Investigation of the complex 3D flow structure within a selective catalytic reduction (SCR) reactor of a coal-fired power plant

• Published in: Experimental thermal and fluid science 2023-10, Vol.148, p.110985, Article 110985
• Main Authors: Han, Joungho, Choi, Woongchul, June Park, Han, Han, Kyuho, Jung, Wonjun, Hwang, Wontae
• Format: Article
• Language: English
• Subjects: denitrification (de-NOx); flow uniformity; magnetic resonance velocimetry (MRV); recirculation zone; Reynolds-averaged Navier-Stokes (RANS); selective catalytic reduction (SCR)
• ISSN: 0894-1777; 1879-2286
• DOI: 10.1016/j.expthermflusci.2023.110985

•Examination of complex 3D flow structure within a coal power plant SCR reactor.•Magnetic resonance velocimetry (MRV) utilized to validate RANS CFD.•Asymmetric recirculation zone observed within the catalytic reactor.•Integral flow parameters were not affected by Reynolds number.•Flow bias caused by recirculation induces uneven de-NOx reactions. A selective catalytic reduction (SCR) reactor is commonly used to remove nitrogen oxides (NOx) from coal-fired boilers. Uniformity of the flow passing through the catalyst layer is important for increasing denitrification (de-NOx) efficiency. In order to examine flow uniformity, this study conducted an experimental and numerical analysis of the complex internal flow within a realistic SCR model. Magnetic resonance velocimetry (MRV) was utilized to obtain non-invasive measurements of three-dimensional three-component average velocity and validate Reynolds-averaged Navier-Stokes (RANS) numerical simulations. The computational results showed similar overall flow structure compared with the MRV results. Parameters representing flow quality such as relative standard deviation (RSD) and recirculation zone strength (RZS) were calculated by integrating the flow field. These parameters have the largest value after the straightener area and decrease towards the catalyst reactor, and are not significantly affected by Reynolds number upstream of the catalyst layer. The recirculation zone size was analyzed using spanwise uniformity and skewness indicators. As the recirculation zone induces biased flow, the non-reacted NOx concentration was more prominent in the outlet zone opposite of the recirculating area in the corresponding actual on-site SCR reactor. Based on this finding, a meaningful correlation between flow maldistribution and de-NOx reaction could be deduced.