A plasmon ruler based on nanoscale photothermal effect

The determination of nanoscale distances or distance changes necessitates a nanoscale ruler. In the present paper, distance dependence of particle temperature in an optically heated gold nanoparticle pair is quantitatively investigated to explore the possibility of creating a plasmon ruler based on...

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Bibliographic Details
Published in:Optics express 2013-01, Vol.21 (1), p.172-181
Main Authors: Zhang, Weichun, Li, Qiang, Qiu, Min
Format: Article
Language:English
Subjects:
Cancer
Gold Nanoparticles
Heat
Metal Nanoparticles
Nanostructures
Particles
Resonances
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Summary:The determination of nanoscale distances or distance changes necessitates a nanoscale ruler. In the present paper, distance dependence of particle temperature in an optically heated gold nanoparticle pair is quantitatively investigated to explore the possibility of creating a plasmon ruler based on this effect. The two origins of the distance-dependence, i.e., electromagnetic coupling and thermal accumulative effect, are studied. For the particle temperature, a scaling behavior is found, and it suggests that the decay of particle temperature with the interparticle gap for different particle sizes follows a common exponential decay equation. This scaling behavior is qualitatively explained with a simple dipolar-coupling model combined with a point heat source interaction model. On the basis of this scaling behavior of absorption power, we further establish a plasmon ruler equation relating the particle temperature and the interparticle distance. Our findings can serve as an excellent guideline for designing and optimizing temperature-based plasmon rulers.
ISSN:1094-4087
1094-4087
DOI:10.1364/OE.21.000172