Nucleation and bubble growth during puffing and micro-explosions in composite droplets

• Published in: Fuel (Guildford) 2023-05, Vol.340, p.126991, Article 126991
• Main Authors: Bar-Kohany, Tali, Antonov, Dmitrii V., Strizhak, Pavel A., Sazhin, Sergei S.
• Format: Article
• Language: English
• Subjects: Bubble growth; Diesel; Emulsion; Heterogeneous nucleation; Puffing and micro-explosion; Rapid heating
• ISSN: 0016-2361; 1873-7153
• DOI: 10.1016/j.fuel.2022.126991

•Breakup time of droplets is evaluated as the sum of heating and bubble growth times.•Heterogeneous nucleation temperature depends on the heating rate and is often lower than the homogeneous nucleation temperature.•Smaller droplets lead to both shorter heating and bubble growth times.•Higher ambient temperature lead to longer heating times yet shorter bubble growth times.•Heating time is dominant over the bubble growth duration throughout the entire domain, under conductive or natural convection conditions.•For micron-sized droplets, puffing and micro-explosions are prone to occur during the inertial bubble growth regime. Heating of droplets composed of water and fuel is known to lead to internal nucleation and bubble growth that can eventually lead to their puffing and to micro-explosions. The time to puffing/micro-explosions includes times spent on: heating (time to nucleationPleasestriketheSymbolt_Nfromtheabstract), bubble growth Pleasestrike:tgrfromtheabstract. In the present paper, we examine the effect of different aspects of bubble growth on the puffing and micro-explosions. Specifically, we address the effects of nucleation temperature and the relative positions of the inner water sub-droplet and the bubble within it. The nucleation temperature of the water sub-droplet is higher than its normal boiling temperature yet lower than its spinodal temperature in most realistic cases. The degree of superheating and the nucleation time depend on the heating rate and the nucleation site density. Higher nucleation temperatures imply larger driving force for the bubble growth. Bubble growth rate is dominated by the degree of superheating, while growth time is dominated by both the degree of superheating and the location of the bubble with respect to the inner and outer interfaces of the composite droplet. It is found that the inertial bubble growth regime is dominant for micron-sized droplets, and thus sensitivity to the modelling of the inertial regime can be of crucial importance to the evaluation of the breakup time for the droplets. The model for puffing and micro-explosion presented in the paper considers an isolated bubble growing at the water/fuel interface at various degrees of superheating, and for a wide range of Jakob numbers. This analysis allows us to assess the sensitivity of bubble growth time to the initial bubble location, and to generalise the previously developed model of the phenomenon taking into account the effect of finite time of bubbl