Heterogeneous Catalysis for CO2 Conversion into Chemicals and Fuels

Catalytic conversion of CO 2 into chemicals and fuels is a viable method to reduce carbon emissions and achieve carbon neutrality. Through thermal catalysis, electrocatalysis, and photo(electro)catalysis, CO 2 can be converted into a wide range of valuable products, including CO, formic acid, methan...

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Bibliographic Details
Published in:Transactions of Tianjin University 2022-08, Vol.28 (4), p.245-264
Main Authors: Gao, Dunfeng, Li, Wanjun, Wang, Hanyu, Wang, Guoxiong, Cai, Rui
Format: Article
Language:English
Subjects:
Acetic acid
Alkenes
Carbon dioxide
Catalytic converters
Conversion
Density functional theory
Engineering
Ethanol
Fine chemicals
Formic acid
Humanities and Social Sciences
Mechanical Engineering
multidisciplinary
Review
Science
Selectivity
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Summary:Catalytic conversion of CO 2 into chemicals and fuels is a viable method to reduce carbon emissions and achieve carbon neutrality. Through thermal catalysis, electrocatalysis, and photo(electro)catalysis, CO 2 can be converted into a wide range of valuable products, including CO, formic acid, methanol, methane, ethanol, acetic acid, propanol, light olefins, aromatics, and gasoline, as well as fine chemicals. In this mini-review, we summarize the recent progress in heterogeneous catalysis for CO 2 conversion into chemicals and fuels and highlight some representative studies of different conversion routes. The structure–performance correlations of typical catalytic materials used for the CO 2 conversion reactions have been revealed by combining advanced in situ/operando spectroscopy and microscopy characterizations and density functional theory calculations. Catalytic selectivity toward a single CO 2 reduction product/fraction should be further improved at an industrially relevant CO 2 conversion rate with considerable stability in the future. Graphical Abstract
ISSN:1006-4982
1995-8196
DOI:10.1007/s12209-022-00326-x