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Facile fabrication and luminescence properties of a new Zn coordination polymer-based fluorescent sensor toward antibiotics
Due to the excellent fluorescence properties of organic fluorescent ligand 4,7-bi(1 H -imidazol-1-yl)benzo-[2,1,3]thiadiazole (BIBT), luminescent coordination polymers (CPs) or metalorganic frameworks constructed from BIBT have received our attention. In this work, by the self-assembly of BIBT and Z...
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Published in: | New journal of chemistry 2022-11, Vol.46 (43), p.2623-2628 |
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container_title | New journal of chemistry |
container_volume | 46 |
creator | Wang, Jin-Jin Li, Le-Qian Zhu, Zi-Hao Zheng, Teng-Fei Xu, Hui Peng, Yan Chen, Jing-Lin Liu, Sui-Jun Wen, He-Rui |
description | Due to the excellent fluorescence properties of organic fluorescent ligand 4,7-bi(1
H
-imidazol-1-yl)benzo-[2,1,3]thiadiazole (BIBT), luminescent coordination polymers (CPs) or metalorganic frameworks constructed from BIBT have received our attention. In this work, by the self-assembly of BIBT and Zn(
ii
) ions, the formation of a two-dimensional (2D) CP with a formula [Zn
2
(BIBT)(AIPA)
2
]
n
(
JXUST-17
, H
2
AIPA = 5-aminoisophthalic acid) has been achieved. X-ray single-crystal diffraction analysis reveals that the adjacent Zn
II
ions are connected by amino and carboxylate groups from AIPA
2
ligands to form a 2D layer structure and the neighboring layers are further linked by BIBT ligands to construct a 2D double-layer structure. Luminescence investigation suggests that
JXUST-17
not only possesses excellent detection capability but also exhibits excellent selectivity toward nitrofurantoin (NFT) and 2.6-dichloro-4-nitroaniline (DCN). Furthermore, mixed matrix membranes are developed by the dispersion of
JXUST-17
with polymethyl methacrylate in DMA solution to realize a rapid and visualizable luminescence response towards NFT.
A new Zn
II
-based coordination polymer could selectively and sensitively recognize NFT and DCN
via
turn-off effect. Interestingly, a mixed matrix film for visualizable sensing has been successfully developed. |
doi_str_mv | 10.1039/d2nj03797a |
format | article |
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H
-imidazol-1-yl)benzo-[2,1,3]thiadiazole (BIBT), luminescent coordination polymers (CPs) or metalorganic frameworks constructed from BIBT have received our attention. In this work, by the self-assembly of BIBT and Zn(
ii
) ions, the formation of a two-dimensional (2D) CP with a formula [Zn
2
(BIBT)(AIPA)
2
]
n
(
JXUST-17
, H
2
AIPA = 5-aminoisophthalic acid) has been achieved. X-ray single-crystal diffraction analysis reveals that the adjacent Zn
II
ions are connected by amino and carboxylate groups from AIPA
2
ligands to form a 2D layer structure and the neighboring layers are further linked by BIBT ligands to construct a 2D double-layer structure. Luminescence investigation suggests that
JXUST-17
not only possesses excellent detection capability but also exhibits excellent selectivity toward nitrofurantoin (NFT) and 2.6-dichloro-4-nitroaniline (DCN). Furthermore, mixed matrix membranes are developed by the dispersion of
JXUST-17
with polymethyl methacrylate in DMA solution to realize a rapid and visualizable luminescence response towards NFT.
