Reducing uncertainties in satellite estimates of aerosol–cloud interactions over the subtropical ocean by integrating vertically resolved aerosol observations

• Published in: Atmospheric chemistry and physics 2020-06, Vol.20 (12), p.7167-7177
• Main Authors: Painemal, David, Chang, Fu-Lung, Ferrare, Richard, Burton, Sharon, Li, Zhujun, Smith Jr., William L, Minnis, Patrick, Feng, Yan, Clayton, Marian
• Format: Article
• Language: English
• Subjects: Aerosol concentrations; Aerosol effects; Aerosol extinction; Aerosol observations; Aerosol optical depth; Aerosol-cloud interactions; Aerosols; Algorithms; CALIPSO (Pathfinder satellite); Climate change; Climate models; Cloud condensation nuclei; Cloud droplet concentration; Cloud droplets; Clouds; Clouds (Meteorology); Coefficients; Condensation nuclei; Correlation; Datasets; Global climate; Global climate models; INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY; Lidar; Meteorological satellites; MODIS; Optical analysis; Optical thickness; Quartiles; Remote sensing; Satellite observation; Satellites; Sensors; Spectroradiometers; Studies; Uncertainty
• ISSN: 1680-7324; 1680-7316; 1680-7324
• DOI: 10.5194/acp-20-7167-2020

Satellite quantification of aerosol effects on clouds relies on aerosol optical depth (AOD) as a proxy for aerosol concentration or cloud condensation nuclei (CCN). However, the lack of error characterization of satellite-based results hampers their use for the evaluation and improvement of global climate models. We show that the use of AOD for assessing aerosol–cloud interactions (ACIs) is inadequate over vast oceanic areas in the subtropics. Instead, we postulate that a more physical approach that consists of matching vertically resolved aerosol data from the Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observations (CALIPSO) satellite at the cloud-layer height with Moderate Resolution Imaging Spectroradiometer (MODIS) Aqua cloud retrievals reduces uncertainties in satellite-based ACI estimates. Combined aerosol extinction coefficients (σ) below cloud top (σBC) from the Cloud-Aerosol Lidar with Orthogonal Polarization (CALIOP) and cloud droplet number concentrations (Nd) from MODIS Aqua yield high correlations across a broad range of σBC values, with σBC quartile correlations ≥0.78. In contrast, CALIOP-based AOD yields correlations with MODIS Nd of 0.54–0.62 for the two lower AOD quartiles. Moreover, σBC explains 41 % of the spatial variance in MODIS Nd, whereas AOD only explains 17 %, primarily caused by the lack of spatial covariability in the eastern Pacific. Compared with σBC, near-surface σ weakly correlates in space with MODIS Nd, accounting for a 16 % variance. It is concluded that the linear regression calculated from ln(Nd)–ln(σBC) (the standard method for quantifying ACIs) is more physically meaningful than that derived from the Nd–AOD pair.