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Effects of Sulfur Dioxide and Nitric Oxide on Mercury Oxidation and Reduction under Homogeneous Conditions
This paper is particularly related to elemental mercury (Hg 0 ) oxidation and divalent mercury (Hg 2+ ) reduction under simulated flue gas conditions in the presence of nitric oxide (NO) and sulfur dioxide (SO 2 ). As a powerful oxidant and chlorinating reagent, Cl 2 has the potential for Hg oxidati...
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| Published in: | Journal of the Air & Waste Management Association (1995) 2006-05, Vol.56 (5), p.628-635 |
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| Main Authors: | , , , , |
| Format: | Article |
| Language: | English |
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| cited_by | cdi_FETCH-LOGICAL-c628t-e8788f98fb201787e4f81316153b12ed408d9434fec2e78850625ce2aea665333 |
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| cites | cdi_FETCH-LOGICAL-c628t-e8788f98fb201787e4f81316153b12ed408d9434fec2e78850625ce2aea665333 |
| container_end_page | 635 |
| container_issue | 5 |
| container_start_page | 628 |
| container_title | Journal of the Air & Waste Management Association (1995) |
| container_volume | 56 |
| creator | Zhao, Yongxin Mann, Michael D. Olson, Edwin S. Pavlish, John H. Dunham, Grant E. |
| description | This paper is particularly related to elemental mercury (Hg
0
) oxidation and divalent mercury (Hg
2+
) reduction under simulated flue gas conditions in the presence of nitric oxide (NO) and sulfur dioxide (SO
2
). As a powerful oxidant and chlorinating reagent, Cl
2
has the potential for Hg oxidation. However, the detailed mechanism for the interactions, especially among chlorine (Cl)-containing species, SO
2
, NO, as well as H
2
O, remains ambiguous. Research described in this paper therefore focused on the impacts of SO
2
and NO on Hg
0
oxidation and Hg
2+
reduction with the intent of unraveling unrecognized interactions among Cl species, SO
2
, and NO most importantly in the presence of H
2
O. The experimental results demonstrated that SO
2
and NO had pronounced inhibitory effects on Hg
0
oxidation at high temperatures when H
2
O was also present in the gas blend. Such a demonstration was further confirmed by the reduction of Hg
2+
back into its elemental form. Data revealed that SO
2
and NO were capable of promoting homogeneous reduction of Hg
2+
to Hg
0
with H
2
O being present. However, the above inhibition or promotion disappeared under homogeneous conditions when H
2
O was removed from the gas blend. |
| doi_str_mv | 10.1080/10473289.2006.10464483 |
| format | article |
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0
) oxidation and divalent mercury (Hg
2+
) reduction under simulated flue gas conditions in the presence of nitric oxide (NO) and sulfur dioxide (SO
2
). As a powerful oxidant and chlorinating reagent, Cl
2
has the potential for Hg oxidation. However, the detailed mechanism for the interactions, especially among chlorine (Cl)-containing species, SO
2
, NO, as well as H
2
O, remains ambiguous. Research described in this paper therefore focused on the impacts of SO
2
and NO on Hg
0
oxidation and Hg
2+
reduction with the intent of unraveling unrecognized interactions among Cl species, SO
2
, and NO most importantly in the presence of H
2
O. The experimental results demonstrated that SO
2
and NO had pronounced inhibitory effects on Hg
0
oxidation at high temperatures when H
2
O was also present in the gas blend. Such a demonstration was further confirmed by the reduction of Hg
2+
back into its elemental form. Data revealed that SO
2
and NO were capable of promoting homogeneous reduction of Hg
2+
to Hg
0
with H
2
O being present. However, the above inhibition or promotion disappeared under homogeneous conditions when H
2