A new Zn
II
-based coordination polymer could selectively and sensitively recognize NFT and DCN
via
turn-off effect. Interestingly, a mixed matrix film for visualizable sensing has been successfully developed.</description><identifier>ISSN: 1144-0546</identifier><identifier>EISSN: 1369-9261</identifier><identifier>DOI: 10.1039/d2nj03797a</identifier><language>eng</language><ispartof>New journal of chemistry, 2022-11, Vol.46 (43), p.2623-2628</ispartof><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,27924,27925</link.rule.ids></links><search><creatorcontrib>Wang, Jin-Jin</creatorcontrib><creatorcontrib>Li, Le-Qian</creatorcontrib><creatorcontrib>Zhu, Zi-Hao</creatorcontrib><creatorcontrib>Zheng, Teng-Fei</creatorcontrib><creatorcontrib>Xu, Hui</creatorcontrib><creatorcontrib>Peng, Yan</creatorcontrib><creatorcontrib>Chen, Jing-Lin</creatorcontrib><creatorcontrib>Liu, Sui-Jun</creatorcontrib><creatorcontrib>Wen, He-Rui</creatorcontrib><title>Facile fabrication and luminescence properties of a new Zn coordination polymer-based fluorescent sensor toward antibiotics</title><title>New journal of chemistry</title><description>Due to the excellent fluorescence properties of organic fluorescent ligand 4,7-bi(1
H
-imidazol-1-yl)benzo-[2,1,3]thiadiazole (BIBT), luminescent coordination polymers (CPs) or metalorganic frameworks constructed from BIBT have received our attention. In this work, by the self-assembly of BIBT and Zn(
ii
) ions, the formation of a two-dimensional (2D) CP with a formula [Zn
2
(BIBT)(AIPA)
2
]
n
(
JXUST-17
, H
2
AIPA = 5-aminoisophthalic acid) has been achieved. X-ray single-crystal diffraction analysis reveals that the adjacent Zn
II
ions are connected by amino and carboxylate groups from AIPA
2
ligands to form a 2D layer structure and the neighboring layers are further linked by BIBT ligands to construct a 2D double-layer structure. Luminescence investigation suggests that
JXUST-17
not only possesses excellent detection capability but also exhibits excellent selectivity toward nitrofurantoin (NFT) and 2.6-dichloro-4-nitroaniline (DCN). Furthermore, mixed matrix membranes are developed by the dispersion of
JXUST-17
with polymethyl methacrylate in DMA solution to realize a rapid and visualizable luminescence response towards NFT.
A new Zn
II
-based coordination polymer could selectively and sensitively recognize NFT and DCN
via
turn-off effect. Interestingly, a mixed matrix film for visualizable sensing has been successfully developed.</description><issn>1144-0546</issn><issn>1369-9261</issn><fulltext>true</fulltext><rsrctype>article</rsrctype><creationdate>2022</creationdate><recordtype>article</recordtype><sourceid/><recordid>eNpFkMtKAzEYRoMoWKsb90JeYDS3ySRLKdYKBTdduSl_bpAyTYYkpRRf3mIFV9_ZnLP4EHqk5JkSrl8cSzvCBz3AFZpRLnWnmaTXZ6ZCdKQX8hbd1bojhNJB0hn6XoKNo8cBTIkWWswJQ3J4POxj8tX6ZD2eSp58adFXnAMGnPwRfyVscy4upos05fG096UzUL3DYTzk8qs3XH2queCWj1DcOd6iiblFW-_RTYCx-oe_naPN8m2zWHXrz_ePxeu6K5q1LlChmPCDJJJoQoUJyhhJiSVakj4YHhgo43qm5EAVtwIo01w75QMBrgY-R0-XbKl2O5W4h3La_h_FfwAmB17T</recordid><startdate>20221107</startdate><enddate>20221107</enddate><creator>Wang, Jin-Jin</creator><creator>Li, Le-Qian</creator><creator>Zhu, Zi-Hao</creator><creator>Zheng, Teng-Fei</creator><creator>Xu, Hui</creator><creator>Peng, Yan</creator><creator>Chen, Jing-Lin</creator><creator>Liu, Sui-Jun</creator><creator>Wen, He-Rui</creator><scope/></search><sort><creationdate>20221107</creationdate><title>Facile fabrication and luminescence properties