Comparison of measured residential black carbon levels outdoors and indoors with fixed-site monitoring data and with dispersion modelling

• Published in: Environmental science and pollution research international 2021-04, Vol.28 (13), p.16264-16271
• Main Authors: Gruzieva, Olena, Georgelis, Antonios, Andersson, Niklas, Bellander, Tom, Johansson, Christer, Merritt, Anne-Sophie
• Format: Article
• Language: English
• Subjects: Air Pollutants - analysis; Air pollution; Air Pollution - analysis; Air pollution effects; Air Pollution, Indoor - analysis; Aquatic Pollution; Atmospheric Protection/Air Quality Control/Air Pollution; Background levels; Black carbon; Carbon; Carbon - analysis; Dispersion; Dispersion modelling; Earth and Environmental Science; Ecotoxicology; Environment; Environmental Chemistry; Environmental Health; Environmental Monitoring; Environmental science; Epidemiology; Humans; Indoor; Indoor air pollution; Indoor environments; Mathematical models; Medicin och hälsovetenskap; Modelling; outdoor ratio; Outdoors; Pollution monitoring; Research Article; Routine monitoring; Temporal variations; Time series; Variability; Waste Water Technology; Water Management; Water Pollution Control
• ISSN: 0944-1344; 1614-7499; 1614-7499
• DOI: 10.1007/s11356-020-12134-8

Epidemiologic studies on health effects of air pollution usually rely on time-series of ambient monitoring data or on spatially modelled levels. Little is known how well these estimate residential outdoor and indoor levels. We investigated the agreement of measured residential black carbon (BC) levels outdoors and indoors with fixed-site monitoring data and with levels calculated using a Gaussian dispersion model. One-week residential outdoor and indoor BC measurements were conducted for 15 families living in central Stockholm. Time-series from urban background and street-level monitors were compared to these measurements. The observed weekly concentrations were also standardized to reflect annual averages, using urban background levels, and compared spatially to long-term levels as estimated by dispersion modelling. Weekly average outdoor BC level was 472 ng/m 3 (range 261–797 ng/m 3 ). The corresponding fixed-site urban background and street levels were 313 and 1039 ng/m 3 , respectively. Urban background variation explained 50% of the temporal variation in residential outdoor levels averaged over 24 h. Modelled residential long-term outdoor levels were on average comparable with the standardized measured home outdoor levels, and explained 49% of the spatial variability. The median indoor/outdoor ratio across all addresses was 0.79, with no difference between day and night time. Common exposure estimation approaches in the epidemiology of health effects related to BC displayed high validity for residencies in central Stockholm. Urban background monitored levels explained half of the outdoor day-to-day variability at residential addresses. Long-term dispersion modelling explained half of the spatial differences in outdoor levels. Indoor BC concentrations tended to be somewhat lower than outdoor levels.