O was removed from the gas blend.</description><identifier>ISSN: 1096-2247</identifier><identifier>EISSN: 2162-2906</identifier><identifier>DOI: 10.1080/10473289.2006.10464483</identifier><identifier>PMID: 16739799</identifier><identifier>CODEN: JAWAFC</identifier><language>eng</language><publisher>Pittsburgh, PA: Taylor & Francis Group</publisher><subject>Air Pollutants - chemistry ; Applied sciences ; Atmospheric pollution ; Chemical engineering ; Chlorine - chemistry ; Coal ; Environmental impact ; Exact sciences and technology ; General processes of purification and dust removal ; Hazardous materials ; Health aspects ; Mercury ; Mercury - chemistry ; Nitric oxide ; Nitric Oxide - chemistry ; Oxidation ; Oxidation-Reduction ; Oxidation-reduction reaction ; Pollution ; Power Plants ; Prevention and purification methods ; Public health ; Reactors ; Sulfur Dioxide - chemistry</subject><ispartof>Journal of the Air & Waste Management Association (1995), 2006-05, Vol.56 (5), p.628-635</ispartof><rights>Copyright 2006 Air & Waste Management Association 2006</rights><rights>2006 INIST-CNRS</rights><rights>COPYRIGHT 2006 Air and Waste Management Association</rights><rights>Copyright Air and Waste Management Association May 2006</rights><lds50>peer_reviewed</lds50><woscitedreferencessubscribed>false</woscitedreferencessubscribed><citedby>FETCH-LOGICAL-c628t-e8788f98fb201787e4f81316153b12ed408d9434fec2e78850625ce2aea665333</citedby><cites>FETCH-LOGICAL-c628t-e8788f98fb201787e4f81316153b12ed408d9434fec2e78850625ce2aea665333</cites></display><links><openurl>$$Topenurl_article</openurl><openurlfulltext>$$Topenurlfull_article</openurlfulltext><thumbnail>$$Tsyndetics_thumb_exl</thumbnail><link.rule.ids>314,780,784,27924,27925</link.rule.ids><backlink>$$Uhttp://pascal-francis.inist.fr/vibad/index.php?action=getRecordDetail&idt=17771188$$DView record in Pascal Francis$$Hfree_for_read</backlink><backlink>$$Uhttps://www.ncbi.nlm.nih.gov/pubmed/16739799$$D View this record in MEDLINE/PubMed$$Hfree_for_read</backlink></links><search><creatorcontrib>Zhao, Yongxin</creatorcontrib><creatorcontrib>Mann, Michael D.</creatorcontrib><creatorcontrib>Olson, Edwin S.</creatorcontrib><creatorcontrib>Pavlish, John H.</creatorcontrib><creatorcontrib>Dunham, Grant E.</creatorcontrib><title>Effects of Sulfur Dioxide and Nitric Oxide on Mercury Oxidation and Reduction under Homogeneous Conditions</title><title>Journal of the Air & Waste Management Association (1995)</title><addtitle>J Air Waste Manag Assoc</addtitle><description>This paper is particularly related to elemental mercury (Hg
0
) oxidation and divalent mercury (Hg
2+
) reduction under simulated flue gas conditions in the presence of nitric oxide (NO) and sulfur dioxide (SO
2
). As a powerful oxidant and chlorinating reagent, Cl
2
has the potential for Hg oxidation. However, the detailed mechanism for the interactions, especially among chlorine (Cl)-containing species, SO
2
, NO, as well as H
2
O, remains ambiguous. Research described in this paper therefore focused on the impacts of SO
2
and NO on Hg
0
oxidation and Hg
2+
reduction with the intent of unraveling unrecognized interactions among Cl species, SO
2
, and NO most importantly in the presence of H
2
O. The experimental results demonstrated that SO
2
and NO had pronounced inhibitory effects on Hg
0
oxidation at high temperatures when H
2
O was also present in the gas blend. Such a demonstration was further confirmed by the reduction of Hg
2+
back into its elemental form. Data revealed that SO
2
and NO were capable of promoting homogeneous reduction of Hg
2+
to Hg
0
with H
2
O being present. However, the above inhibition or promotion disappeared under homogeneous conditions when H
2