of a new Zn coordination polymer-based fluorescent sensor toward antibiotics</title><author>Wang, Jin-Jin ; Li, Le-Qian ; Zhu, Zi-Hao ; Zheng, Teng-Fei ; Xu, Hui ; Peng, Yan ; Chen, Jing-Lin ; Liu, Sui-Jun ; Wen, He-Rui</author></sort><facets><frbrtype>5</frbrtype><frbrgroupid>cdi_FETCH-LOGICAL-r92t-f14824e760609014bf8bb610c09605fb3f2a8bd52867183c4a12939d8ef0a3873</frbrgroupid><rsrctype>articles</rsrctype><prefilter>articles</prefilter><language>eng</language><creationdate>2022</creationdate><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Wang, Jin-Jin</creatorcontrib><creatorcontrib>Li, Le-Qian</creatorcontrib><creatorcontrib>Zhu, Zi-Hao</creatorcontrib><creatorcontrib>Zheng, Teng-Fei</creatorcontrib><creatorcontrib>Xu, Hui</creatorcontrib><creatorcontrib>Peng, Yan</creatorcontrib><creatorcontrib>Chen, Jing-Lin</creatorcontrib><creatorcontrib>Liu, Sui-Jun</creatorcontrib><creatorcontrib>Wen, He-Rui</creatorcontrib><jtitle>New journal of chemistry</jtitle></facets><delivery><delcategory>Remote Search Resource</delcategory><fulltext>fulltext</fulltext></delivery><addata><au>Wang, Jin-Jin</au><au>Li, Le-Qian</au><au>Zhu, Zi-Hao</au><au>Zheng, Teng-Fei</au><au>Xu, Hui</au><au>Peng, Yan</au><au>Chen, Jing-Lin</au><au>Liu, Sui-Jun</au><au>Wen, He-Rui</au><format>journal</format><genre>article</genre><ristype>JOUR</ristype><atitle>Facile fabrication and luminescence properties of a new Zn coordination polymer-based fluorescent sensor toward antibiotics</atitle><jtitle>New journal of chemistry</jtitle><date>2022-11-07</date><risdate>2022</risdate><volume>46</volume><issue>43</issue><spage>2623</spage><epage>2628</epage><pages>2623-2628</pages><issn>1144-0546</issn><eissn>1369-9261</eissn><abstract>Due to the excellent fluorescence properties of organic fluorescent ligand 4,7-bi(1
H
-imidazol-1-yl)benzo-[2,1,3]thiadiazole (BIBT), luminescent coordination polymers (CPs) or metalorganic frameworks constructed from BIBT have received our attention. In this work, by the self-assembly of BIBT and Zn(
ii
) ions, the formation of a two-dimensional (2D) CP with a formula [Zn
2
(BIBT)(AIPA)
2
]
n
(
JXUST-17
, H
2
AIPA = 5-aminoisophthalic acid) has been achieved. X-ray single-crystal diffraction analysis reveals that the adjacent Zn
II
ions are connected by amino and carboxylate groups from AIPA
2
ligands to form a 2D layer structure and the neighboring layers are further linked by BIBT ligands to construct a 2D double-layer structure. Luminescence investigation suggests that
JXUST-17
not only possesses excellent detection capability but also exhibits excellent selectivity toward nitrofurantoin (NFT) and 2.6-dichloro-4-nitroaniline (DCN). Furthermore, mixed matrix membranes are developed by the dispersion of
JXUST-17
with polymethyl methacrylate in DMA solution to realize a rapid and visualizable luminescence response towards NFT.
A new Zn
II
-based coordination polymer could selectively and sensitively recognize NFT and DCN
via
turn-off effect. Interestingly, a mixed matrix film for visualizable sensing has been successfully developed.</abstract><doi>10.1039/d2nj03797a</doi><tpages>6</tpages></addata></record> |
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language | eng |
recordid | cdi_rsc_primary_d2nj03797a |
source | Royal Society of Chemistry |
title | Facile fabrication and luminescence properties of a new Zn coordination polymer-based fluorescent sensor toward antibiotics |
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