A heat flux sensor leveraging the transverse Seebeck effect in elemental antimony

• Published in: Sensors and actuators. A. Physical. 2023-12, Vol.363 (C), p.114729, Article 114729
• Main Authors: McAfee, Kenneth, Sunderland, Peter B., Rabin, Oded
• Format: Article
• Language: English
• Subjects: anisotropy; antimony; Heat flux sensor; single crystal; thermoelectrics; transverse Seebeck effect
• ISSN: 0924-4247; 1873-3069
• DOI: 10.1016/j.sna.2023.114729

Certain configurations of anisotropic single crystal materials can generate a thermoelectric voltage orthogonal to an induced temperature gradient. This phenomenon is known as the Transverse Seebeck Effect (TSE) and can be leveraged to fabricate simple and robust heat flux sensors. Only a small number of materials have been considered as TSE-based transducers and, among these, few have been developed into sensors with ruggedization against chemical and mechanical degradation. Here, we report on the fabrication and characterization of a rugged TSE-based heat flux sensor using prismatic antimony single crystals. The heat flux sensor was tested under static and dynamic heating scenarios. The sensor has a linear responsivity of 16.8 µV/(W/cm2) to heat fluxes spanning more than two orders of magnitude and a time constant of 4.4s. The sensor’s response to localized heating, probed with a laser scanning technique, validated that the transduction mechanism is primarily the TSE by ruling out a sizable contribution from the conventional Seebeck effect. Finite element analysis corroborated that components used in the sensor package are the primary determinants of the time constant and the decrement of the responsivity from its theoretical maximum. Design principles that may be applied to elicit a faster transient response or higher responsivity are proposed. The results establish single crystal antimony as a promising transducer material for heat flux measurement systems and demonstrate potential effects of ruggedization on sensor performance. [Display omitted] •The transverse Seebeck effect was demonstrated in antimony single crystals•The antimony heat flux sensor has a linear response over the range of 0.06–7W/cm2•The sensor was studied under uniform, localized and time-varying heating scenarios•The sensor has a responsivity of 16.8 μV/(W/cm2) and a time constant of 4.4sec•The package design and its materials affect many aspects of the sensor performance