O was removed from the gas blend.</description><subject>Air Pollutants - chemistry</subject><subject>Applied sciences</subject><subject>Atmospheric pollution</subject><subject>Chemical engineering</subject><subject>Chlorine - chemistry</subject><subject>Coal</subject><subject>Environmental impact</subject><subject>Exact sciences and technology</subject><subject>General processes of purification and dust removal</subject><subject>Hazardous materials</subject><subject>Health aspects</subject><subject>Mercury</subject><subject>Mercury - chemistry</subject><subject>Nitric oxide</subject><subject>Nitric Oxide - chemistry</subject><subject>Oxidation</subject><subject>Oxidation-Reduction</subject><subject>Oxidation-reduction reaction</subject><subject>Pollution</subject><subject>Power Plants</subject><subject>Prevention and purification methods</subject><subject>Public health</subject><subject>Reactors</subject><subject>Sulfur Dioxide - 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chemistry</topic><topic>Oxidation</topic><topic>Oxidation-Reduction</topic><topic>Oxidation-reduction reaction</topic><topic>Pollution</topic><topic>Power Plants</topic><topic>Prevention and purification methods</topic><topic>Public health</topic><topic>Reactors</topic><topic>Sulfur Dioxide - chemistry</topic><toplevel>peer_reviewed</toplevel><toplevel>online_resources</toplevel><creatorcontrib>Zhao, Yongxin</creatorcontrib><creatorcontrib>Mann, Michael D.</creatorcontrib><creatorcontrib>Olson, Edwin S.</creatorcontrib><creatorcontrib>Pavlish, John H.</creatorcontrib><creatorcontrib>Dunham, Grant E.</creatorcontrib><collection>Pascal-Francis</collection><collection>Medline</collection><collection>MEDLINE</collection><collection>MEDLINE (Ovid)</collection><collection>MEDLINE</collection><collection>MEDLINE</collection><collection>PubMed</collection><collection>CrossRef</collection><collection>ProQuest Central (Corporate)</collection><collection>Aluminium Industry 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Assoc</addtitle><date>2006-05-01</date><risdate>2006</risdate><volume>56</volume><issue>5</issue><spage>628</spage><epage>635</epage><pages>628-635</pages><issn>1096-2247</issn><eissn>2162-2906</eissn><coden>JAWAFC</coden><abstract>This paper is particularly related to elemental mercury (Hg
0
) oxidation and divalent mercury (Hg
2+
) reduction under simulated flue gas conditions in the presence of nitric oxide (NO) and sulfur dioxide (SO
2
). As a powerful oxidant and chlorinating reagent, Cl
2
has the potential for Hg oxidation. However, the detailed mechanism for the interactions, especially among chlorine (Cl)-containing species, SO
2
, NO, as well as H
2
O, remains ambiguous. Research described in this paper therefore focused on the impacts of SO
2
and NO on Hg
0
oxidation and Hg
2+
reduction with the intent of unraveling unrecognized interactions among Cl species, SO
2
, and NO most importantly in the presence of H
2
O. The experimental results demonstrated that SO
2
and NO had pronounced inhibitory effects on Hg
0
oxidation at high temperatures when H
2
O was also present in the gas blend. Such a demonstration was further confirmed by the reduction of Hg
2+
back into its elemental form. Data revealed that SO
2
and NO were capable of promoting homogeneous reduction of Hg
2+
to Hg
0
with H
2
O being present. However, the above inhibition or promotion disappeared under homogeneous conditions when H
2
O was removed from the gas blend.</abstract><cop>Pittsburgh, PA</cop><pub>Taylor & Francis Group</pub><pmid>16739799</pmid><doi>10.1080/10473289.2006.10464483</doi><tpages>8</tpages></addata></record> |
| fulltext | fulltext |
| identifier | ISSN: 1096-2247 |
| ispartof | Journal of the Air & Waste Management Association (1995), 2006-05, Vol.56 (5), p.628-635 |
| issn | 1096-2247 2162-2906 |
| language | eng |
| recordid | cdi_proquest_journals_214378185 |
| source | Taylor and Francis Science and Technology Collection |
| subjects | Air Pollutants - chemistry Applied sciences Atmospheric pollution Chemical engineering Chlorine - chemistry Coal Environmental impact Exact sciences and technology General processes of purification and dust removal Hazardous materials Health aspects Mercury Mercury - chemistry Nitric oxide Nitric Oxide - chemistry Oxidation Oxidation-Reduction Oxidation-reduction reaction Pollution Power Plants Prevention and purification methods Public health Reactors Sulfur Dioxide - chemistry |
| title | Effects of Sulfur Dioxide and Nitric Oxide on Mercury Oxidation and Reduction under Homogeneous Conditions |
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