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Controlling the Scattering Length of Ultracold Dipolar Molecules

By applying a circularly polarized and slightly blue-detuned microwave field with respect to the first excited rotational state of a dipolar molecule, one can engineer a long-range, shallow potential well in the entrance channel of the two colliding partners. As the applied microwave ac field is inc...

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Bibliographic Details
Published in:Physical review letters 2018-10, Vol.121 (16), p.163402-163402, Article 163402
Main Authors: Lassablière, Lucas, Quéméner, Goulven
Format: Article
Language:English
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Summary:By applying a circularly polarized and slightly blue-detuned microwave field with respect to the first excited rotational state of a dipolar molecule, one can engineer a long-range, shallow potential well in the entrance channel of the two colliding partners. As the applied microwave ac field is increased, the long-range well becomes deeper and can support a certain number of bound states, which in turn bring the value of the molecule-molecule scattering length from a large negative value to a large positive one. We adopt an adimensional approach where the molecules are described by a rescaled rotational constant B[over ˜]=B/s_{E_{3}} where s_{E_{3}} is a characteristic dipolar energy. We found that molecules with B[over ˜]>10^{8} are immune to any quenching losses when a sufficient ac field is applied, the ratio elastic to quenching processes can reach values above 10^{3}, and that the value and sign of the scattering length can be tuned. The ability to control the molecular scattering length opens the door for a rich, strongly correlated, many-body physics for ultracold molecules, similar to that for ultracold atoms.
ISSN:0031-9007
1079-7114
DOI:10.1103/PhysRevLett.121.163402