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New Measurement of the Thermal-capture Cross Section for the Minor Isotope 180W

Tungsten occurs naturally in five isotopic forms; four of them, 182,183,184,186W, contribute significantly to the overall elemental abundance (with each contribution between 14 and 30 %), whereas 180W only occurs at the 0.12 % level and is a minor isotope. Given its very low abundance, a precise mea...

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Bibliographic Details
Published in:Nuclear data sheets 2014-05, Vol.119, p.91-93
Main Authors: Hurst, A.M., Firestone, R.B., Szentmiklósi, L., Révay, Zs, Basunia, M.S., Belgya, T., Escher, J.E., Krtička, M., Summers, N.C., Sleaford, B.W.
Format: Article
Language:English
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Summary:Tungsten occurs naturally in five isotopic forms; four of them, 182,183,184,186W, contribute significantly to the overall elemental abundance (with each contribution between 14 and 30 %), whereas 180W only occurs at the 0.12 % level and is a minor isotope. Given its very low abundance, a precise measurement of the thermal neutron-capture cross section is extremely challenging. This work reports a new value of the thermal neutron-capture cross section from a direct 180W(n,γ) measurement using a guided-thermal beam at the Budapest Research Reactor, incident upon an 11.35 % enriched sample to induce prompt γ-ray activation within the sample. The thermal-capture cross section was determined as the sum of experimentally observed partial neutron-capture γ-ray cross sections feeding the ground state directly, and, the modeled contribution from the (unobserved) ground-state feeding predicted from statistical-model calculations using the Monte Carlo program DICEBOX. The preliminary value of the 180W(n,γ) thermal neutron-capture cross section is 20.5(42) b.
ISSN:0090-3752
1095-9904
DOI:10.1016/j.nds.2014.08.026