au nanoparticles underneath the monolayer MoS2 and bis(trifluoromethane)sulfonimide (TFSI) treatment to the MoS2 surface are used to boost the excitation field and the QY, respectively. An enhancement factor of the PL intensity as high as 280 is achieved. The enhancement mechanisms are analyzed by inspecting the contribution of the PL spectra from A excitons and A− trions under different conditions. 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Our study takes a further step to developing high-performance optoelectronic devices based on monolayer MoS2.</description><subject>Chemistry</subject><subject>Electromagnetic fields</subject><subject>Excitation spectra</subject><subject>Gold</subject><subject>Molybdenum disulfide</subject><subject>Monolayers</subject><subject>Optoelectronic devices</subject><subject>Photoluminescence</subject><subject>Self-assembly</subject><subject>Surface plasmon resonance</subject><subject>Trifluoromethane</subject><subject>Trions</subject><issn>2046-2069</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2018</creationdate><recordtype>article</recordtype><recordid>eNpVkMtqwzAQRUWhNCHNpl8g6DqtHrYem0IJfUFKF2nXRpbHiYItuZIdyN9Xpdl0NhfmzhzuDEI3lNxRwvW9VdEQLqWGCzRnpBArRoSeoWVKB5JLlJQJeoVmvCwLwpSYI7c9eYg7GJ3Fwz6MoZt65yFZ8BYw-L3J2oMfcWhxH3zozAkifg9bdnQGpym2Jg8OnUnZxRFS8L8r2PgGN9CCHXNzMC5eo8vWdAmWZ12gr-enz_XravPx8rZ-3KwOVJWwqq0opC1ErQivGehC1kww2irJgXNBTWlBNFTrsiRKc103utWWa6JaSVnd8AV6-OMOU91Dkw8Zo-mqIbrexFMVjKv-O97tq104VhlBJZcZcHsGxPA9QRqrQ5iiz5mr_E7OtWRC8R9rQXHx</recordid><startdate>20180101</startdate><enddate>20180101</enddate><creator>Zeng, Yi</creator><creator>Chen, Weibing</creator><creator>Tang, Bin</creator><creator>Liao, Jianhui</creator><creator>Lou, Jun</creator><creator>Chen, Qing</creator><general>Royal Society of Chemistry</general><general>The Royal Society of Chemistry</general><scope>7SR</scope><scope>8BQ</scope><scope>8FD</scope><scope>JG9</scope><scope>5PM</scope></search><sort><creationdate>20180101</creationdate><title>Synergetic photoluminescence enhancement of monolayer MoS2via surface plasmon resonance and defect repair</title><author>Zeng, Yi ; Chen, Weibing ; Tang, Bin ; Liao, Jianhui ; Lou, Jun ; Chen, Qing</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-j185e-bc647c46b803b2e947b2621f873e3361a5ce6d1995508939bd9f9c3908f712bd3</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2018</creationdate><topic>Chemistry</topic><topic>Electromagnetic fields</topic><topic>Excitation spectra</topic><topic>Gold</topic><topic>Molybdenum disulfide</topic><topic>Monolayers</topic><topic>Optoelectronic devices</topic><topic>Photoluminescence</topic><topic>Self-assembly</topic><topic>Surface plasmon resonance</topic><topic>Trifluoromethane</topic><topic>Trions</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Zeng, Yi</creatorcontrib><creatorcontrib>Chen, Weibing</creatorcontrib><creatorcontrib>Tang, Bin</creatorcontrib><creatorcontrib>Liao, Jianhui</creatorcontrib><creatorcontrib>Lou, Jun</creatorcontrib><creatorcontrib>Chen, Qing</creatorcontrib><collection>Engineered Materials Abstracts</collection><collection>METADEX</collection><collection>Technology Research Database</collection><collection>Materials Research Database</collection><collection>PubMed Central (Full Participant titles)</collection><jtitle>RSC advances</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Zeng, Yi</au><au>Chen, Weibing</au><au>Tang, Bin</au><au>Liao, Jianhui</au><au>Lou, Jun</au><au>Chen, Qing</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Synergetic photoluminescence enhancement of monolayer MoS2via surface plasmon resonance and defect repair</atitle><jtitle>RSC advances</jtitle><date>2018-01-01</date><risdate>2018</risdate><volume>8</volume><issue>42</issue><spage>23591</spage><epage>23598</epage><pages>23591-23598</pages><eissn>2046-2069</eissn><abstract>The weak light-absorption and low quantum yield (QY) in monolayer MoS2 are great challenges for the applications of this material in practical optoelectronic devices. 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subjects | Chemistry Electromagnetic fields Excitation spectra Gold Molybdenum disulfide Monolayers Optoelectronic devices Photoluminescence Self-assembly Surface plasmon resonance Trifluoromethane Trions |
title | Synergetic photoluminescence enhancement of monolayer MoS2via surface plasmon resonance and defect repair |
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