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Effective radiation field model to scattering - absorption applied in heterogeneous photocatalytic reactors

A new mathematical model for the calculation of the radiation field in heterogeneous photocatalytic reactors using the new concept of ‘‘effective radiation field model’’ or ERFM is proposed. In this concept, the incident radiation associated to the photons flow is an energy cloud. The generated spac...

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Main Authors: Miguel Angel Mueses, Fiderman Machuca-Martinez, Aracely Hernandez-Ramirez, Gianluca Li-Puma
Format: Default Article
Published: 2015
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Online Access:https://hdl.handle.net/2134/19053
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author Miguel Angel Mueses
Fiderman Machuca-Martinez
Aracely Hernandez-Ramirez
Gianluca Li-Puma
author_facet Miguel Angel Mueses
Fiderman Machuca-Martinez
Aracely Hernandez-Ramirez
Gianluca Li-Puma
author_sort Miguel Angel Mueses (7128200)
collection Figshare
description A new mathematical model for the calculation of the radiation field in heterogeneous photocatalytic reactors using the new concept of ‘‘effective radiation field model’’ or ERFM is proposed. In this concept, the incident radiation associated to the photons flow is an energy cloud. The generated space-phase and the properties of the cloud are considered isotropic and independent of the propagation angle and photon frequency. The isotropic nature of the ERFM concept provides a simple estimation of the radiation field of a catalyst in suspension (particles and fluid) for polychromatic radiation and the solar spectrum. The ERFM is an alternative model for the calculus of the radiant energy distribution in heterogeneous photocatalytic reactors as an extension of concept to the overall volumetric rate photon absorption – OVRPA. The local volumetric rate of photon absorption (LVRPA) predicted by the ERFM were compared with the Six Flux Model (SFM) and the rigorous solution using Discrete Ordinate Method (DOM) for the radiative transfer equation (RTE). The calculated LVRPA with the ERFM was found to be closer to the solution of the RTE-DOM. These results were attributed to the performance of the phase function in both models.
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institution Loughborough University
publishDate 2015
record_format Figshare
spelling rr-article-92433832015-01-01T00:00:00Z Effective radiation field model to scattering - absorption applied in heterogeneous photocatalytic reactors Miguel Angel Mueses (7128200) Fiderman Machuca-Martinez (7128203) Aracely Hernandez-Ramirez (7129751) Gianluca Li-Puma (1252566) Chemical engineering not elsewhere classified Radiation field SFM LVRPA Solar photoreactors Photocatalyst Chemical Engineering not elsewhere classified A new mathematical model for the calculation of the radiation field in heterogeneous photocatalytic reactors using the new concept of ‘‘effective radiation field model’’ or ERFM is proposed. In this concept, the incident radiation associated to the photons flow is an energy cloud. The generated space-phase and the properties of the cloud are considered isotropic and independent of the propagation angle and photon frequency. The isotropic nature of the ERFM concept provides a simple estimation of the radiation field of a catalyst in suspension (particles and fluid) for polychromatic radiation and the solar spectrum. The ERFM is an alternative model for the calculus of the radiant energy distribution in heterogeneous photocatalytic reactors as an extension of concept to the overall volumetric rate photon absorption – OVRPA. The local volumetric rate of photon absorption (LVRPA) predicted by the ERFM were compared with the Six Flux Model (SFM) and the rigorous solution using Discrete Ordinate Method (DOM) for the radiative transfer equation (RTE). The calculated LVRPA with the ERFM was found to be closer to the solution of the RTE-DOM. These results were attributed to the performance of the phase function in both models. 2015-01-01T00:00:00Z Text Journal contribution 2134/19053 https://figshare.com/articles/journal_contribution/Effective_radiation_field_model_to_scattering_-_absorption_applied_in_heterogeneous_photocatalytic_reactors/9243383 CC BY-NC-ND 4.0
spellingShingle Chemical engineering not elsewhere classified
Radiation field
SFM
LVRPA
Solar photoreactors
Photocatalyst
Chemical Engineering not elsewhere classified
Miguel Angel Mueses
Fiderman Machuca-Martinez
Aracely Hernandez-Ramirez
Gianluca Li-Puma
Effective radiation field model to scattering - absorption applied in heterogeneous photocatalytic reactors
title Effective radiation field model to scattering - absorption applied in heterogeneous photocatalytic reactors
title_full Effective radiation field model to scattering - absorption applied in heterogeneous photocatalytic reactors
title_fullStr Effective radiation field model to scattering - absorption applied in heterogeneous photocatalytic reactors
title_full_unstemmed Effective radiation field model to scattering - absorption applied in heterogeneous photocatalytic reactors
title_short Effective radiation field model to scattering - absorption applied in heterogeneous photocatalytic reactors
title_sort effective radiation field model to scattering - absorption applied in heterogeneous photocatalytic reactors
topic Chemical engineering not elsewhere classified
Radiation field
SFM
LVRPA
Solar photoreactors
Photocatalyst
Chemical Engineering not elsewhere classified
url https://hdl.handle.net/2134/19053