POD-DEIM for efficient reduction of a dynamic 2D catalytic reactor model

•Detailed, dynamic, two-dimensional reactor model for catalytic carbon dioxide methanation, with close connection to real world application.•POD-DEIM applied to the highly nonlinear reactor model based on partial differential equations.•Special treatment of POD-DEIM for models with a various number...

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Bibliographic Details
Published in:Computers & chemical engineering 2017-11, Vol.106, p.777-784
Main Authors: Bremer, Jens, Goyal, Pawan, Feng, Lihong, Benner, Peter, Sundmacher, Kai
Format: Article
Language:English
Subjects:
Catalytic reactor
Empirical interpolation methods
Methanation
Nonlinear model reduction
Proper orthogonal decomposition
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Summary:•Detailed, dynamic, two-dimensional reactor model for catalytic carbon dioxide methanation, with close connection to real world application.•POD-DEIM applied to the highly nonlinear reactor model based on partial differential equations.•Special treatment of POD-DEIM for models with a various number of nonlinearities.•Very accurate reduced models, even under different real world operation scenarios.•Reduced models are at least by one order of magnitude faster to evaluate than the original model. Many computational difficulties in dealing with chemical process models often result from spatially distributed states as well as nonlinear correlations (e.g., for transport coefficients or reaction kinetics). Surrogate models with sufficient accuracy represent one remedy to this problem. Featuring a lower number of states, model order reduction (MOR) generates considerably less complex models and leads to faster model evaluations. Especially for nonlinear systems, snapshot-based MOR techniques are considered to be one of the most promising methods. In this study, we apply proper orthogonal decomposition together with the discrete empirical interpolation method (POD-DEIM) to a dynamic, two-dimensional reactor model for catalytic carbon dioxide methanation. Motivated by renewable energy integration, we consider this reactor in two different dynamic scenarios: Disturbed continuous operation and start-up. It can be shown that the reduced order model (ROM) is accurate and, furthermore, the solution of the FOM is accelerated at least by one order of magnitude.
ISSN:0098-1354
1873-4375
DOI:10.1016/j.compchemeng.2017.02.032