2020 Roadmap on two-dimensional nanomaterials for environmental catalysis

• Published in: Chinese chemical letters 2019-12, Vol.30 (12), p.2065-2088
• Main Authors: Yang, Yulu, Wu, Mingguang, Zhu, Xingwang, Xu, Hui, Ma, Si, Zhi, Yongfeng, Xia, Hong, Liu, Xiaoming, Pan, Jun, Tang, Jie-Yinn, Chai, Siang-Piao, Palmisano, Leonardo, Parrino, Francesco, Liu, Junli, Ma, Jianzhong, Wang, Ze-Lin, Tan, Ling, Zhao, Yu-Fei, Song, Yu-Fei, Singh, Pardeep, Raizada, Pankaj, Jiang, Deli, Li, Di, Geioushy, R.A., Ma, Jizhen, Zhang, Jintao, Hu, Song, Feng, Rongjuan, Liu, Gang, Liu, Minghua, Li, Zhenhua, Shao, Mingfei, Li, Neng, Peng, Jiahe, Ong, Wee-Jun, Kornienko, Nikolay, Xing, Zhenyu, Fan, Xiujun, Ma, Jianmin
• Format: Article
• Language: English
• Subjects: Black phosphorus; C3N4; Graphene; Metal organic frameworks; MXenes; Two-dimensional materials
• ISSN: 1001-8417; 1878-5964
• DOI: 10.1016/j.cclet.2019.11.001

This roadmap demonstrates a series of two-dimensional nanomaterials, such as graphene, black phosphorus, oxides, layered double hydroxides, chalcogenides, bismuth-based layered compounds, MXenes, metal organic frameworks, covalent organic frameworks, and others, for environmental catalysis. [Display omitted] Environmental catalysis has drawn a great deal of attention due to its clean ways to produce useful chemicals or carry out some chemical processes. Photocatalysis and electrocatalysis play important roles in these fields. They can decompose and remove organic pollutants from the aqueous environment, and prepare some fine chemicals. Moreover, they also can carry out some important reactions, such as O2 reduction reaction (ORR), O2 evolution reaction (OER), H2 evolution reaction (HER), CO2 reduction reaction (CO2RR), and N2 fixation (NRR). For catalytic reactions, it is the key to develop high-performance catalysts to meet the demand for targeted reactions. In recent years, two-dimensional (2D) materials have attracted great interest in environmental catalysis due to their unique layered structures, which offer us to make use of their electronic and structural characteristics. Great progress has been made so far, including graphene, black phosphorus, oxides, layered double hydroxides (LDHs), chalcogenides, bismuth-based layered compounds, MXenes, metal organic frameworks (MOFs), covalent organic frameworks (COFs), and others. This content drives us to invite many famous groups in these fields to write the roadmap on two-dimensional nanomaterials for environmental catalysis. We hope that this roadmap can give the useful guidance to researchers in future researches, and provide the research directions.