Emergence of novel phenomena on the border of low dimensional spin and charge order

• Published in: The European physical journal. B, Condensed matter physics Condensed matter physics, 2020-01, Vol.91 (9), Article 196
• Main Authors: Haines, Charles R. S., Saxena, Siddharth S.
• Format: Article
• Language: English
• Subjects: Anisotropy; Antiferromagnetism; Complex Systems; Condensed Matter Physics; Couplings; Crystal structure; Fermions; Ferroalloys; Fluid- and Aerodynamics; Giant magnetoresistance; High temperature; Honeycomb construction; Insulators; Magnetic properties; Magnetism; Magnetoresistance; Magnetoresistivity; Magnets; Physics; Physics and Astronomy; Pressure; Regular Article; Solid State Physics; Spin liquid; Superconductivity; Superconductors; Topical issue: Coexistence of Long-Range Orders in Low-dimensional Systems; Variations
• ISSN: 1434-6028; 1434-6036
• DOI: 10.1140/epjb/e2018-90358-3

Proximity to magnetic order as well as low dimensionality are both beneficial to superconductivity at elevated temperatures. Materials on the border of magnetism display a wide range of novel and potentially useful phenomena: high T c s, heavy fermions, coexistence of magnetism and superconductivity and giant magnetoresistance. Low dimensionality is linked to enhanced fluctuations and, in the case of heavy fermions, has been experimentally shown to be beneficial for the fluctuations that are responsible for the rich abundance of novel emergent phases. This experimental strategy motivated us to explore 2D insulating magnets with a view to investigate phase evolution across metal-insulator and magnetic-non-magnetic boundaries. This has been a fruitful venture with totally novel results different to our expectations. We present results from 2 distinct systems. The MPS 3 family are highly anisotropic in both their crystal and magnetic structures. FePS 3 in particular is a model insulating honeycomb antiferromagnet. We find that the application of pressure to FePS 3 induces an insulator to metal transition. The second system, Cs 2 CuCl 4 , is a highly-frustrated quantum spin liquid at low temperature. The competition of the 3 relevant exchange couplings is delicately balanced. It has been shown to become antiferromagnetic at very low temperatures (~1 K). We have found that the application of pressure for 3 days or more followed by a return to ambient pressure stabilises a totally distinct magnetic ground state.