Development of a model for radionuclide transport in streams for biosphere assessment purpose

• Published in: Journal of environmental radioactivity 2023-08, Vol.264, p.107188-107188, Article 107188
• Main Authors: Xu, Shulan, Dverstorp, Björn, Guerfi, Reda, Wörman, Anders, Riml, Joakim, Kłos, Richard
• Format: Article
• Language: English
• Subjects: Biosphere assessment models; Deep groundwater upwelling; Geological repository; Hyporheic exchange flow; Long-term radiological assessment
• ISSN: 0265-931X; 1879-1700; 1879-1700
• DOI: 10.1016/j.jenvrad.2023.107188

As a part of the overall safety assessment for a geological disposal of radioactive waste, models for different ecosystems are used to evaluate doses to humans and biota from possible radionuclide discharges to the biosphere. In previous safety assessments, transport modelling of radionuclides in running waters such as streams has been much simplified to the extent that only dilution of the inflow of radionuclides has been considered with no regard of any other interactions. Hyporheic exchange flow (HEF) is the flow of surface water in streams that enters the subsurface zone and, after some time, returns to the surface. HEF has been studied for decades. Hyporheic exchange and the residence time in the hyporheic zone are key parameters controlling the transport of radionuclides in a stream. Furthermore, recent studies have shown that HEF can reduce the groundwater upwelling area and increase the upwelling velocity in areas closest to the streambed water interface. In this paper, the development of an assessment model describing radionuclide transport with consideration of HEF and deep groundwater upwelling along streams is presented. An approach to parameterising the hyporheic exchange processes into an assessment model is based on a comprehensive study that has been performed in five different Swedish catchments. Sensitivity analyses are performed to explore the effect with consideration of the inflow of radionuclides with regard to HEF and deep groundwater upwelling in a safety assessment perspective. Finally, we include some suggestions for the application of the assessment model to long-term radiological safety assessments. •Investigation of the effect of hyporheic exchange flow on solute transport in streams for long-term safety assessments.•Utilizing national databases to develop assessment models for radiological safety assessment purposes.•Illustration of the effect of discretization on the behavior of the compartmental model.